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Polymer-Based n-Type Yarn for Organic Thermoelectric Textiles

Darabi, Sozan, 1994 (author)
Chalmers tekniska högskola,Chalmers University of Technology,Chalmers Univ Technol, Sweden; Chalmers Univ Technol, Sweden
Yang, Chi Yuan (author)
Linköpings universitet,Linköping University
Li, Zerui, 1996 (author)
Sichuan University,Chalmers tekniska högskola,Chalmers University of Technology,Chalmers Univ Technol, Sweden; Sichuan Univ, Peoples R China
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Huang, Jun-Da (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten
Hummel, Michael (author)
Aalto-Yliopisto,Aalto University,Aalto Univ, Finland
Sixta, Herbert (author)
Aalto-Yliopisto,Aalto University,Aalto Univ, Finland
Fabiano, Simone, 1985- (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten,n Ink AB, Sweden,Wallenberg Wood Science Center
Müller, Christian, 1980 (author)
Chalmers tekniska högskola,Chalmers University of Technology,Chalmers Univ Technol, Sweden; Chalmers Univ Technol, Sweden
Yang, Chiyuan (author)
Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten,n Ink AB, Sweden
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 (creator_code:org_t)
2023-02-14
2023
English.
In: Advanced Electronic Materials. - : Wiley. - 2199-160X .- 2199-160X. ; 9:4
  • Journal article (peer-reviewed)
Abstract Subject headings
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  • A conjugated-polymer-based n-type yarn for thermoelectric textiles is presented. Thermoelectric textile devices are intriguing power sources for wearable electronic devices. The use of yarns comprising conjugated polymers is desirable because of their potentially superior mechanical properties compared to other thermoelectric materials. While several examples of p-type conducting yarns exist, there is a lack of polymer-based n-type yarns. Here, a regenerated cellulose yarn is spray-coated with an n-type conducting-polymer-based ink composed of poly(benzimidazobenzophenanthroline) (BBL) and poly(ethyleneimine) (PEI). The n-type yarns display a bulk electrical conductivity of 8 × 10−3 S cm−1 and Seebeck coefficient of −79 µV K−1. A promising level of air-stability for at least 13 days can be achieved by applying an additional thermoplastic elastomer coating. A prototype in-plane thermoelectric textile, produced with the developed n-type yarns and p-type yarns, composed of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)-coated regenerated cellulose, displays a stable device performance in air for at least 4 days with an open-circuit voltage per temperature difference of 1 mV °C−1. Evidently, polymer-based n-type yarns are a viable component for the construction of thermoelectric textile devices.

Subject headings

NATURVETENSKAP  -- Kemi -- Polymerkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Polymer Chemistry (hsv//eng)
TEKNIK OCH TEKNOLOGIER  -- Materialteknik -- Textil-, gummi- och polymermaterial (hsv//swe)
ENGINEERING AND TECHNOLOGY  -- Materials Engineering -- Textile, Rubber and Polymeric Materials (hsv//eng)
NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)
TEKNIK OCH TEKNOLOGIER  -- Materialteknik -- Annan materialteknik (hsv//swe)
ENGINEERING AND TECHNOLOGY  -- Materials Engineering -- Other Materials Engineering (hsv//eng)

Keyword

poly(benzimidazobenzophenanthroline) (BBL)
electrically conducting regenerated cellulose yarn
thermoelectric textile devices
organic thermoelectrics
electronic textiles (e-textiles)

Publication and Content Type

art (subject category)
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