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Roadmap of ultrafas...
Roadmap of ultrafast x-ray atomic and molecular physics
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- Young, Linda (author)
- Argonne National Laboratory,University of Chicago
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- Ueda, Kiyoshi (author)
- Tohoku University
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- Gühr, Markus (author)
- Stanford Linear Accelerator Center (SLAC),University of Potsdam
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- Bucksbaum, Philip H. (author)
- Stanford University,Stanford Linear Accelerator Center (SLAC)
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- Simon, Marc (author)
- Paris-Sorbonne University
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- Mukamel, Shaul (author)
- University of California, Irvine
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- Rohringer, Nina (author)
- University of Hamburg,German Electron Synchrotron (DESY)
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- Prince, Kevin C. (author)
- Elettra Sincrotrone Trieste
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- Masciovecchio, Claudio (author)
- Elettra Sincrotrone Trieste
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- Meyer, Michael (author)
- European XFEL GmbH
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- Rudenko, Artem (author)
- Kansas State University
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- Rolles, Daniel (author)
- Kansas State University
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- Bostedt, Christoph (author)
- Argonne National Laboratory
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- Fuchs, Matthias (author)
- Stanford Linear Accelerator Center (SLAC),University of Nebraska - Lincoln
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- Reis, David A. (author)
- Stanford Linear Accelerator Center (SLAC)
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- Santra, Robin (author)
- German Electron Synchrotron (DESY),University of Hamburg
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- Kapteyn, Henry (author)
- JILA,University of Colorado
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- Murnane, Margaret (author)
- JILA,University of Colorado
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- Ibrahim, Heide (author)
- INRS-EMT, Energy, Materials and Telecommunications
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- Légaré, François (author)
- INRS-EMT, Energy, Materials and Telecommunications
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- Vrakking, Marc (author)
- Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy
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- Isinger, Marcus (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Kroon, David (author)
- Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
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- Gisselbrecht, Mathieu (author)
- Lund University,Lunds universitet,Synkrotronljusfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Synchrotron Radiation Research,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- L'Huillier, Anne (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Wörner, Hans Jakob (author)
- ETH Zürich
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- Leone, Stephen R. (author)
- University of California, Berkeley
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(creator_code:org_t)
- 2018-01-09
- 2018
- English.
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In: Journal of Physics B: Atomic, Molecular and Optical Physics. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 51:3
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Abstract
Subject headings
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- X-ray free-electron lasers (XFELs) and table-top sources of x-rays based upon high harmonic generation (HHG) have revolutionized the field of ultrafast x-ray atomic and molecular physics, largely due to an explosive growth in capabilities in the past decade. XFELs now provide unprecedented intensity (1020 W cm-2) of x-rays at wavelengths down to ∼1 Ångstrom, and HHG provides unprecedented time resolution (∼50 attoseconds) and a correspondingly large coherent bandwidth at longer wavelengths. For context, timescales can be referenced to the Bohr orbital period in hydrogen atom of 150 attoseconds and the hydrogen-molecule vibrational period of 8 femtoseconds; wavelength scales can be referenced to the chemically significant carbon K-edge at a photon energy of ∼280 eV (44 Ångstroms) and the bond length in methane of ∼1 Ångstrom. With these modern x-ray sources one now has the ability to focus on individual atoms, even when embedded in a complex molecule, and view electronic and nuclear motion on their intrinsic scales (attoseconds and Ångstroms). These sources have enabled coherent diffractive imaging, where one can image non-crystalline objects in three dimensions on ultrafast timescales, potentially with atomic resolution. The unprecedented intensity available with XFELs has opened new fields of multiphoton and nonlinear x-ray physics where behavior of matter under extreme conditions can be explored. The unprecedented time resolution and pulse synchronization provided by HHG sources has kindled fundamental investigations of time delays in photoionization, charge migration in molecules, and dynamics near conical intersections that are foundational to AMO physics and chemistry. This roadmap coincides with the year when three new XFEL facilities, operating at Ångstrom wavelengths, opened for users (European XFEL, Swiss-FEL and PAL-FEL in Korea) almost doubling the present worldwide number of XFELs, and documents the remarkable progress in HHG capabilities since its discovery roughly 30 years ago, showcasing experiments in AMO physics and other applications. Here we capture the perspectives of 17 leading groups and organize the contributions into four categories: ultrafast molecular dynamics, multidimensional x-ray spectroscopies; high-intensity x-ray phenomena; attosecond x-ray science.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Keyword
- attosecond phenomena
- table-top sources
- ultrafast molecular dynamics
- x-ray free-electron lasers
- x-ray spectroscopies and phenomena
Publication and Content Type
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- ref (subject category)
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- By the author/editor
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Young, Linda
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Ueda, Kiyoshi
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Gühr, Markus
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Bucksbaum, Phili ...
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Simon, Marc
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Mukamel, Shaul
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Rohringer, Nina
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Prince, Kevin C.
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Masciovecchio, C ...
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Meyer, Michael
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Rudenko, Artem
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Rolles, Daniel
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Bostedt, Christo ...
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Fuchs, Matthias
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Reis, David A.
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Santra, Robin
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Kapteyn, Henry
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Murnane, Margare ...
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Ibrahim, Heide
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Légaré, François
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Vrakking, Marc
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Isinger, Marcus
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Kroon, David
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Gisselbrecht, Ma ...
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L'Huillier, Anne
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Wörner, Hans Jak ...
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Leone, Stephen R ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
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Lund University