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LIBRIS Formathandbok  (Information om MARC21)
FältnamnIndikatorerMetadata
00003301naa a2200541 4500
001oai:lup.lub.lu.se:dcf1a443-9398-48c9-8ea5-3071dcede85c
003SwePub
008160401s2013 | |||||||||||000 ||eng|
024a https://lup.lub.lu.se/record/42728692 URI
024a https://doi.org/10.1038/NPHYS27882 DOI
040 a (SwePub)lu
041 a engb eng
042 9 SwePub
072 7a art2 swepub-publicationtype
072 7a ref2 swepub-contenttype
100a Trigo, M.4 aut
2451 0a Fourier-transform inelastic X-ray scattering from time- and momentum-dependent phonon-phonon correlations
264 1c 2013
520 a The macroscopic characteristics of a material are determined by its elementary excitations, which dictate the response of the system to external stimuli. The spectrum of excitations is related to fluctuations in the density-density correlations and is typically measured through frequency-domain neutron(1) or X-ray(2-4) scattering. Time-domain measurements of these correlations could yield a more direct way to investigate the excitations of solids and their couplings both near to and far from equilibrium. Here we show that we can access large portions of the phonon dispersion of germanium by measuring the diffuse scattering from femtosecond X-ray free-electron laser pulses. A femtosecond optical laser pulse slightly quenches the vibrational frequencies, producing pairs of high-wavevector phonons with opposite momenta. These phonons manifest themselves as time-dependent coherences in the displacement correlations(5) probed by the X-ray scattering. As the coherences are preferentially created in regions of strong electron-phonon coupling, the time-resolved approach is a natural spectroscopic tool for probing low-energy collective excitations in solids, and their microscopic interactions.
650 7a NATURVETENSKAPx Fysikx Atom- och molekylfysik och optik0 (SwePub)103022 hsv//swe
650 7a NATURAL SCIENCESx Physical Sciencesx Atom and Molecular Physics and Optics0 (SwePub)103022 hsv//eng
700a Fuchs, M.4 aut
700a Chen, J.4 aut
700a Jiang, M. P.4 aut
700a Cammarata, M.4 aut
700a Fahy, S.4 aut
700a Fritz, D. M.4 aut
700a Gaffney, K.4 aut
700a Ghimire, S.4 aut
700a Higginbotham, A.4 aut
700a Johnson, S. L.4 aut
700a Kozina, M. E.4 aut
700a Larsson, Jörgenu Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH4 aut0 (Swepub:lu)fysi-jla
700a Lemke, H.4 aut
700a Lindenberg, A. M.4 aut
700a Ndabashimiye, G.4 aut
700a Quirin, F.4 aut
700a Sokolowski-Tinten, K.4 aut
700a Uher, C.4 aut
700a Wang, G.4 aut
700a Wark, J. S.4 aut
700a Zhu, D.4 aut
700a Reis, D. A.4 aut
710a Atomfysikb Fysiska institutionen4 org
773t Nature Physicsg 9:12, s. 790-794q 9:12<790-794x 1745-2473
856u http://dx.doi.org/10.1038/NPHYS2788y FULLTEXT
8564 8u https://lup.lub.lu.se/record/4272869
8564 8u https://doi.org/10.1038/NPHYS2788

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