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Diastereomeric control of enantioselectivity: evidence for metal cluster catalysis.
- Abdel-Magied, Ahmed (author)
-
- Singh, Amrendra (author)
- Lund University,Lunds universitet,Kemisk fysik,Enheten för fysikalisk och teoretisk kemi,Kemiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Chemical Physics,Physical and theoretical chemistry,Department of Chemistry,Departments at LTH,Faculty of Engineering, LTH
- Haukka, Matti (author)
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- Richmond, Michael G (author)
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- (creator_code:org_t)
- 2014
- 2014
- English.
- In: Chemical Communications. - : Royal Society of Chemistry (RSC). - 1364-548X. ; 50:57, s. 7705-7708
- Journal article (peer-reviewed)
Abstract
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- Enantioselective hydrogenation of tiglic acid effected by diastereomers of the general formula [(μ-H)2Ru3(μ3-S)(CO)7(μ-P-P*)] (P-P* = chiral Walphos diphosphine ligand) strongly supports catalysis by intact Ru3 clusters. A catalytic mechanism involving Ru3 clusters has been established by DFT calculations.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
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- ref (subject category)
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