1. |
- Al-Adili, Ali, et al.
(författare)
-
Ambiguities in the grid-inefficiency correction for Frisch-Grid Ionization Chambers
- 2012
-
Ingår i: Nuclear Instruments and Methods in Physics Research Section A. - : Elsevier. - 0168-9002 .- 1872-9576. ; 673, s. 116-121
-
Tidskriftsartikel (refereegranskat)abstract
- Ionization chambers with Frisch grids have been very successfully applied to neutron-induced fission-fragment studies during the past 20 years. They are radiation resistant and can be easily adapted to the experimental conditions. The use of Frisch grids has the advantage to remove the angular dependency from the charge induced on the anode plate. However, due to the Grid Inefficiency (GI) in shielding the charges, the anode signal remains slightly angular dependent. The correction for the GI is, however, essential to determine the correct energy of the ionizing particles. GI corrections can amount to a few percent of the anode signal. Presently, two contradicting correction methods are considered in literature. The first method adding the angular-dependent part of the signal to the signal pulse height; the second method subtracting the former from the latter. Both additive and subtractive approaches were investigated in an experiment where a Twin Frisch-Grid Ionization Chamber (TFGIC) was employed to detect the spontaneous fission fragments (FF) emitted by a 252Cf source. Two parallel-wire grids with different wire spacing (1 and 2 mm, respectively), were used individually, in the same chamber side. All the other experimental conditions were unchanged. The 2 mm grid featured more than double the GI of the 1 mm grid. The induced charge on the anode in both measurements was compared, before and after GI correction. Before GI correction, the 2 mm grid resulted in a lower pulse-height distribution than the 1 mm grid. After applying both GI corrections to both measurements only the additive approach led to consistent grid independent pulse-height distributions. The application of the subtractive correction on the contrary led to inconsistent, grid-dependent results. It is also shown that the impact of either of the correction methods is small on the FF mass distributions of 235U(nth, f).
|
|
2. |
- Al-Adili, Ali, et al.
(författare)
-
Analysis of prompt fission neutrons in U-235(nth,f) and fission fragment distributions for the thermal neutron induced fission of U-234
- 2016
-
Ingår i: CNR*15 - 5th International Workshop On Compound-Nuclear Reactions And Related Topics. - : EDP Sciences.
-
Konferensbidrag (refereegranskat)abstract
- This paper presents the ongoing analysis of two fission experiments. Both projects are part of the collaboration between the nuclear reactions group at Uppsala and the JRC-IRMM. The first experiment deals with the prompt fission neutron multiplicity in the thermal neutron induced fission of U-235(n,f). The second, on the fission fragment properties in the thermal fission of U-234(n,f). The prompt fission neutron multiplicity has been measured at the JRC-IRMM using two liquid scintillators in coincidence with an ionization chamber. The first experimental campaign focused on U-235(nth,f) whereas a second experimental campaign is foreseen later for the same reaction at 5.5 MeV. The goal is to investigate how the so-called saw-tooth shape changes as a function of fragment mass and excitation energy. Some harsh experimental conditions were experienced due to the large radiation background. The solution to this will be discussed along with preliminary results. In addition, the analysis of thermal neutron induced fission of U-234(n,f) will be discussed. Currently analysis of data is ongoing, originally taken at the ILL reactor. The experiment is of particular interest since no measurement exist of the mass and energy distributions for this system at thermal energies. One main problem encountered during analysis was the huge background of U-235(nth, f). Despite the negligible isotopic traces in the sample, the cross section difference is enormous. Solution to this parasitic background will be highlighted.
|
|
3. |
- Al-Adili, Ali, et al.
(författare)
-
Comparison of digital and analogue data acquisition systems for nuclear spectroscopy
- 2010
-
Ingår i: Nuclear Instruments and Methods in Physics Research Section A. - : Elsevier BV. - 0168-9002 .- 1872-9576. ; 624:3, s. 684-690
-
Tidskriftsartikel (refereegranskat)abstract
- In the present investigation the performance of digital data acquisition (DA) and analogue data acquisition (AA) systems are compared in neutron-induced fission experiments. The DA results are practically identical to the AA results in terms of angular-, energy- and mass-resolution, and both compare very well with literature data. However, major advantages were found with the digital techniques. DA allows for a very efficient αparticle pile-up correction. This is important when considering the accurate measurement of fission-fragment characteristics of highly αactive actinide isotopes relevant for the safe operation of Generation IV reactors and the successful reduction of long-lived radioactive nuclear waste. In case of a strong αemitter, when applying the αparticle pile-up correction, the peak-to-valley ratio of the energy distribution was significantly improved. In addition, DA offers a very flexible expanded off-line analysis and reduces the number of electronic modules drastically, leading to an increased stability against electronic drifts when long measurement times are required.
|
|
4. |
|
|
5. |
- Al-Adili, Ali, et al.
