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  • Maroju, Praveen KumarLund University,Lunds universitet,LTH profilområde: Avancerade ljuskällor,LTH profilområden,Lunds Tekniska Högskola,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,Albert-Ludwigs University Freiburg (author)

Attosecond coherent control of electronic wave packets in two-colour photoionization using a novel timing tool for seeded free-electron laser

  • Article/chapterEnglish2023

Publisher, publication year, extent ...

  • 2023-01-12
  • Springer Science and Business Media LLC,2023

Numbers

  • LIBRIS-ID:oai:gup.ub.gu.se/324132
  • https://gup.ub.gu.se/publication/324132URI
  • https://doi.org/10.1038/s41566-022-01127-3DOI
  • https://lup.lub.lu.se/record/ab827ea0-c232-461a-8a8d-b9668ed01762URI

Supplementary language notes

  • Language:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • In ultrafast spectroscopy, the temporal resolution of time-resolved experiments depends on the duration of the pump and probe pulses, and on the control and characterization of their relative synchronization. Free-electron lasers operating in the extreme ultraviolet and X-ray spectral regions deliver pulses with femtosecond and attosecond duration in a broad array of pump-probe configurations to study a wide range of physical processes. However, this flexibility, together with the large dimensions and high complexity of the experimental set-ups, limits control of the temporal delay to the femtosecond domain, thus precluding a time resolution below the optical cycle. Here we demonstrate a novel single-shot technique able to determine the relative synchronization between an attosecond pulse train-generated by a seeded free-electron laser-and the optical oscillations of a near-infrared field, with a resolution of one atomic unit (24 as). Using this attosecond timing tool, we report the first example of attosecond coherent control of photoionization in a two-colour field by manipulating the phase of high-order near-infrared transitions.

Subject headings and genre

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  • Di Fraia, M.Elettra Sincrotrone Trieste (author)
  • Plekan, O.Elettra Sincrotrone Trieste (author)
  • Bonanomi, M.Polytechnic University of Milan,CNR Institute for Photonics and Nanotechnologies (IFN-CNR) (author)
  • Merzuk, B.Albert-Ludwigs University Freiburg (author)
  • Busto, DavidLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas,Albert-Ludwigs University Freiburg(Swepub:lu)da4401bu (author)
  • Makos, I.Albert-Ludwigs University Freiburg (author)
  • Schmoll, M.Albert-Ludwigs University Freiburg (author)
  • Shah, R. A.Albert-Ludwigs University Freiburg (author)
  • Ribic, P. R.Elettra Sincrotrone Trieste (author)
  • Giannessi, L.Elettra Sincrotrone Trieste,INFN Frascati National Laboratory (author)
  • De Ninno, G.University of Nova Gorica,Elettra Sincrotrone Trieste (author)
  • Spezzani, C.Elettra Sincrotrone Trieste,University of Nova Gorica (author)
  • Penco, G.Elettra Sincrotrone Trieste (author)
  • Demidovich, A.Elettra Sincrotrone Trieste (author)
  • Danailov, M.Elettra Sincrotrone Trieste (author)
  • Coreno, M.Elettra Sincrotrone Trieste,INFN Frascati National Laboratory,CNR Istituto di Struttura della Materia (CNR-ISM) (author)
  • Zangrando, M.Elettra Sincrotrone Trieste (author)
  • Simoncig, A.Elettra Sincrotrone Trieste (author)
  • Manfredda, M. (author)
  • Squibb, Richard J.University of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)(Swepub:gu)xsquri (author)
  • Feifel, RaimundUniversity of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)(Swepub:gu)xfeira (author)
  • Bengtsson, SamuelLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas(Swepub:lu)fysi-sub (author)
  • Simpson, Emma RoseLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas(Swepub:lu)em2024si (author)
  • Csizmadia, T. (author)
  • Dumergue, M. (author)
  • Kuehn, S. (author)
  • Ueda, K.Tohoku University (author)
  • Li, J. X.Louisiana State University (author)
  • Schafer, Kenneth J.Louisiana State University(Swepub:lu)fysi-ksc (author)
  • Frassetto, F.CNR Institute for Photonics and Nanotechnologies (IFN-CNR) (author)
  • Poletto, L.CNR Institute for Photonics and Nanotechnologies (IFN-CNR) (author)
  • Prince, K. C.Elettra Sincrotrone Trieste (author)
  • Mauritsson, JohanLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas(Swepub:lu)fysi-jma (author)
  • Callegari, C. (author)
  • Sansone, G.Albert-Ludwigs University Freiburg (author)
  • LTH profilområde: Avancerade ljuskällorLTH profilområden (creator_code:org_t)

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  • In:Nature Photonics: Springer Science and Business Media LLC17, s. 200-2071749-48851749-4893

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