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- Normann, Fredrik,1982Chalmers tekniska högskola,Chalmers University of Technology (author)
Oxidation of ammonia over a copper oxide-containing solid oxygen carrier with oxygen uncoupling capability
- Article/chapterEnglish2016
Publisher, publication year, extent ...
- Elsevier BV,2016
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- LIBRIS-ID:oai:research.chalmers.se:dc878821-b380-4999-a97a-14933acc563e
- https://research.chalmers.se/publication/234213URI
- https://doi.org/10.1016/j.combustflame.2015.12.029DOI
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- Language:English
- Summary in:English
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- Measurements and modelling of the oxidation of ammonia over copper oxide (CuO) under conditions relevant to chemical-looping combustion with oxygen uncoupling show that CuO fully converts NH3 into NO or N-2 under most of these conditions. Our experiments demonstrate that considerable amounts of NO are formed when the oxygen carrier is fully oxidised. Decreasing the degree of oxidation of the oxygen carrier affected the selectivity of the NH3 oxidation towards NO. Ageing of the oxygen carrier had a similar effect. Modelling suggests that these results reflect a change in the rate of oxygen release from the CuO particles.
Subject headings and genre
- TEKNIK OCH TEKNOLOGIER Kemiteknik hsv//swe
- ENGINEERING AND TECHNOLOGY Chemical Engineering hsv//eng
- Nitrogen oxides
- Ammonia oxidation
- Solid oxygen carrier
- Copper oxide
- Oxygen uncoupling
Added entries (persons, corporate bodies, meetings, titles ...)
- Cheng, M. (author)
- Zhao, Dongmei,1963Chalmers tekniska högskola,Chalmers University of Technology(Swepub:cth)dongmei (author)
- Li, Z. S. (author)
- Cai, N. S. (author)
- Leion, Henrik,1976Chalmers tekniska högskola,Chalmers University of Technology(Swepub:cth)leion (author)
- Chalmers tekniska högskola (creator_code:org_t)
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- In:Combustion and Flame: Elsevier BV165, s. 445-4521556-29210010-2180
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