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  • Schalk, Oliver, et al. (author)
  • Time-resolved photoelectron spectroscopy of nitrobenzene and its aldehydes
  • 2018
  • In: Chemical Physics Letters. - : Elsevier BV. - 0009-2614 .- 1873-4448. ; 691, s. 379-387
  • Journal article (peer-reviewed)abstract
    • We report the first femtosecond time-resolved photoelectron spectroscopy study of 2-, 3-and 4-nitrobenzaldehyde (NBA) and nitrobenzene (NBE) in the gas phase upon excitation at 200 nm. In 3- and 4-NBA, the dynamics follow fast intersystem crossing within 1-2 picoseconds. In 2-NBA and NBE, the dynamics are faster (similar to 0.5 ps). 2-NBA undergoes hydrogen transfer similar to solution phase dynamics. NBE either releases NO2 in the excited state or converts internally back to the ground state. We discuss why these channels are suppressed in the other nitrobenzaldehydes.
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Type of publication
journal article (1)
Type of content
peer-reviewed (1)
Author/Editor
Holland, David M. P. (1)
Boguslavskiy, Andrey ... (1)
Stolow, Albert (1)
Wolf, Thomas J.A. (1)
Schalk, Oliver (1)
Townsend, Dave (1)
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Szori, Milan (1)
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University
Stockholm University (1)
Language
English (1)
Research subject (UKÄ/SCB)
Natural sciences (1)
Year
2018 (1)

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