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- Walmsley, T.University of Oxford (author)
Characterizing the multi-dimensional reaction dynamics of dihalomethanes using XUV-induced Coulomb explosion imaging
- Article/chapterEnglish2023
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- 2023
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- LIBRIS-ID:oai:lup.lub.lu.se:668dc4a6-fbf0-4450-96d1-cfab0ae9c57f
- https://lup.lub.lu.se/record/668dc4a6-fbf0-4450-96d1-cfab0ae9c57fURI
- https://doi.org/10.1063/5.0172749DOI
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- Language:English
- Summary in:English
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- Site-selective probing of iodine 4d orbitals at 13.1 nm was used to characterize the photolysis of CH2I2 and CH2BrI initiated at 202.5 nm. Time-dependent fragment ion momenta were recorded using Coulomb explosion imaging mass spectrometry and used to determine the structural dynamics of the dissociating molecules. Correlations between these fragment momenta, as well as the onset times of electron transfer reactions between them, indicate that each molecule can undergo neutral three-body photolysis. For CH2I2, the structural evolution of the neutral molecule was simultaneously characterized along the C-I and I-C-I coordinates, demonstrating the sensitivity of these measurements to nuclear motion along multiple degrees of freedom.
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- Unwin, J.University of Oxford (author)
- Allum, F.University of Oxford (author)
- Bari, S.German Electron Synchrotron (DESY) (author)
- Boll, R.European XFEL GmbH (author)
- Borne, K.Kansas State University (author)
- Brouard, M.University of Oxford (author)
- Bucksbaum, P.Stanford Linear Accelerator Center (SLAC) (author)
- Ekanayake, N.German Electron Synchrotron (DESY) (author)
- Erk, B.German Electron Synchrotron (DESY) (author)
- Forbes, R.Stanford Linear Accelerator Center (SLAC) (author)
- Howard, A. J.Stanford Linear Accelerator Center (SLAC) (author)
- Eng-Johnsson, P.Lund University,Lunds universitet,Lunds lasercentrum, LLC,Annan verksamhet, LTH,Lunds Tekniska Högskola,Atomfysik,Fysiska institutionen,Institutioner vid LTH,LTH profilområde: Avancerade ljuskällor,LTH profilområden,LU profilområde: Ljus och material,Lunds universitets profilområden,Lund Laser Centre, LLC,Other operations, LTH,Faculty of Engineering, LTH,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH,LU Profile Area: Light and Materials,Lund University Profile areas(Swepub:lu)fysi-pj0 (author)
- Lee, J. W.L.German Electron Synchrotron (DESY) (author)
- Liu, Z.University of Oxford (author)
- Manschwetus, B.German Electron Synchrotron (DESY) (author)
- Mason, R.University of Oxford (author)
- Passow, C.German Electron Synchrotron (DESY) (author)
- Peschel, J.Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)ja7503pe (author)
- Rivas, D.European XFEL GmbH (author)
- Rolles, D.Kansas State University (author)
- Rörig, A.European XFEL GmbH (author)
- Rouzée, A.Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy (author)
- Vallance, C.University of Oxford (author)
- Ziaee, F.Kansas State University (author)
- Burt, M.University of Oxford (author)
- University of OxfordGerman Electron Synchrotron (DESY) (creator_code:org_t)
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- In:Journal of Chemical Physics159:140021-9606
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- Brouard, M.
- Bucksbaum, P.
- Ekanayake, N.
- Erk, B.
- Forbes, R.
- Howard, A. J.
- Eng-Johnsson, P.
- Lee, J. W.L.
- Liu, Z.
- Manschwetus, B.
- Mason, R.
- Passow, C.
- Peschel, J.
- Rivas, D.
- Rolles, D.
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- Rouzée, A.
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