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- Li, Shuangjun, et al.
(författare)
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Cyclic performance evaluation of CO2 adsorption using polyethylene terephthalate plastic-waste-derived activated carbon
- 2023
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Ingår i: Fuel. - : ELSEVIER SCI LTD. - 0016-2361 .- 1873-7153. ; 331
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Tidskriftsartikel (refereegranskat)abstract
- Polyethylene terephthalate (PET) plastic-waste-derived activated carbons have recently been developed and exhibit excellent CO(2 )adsorption uptake. However, the CO2-adsorption performance of such recycled materials has only been considered on a basic characterization level and has not yet been evaluated in carbon capture cycles, thereby making biased analyses inevitable. Consequently, a whole chain including the material, process, and cycle is essential for comprehensively analyzing and evaluating novel CO2 adsorbents. Therefore, in this study, various CO2-capture cycles using PET plastic-waste-derived activated carbon adsorbents were numerically simulated, the cyclic CO2-adsorption performances were evaluated, and the application scenario was optimized. A methodology for evaluating the cyclic CO2-adsorption performance of PET plastic-waste-derived activated carbon was proposed for CO(2 )capture. The results suggested that the temperature/vacuum swing adsorption cycle was superior and that its maximum exergy efficiency reached 32.90%.
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2. |
- Li, Shuangjun, et al.
(författare)
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Entropy analysis on energy-consumption process and improvement method of temperature/vacuum swing adsorption (TVSA) cycle
- 2019
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Ingår i: Energy. - : PERGAMON-ELSEVIER SCIENCE LTD. - 0360-5442 .- 1873-6785. ; 179, s. 876-889
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Tidskriftsartikel (refereegranskat)abstract
- CO2 adsorption capture, which could be driven by various forms of energy, has been widely studied in recent years due to the equipment is easy to control with low energy consumption required. However, the existing research on the energy-efficiency aspects of temperature/vacuum swing adsorption (TVSA) for CO2 capture are primarily focus on the quantification of input energy in specific cases. As a classical concept in thermodynamics, entropy has been widely applied in researches on the energy conversion process, which could benefit an in-depth understanding on the mechanism of "heatgeneralized chemical energy" conversion. However, an integrated thermodynamic research framework, which could clarify how to conduct a reasonable energy-consumption analysis of TVSA, has not been established yet. In this paper, a simplified thermodynamic cycle of 4-step TVSA was established, with the assumption of CO2 in adsorbed phase as loop fluid. With the application of the thermodynamic research framework proposed in this paper, the entropy analysis on the thermodynamic cycle was conducted. This study is concerned with application of thermodynamics concept to the CO2 adsorption engineering, which is mainly based on classical thermodynamics but also relying on adsorption physics to supply insight into the energy conversion and energy-efficient mechanism of TVSA technologies.
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3. |
- Zhong, Ziqian, 1995, et al.
(författare)
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Reversed asymmetric warming of sub-diurnal temperature over land during recent decades
- 2023
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Ingår i: Nature Communications. - 2041-1723. ; 14
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Tidskriftsartikel (refereegranskat)abstract
- In the latter half of the twentieth century, a significant climate phenomenon “diurnal asymmetric warming” emerged, wherein global land surface temperatures increased more rapidly during the night than during the day. However, recent episodes of global brightening and regional droughts and heatwaves have brought notable alterations to this asymmetric warming trend. Here, we re-evaluate sub-diurnal temperature patterns, revealing a substantial increase in the warming rates of daily maximum temperatures (Tmax), while daily minimum temperatures have remained relatively stable. This shift has resulted in a reversal of the diurnal warming trend, expanding the diurnal temperature range over recent decades. The intensified Tmax warming is attributed to a widespread reduction in cloud cover, which has led to increased solar irradiance at the surface. Our findings underscore the urgent need for enhanced scrutiny of recent temperature trends and their implications for the wider earth system.
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