Resonant Inner-Shell Photofragmentation of Adamantane (C10H16)

Ganguly, Smita (author): Lund University,Lunds universitet,Lund University Bioimaging Center,Medicinska fakulteten,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Faculty of Medicine,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Gisselbrecht, Mathieu (author): Lund University,Lunds universitet,Lund University Bioimaging Center,Medicinska fakulteten,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Faculty of Medicine,Department of Physics,Departments at LTH,Faculty of Engineering, LTH

Eng-Johnsson, Per (author): Lund University,Lunds universitet,Lunds lasercentrum, LLC,Annan verksamhet, LTH,Lunds Tekniska Högskola,Atomfysik,Fysiska institutionen,Institutioner vid LTH,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Lund Laser Centre, LLC,Other operations, LTH,Faculty of Engineering, LTH,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas

Feifel, Raimund (author): Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Gothenburg Responsibility Project, Gothenburg University

Diaz-Tendero, S. (author)

Maclot, Sylvain, 1986 (author): Lund University,Lunds universitet,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,CNRS-Luminy,Gothenburg Responsibility Project, Gothenburg University

(creator_code:org_t)

Related links:: http://dx.doi.org/10... (free); show more...; https://gup.ub.gu.se...; https://doi.org/10.3...; https://lup.lub.lu.s...; show less...

Abstract Subject headings

Adamantane, the smallest diamondoid molecule with a symmetrical cage, contains two distinct carbon sites, CH and CH2. The ionization/excitation of the molecule leads to the cage opening and strong structural reorganization. While theoretical predictions suggest that the carbon site CH primarily causes the cage opening, the role of the other CH2 site remains unclear. In this study, we used advanced experimental Auger electron-ion coincidence techniques and theoretical calculations to investigate the fragmentation dynamics of adamantane after resonant inner-shell photoexcitation. Our results demonstrate that some fragmentation channels exhibit site-sensitivity of the initial core-hole location, indicating that different carbon site excitations could lead to unique cage opening mechanisms.

By the author/editor: Ganguly, Smita; Gisselbrecht, Ma ...; Eng-Johnsson, Pe ...; Feifel, Raimund; Diaz-Tendero, S.; Muchova, E.; show more...; Milosavljevic, A ...; Rousseau, P.; Maclot, Sylvain, ...; show less...

About the subject

NATURAL SCIENCES: NATURAL SCIENCES; and Biological Scien ...; and Biochemistry and ...

NATURAL SCIENCES: NATURAL SCIENCES; and Physical Science ...; and Atom and Molecul ...

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