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High resolution multiphoton spectroscopy by a tunable free-electron-laser light.

Zitnik, M (author)
Mihelič, A (author)
Bučar, K (author)
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Kavčič, M (author)
Rubensson, Jan-Erik (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik
Svanquist, M (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik
Söderström, Johan (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik
Feifel, Raimund (author)
Uppsala universitet,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Molekyl- och kondenserade materiens fysik
Såthe, Conny (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Ovcharenko, Y (author)
Lyamayev, V (author)
Mazza, T (author)
Meyer, M (author)
Simon, M (author)
Journel, L (author)
Lüning, J (author)
Plekan, O (author)
Coreno, M (author)
Devetta, M (author)
Di Fraia, M (author)
Finetti, P (author)
Richter, R (author)
Grazioli, C (author)
Prince, K C (author)
Callegari, C (author)
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 (creator_code:org_t)
2014
2014
English.
In: Physical Review Letters. - 1079-7114 .- 0031-9007. ; 113:19
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Seeded free electron lasers theoretically have the intensity, tunability, and resolution required for multiphoton spectroscopy of atomic and molecular species. Using the seeded free electron laser FERMI and a novel detection scheme, we have revealed the two-photon excitation spectra of dipole-forbidden doubly excited states in helium. The spectral profiles of the lowest (-1,0)^{+1} ^{1}S^{e} and (0,1)^{0} ^{1}D^{e} resonances display energy shifts in the meV range that depend on the pulse intensity. The results are explained by an effective two-level model based on calculated Rabi frequencies and decay rates.

Subject headings

NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)

Publication and Content Type

art (subject category)
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