(författare)
-
Employing TALYS to deduce angular momentum rootmean-square values, J(rms), in fission fragments
- 2020
-
Ingår i: ND 2019. - : E D P SCIENCES. - 9782759891061
-
Konferensbidrag (refereegranskat)abstract
- Fission fragments exhibit large angular momenta J, which constitutes a challenge for fission models to fully explain. Systematic measurements of isomeric yield ratios (IYR) are needed for basic nuclear reaction physics and nuclear applications, especially as a function of mass number and excitation energy. One goal is to improve the current understanding of the angular momentum generation and sharing in the fission process. To do so, one needs to improve the modeling of nuclear de-excitation. In this work, we have used the TALYS nuclear-reaction code to relax excited fission fragments and to extract root-mean-square (rms) values of initial spin distributions, after comparison with experimentally determined IYRs. The method was assessed by a comparative study on Cf-252(sf) and (235)(nth,f). The results show a consistent performance of TALYS, both in comparison to reported literature values and to other fission codes. A few discrepant Jrms values were also found. The discrepant literature values could need a second consideration as they could possibly be caused by outdated models. Our TALYS method will be refined to better comply with contemporary sophisticated models and to reexamine older deduced values in literature.
|
|
6. |
- Al-Adili, Ali, et al.
(författare)
-
Extraction of angular momenta from isomeric yield ratios : Employing TALYS to de-excite primary fission fragments
- 2019
-
Ingår i: European Physical Journal A. - : Springer Science and Business Media LLC. - 1434-6001 .- 1434-601X. ; 55:4
-
Tidskriftsartikel (refereegranskat)abstract
- The generation of angular momentum in fission is difficult to model, in particular at higher excitation energies where data are scarce. Isomeric yield ratios (IYR) play an important role in deducing angular momentum properties of fission fragments (FF), albeit this requires some assumptions and simplifications. To estimate FF angular momentum, fission codes can be used to calculate IYRs and compare them to experimental data. Such measurements have systematically been performed at the IGISOL facility using novel experimental techniques. In conjunction, a new method has been developed to infer the angular momentum of the primary FF using the nuclear reaction code TALYS. In this work, we evaluate this new method by comparing our TALYS calculations with values found in the literature and with results from the GEF fission code, for a few well-studied reactions. The overall results show a consistent performance of TALYS and GEF, as well as of many reported literature values. However, some deviations were found, possibly pinpointing the need to re-examine some of the reported literature values. A sensitivity analysis was also performed, in which the role of excitation energy, neutron emission, discrete level structure and level density models were studied. Finally, the role of multiple chance fission, of relevance for the reactions studied at IGISOL, is discussed. Some literature data for this reaction were also re-analyzed using TALYS, revealing significant differences.
|
|
7. |
|
|
8. |
- Al-Adili, Ali, et al.
(författare)
-
First evidence of correlation between vibrational resonances and an anisotropy in the fission mass distribution
-
Annan publikation (övrigt vetenskapligt/konstnärligt)abstract
- In this work we present evidence of anisotropic emission of fragment masses in 234U(n,f). The discovered mass anisotropy is correlated with the prominent vibrational resonances at En = 0.5 and 0.77 MeV and coincides with a verified strong angular anisotropy. From the outcome of this experimental work one may infer unequal fission barrier heights for different degrees of fission asymmetry.
|
|
9. |
- Al-Adili, Ali, et al.
(författare)
-
Fission Activities of the Nuclear Reactions Group in Uppsala
- 2015
-
Ingår i: Scientific Workshop on Nuclear Fission Dynamics and the Emission of Prompt Neutrons and Gamma Rays, THEORY-3. - : Elsevier BV. ; , s. 145-149
-
Konferensbidrag (refereegranskat)abstract
- This paper highlights some of the main activities related to fission of the nuclear reactions group at Uppsala University. The group is involved for instance in fission yield experiments at the IGISOL facility, cross-section measurements at the NFS facility, as well as fission dynamics studies at the IRMM JRC-EC. Moreover, work is ongoing on the Total Monte Carlo (TMC) methodology and on including the GEF fission code into the TALYS nuclear reaction code. Selected results from these projects are discussed.
|
|
10. |
- Al-Adili, Ali, et al.
(författare)
-
Fragment mass-, kinetic energy- and angular distributions for 234U(n, f) at incident neutron energies from En = 0.2 to 5.0 MeV
- 2016
-
Ingår i: Physical review C. - 2469-9985. ; 93:3
-
Tidskriftsartikel (refereegranskat)abstract
- This work investigates the neutron-induced fission of U-234 and the fission-fragment properties for neutron energies between E-n = 0.2 and 5.0 MeV with a special highlight on the prominent vibrational resonance at E-n = 0.77 MeV. Angular, energy, and mass distributions were determined based on the double-energy technique by means of a twin Frisch-grid ionization chamber. The experimental data are parametrized in terms of fission modes based on the multimodal random neck-rupture model. The main results are a verified strong angular anisotropy and fluctuations in the energy release as a function of incident-neutron energy.
|
|
11. |
- Al-Adili, Ali, et al.
(författare)
-
Impact of prompt-neutron corrections on final fission-fragment distributions
- 2012
-
Ingår i: Physical Review C. Nuclear Physics. - 0556-2813 .- 1089-490X. ; 86:5, s. 054601-
-
Tidskriftsartikel (refereegranskat)abstract
- Background: One important quantity in nuclear fission is the average number of prompt neutrons emitted from the fission fragments, the prompt neutron multiplicity, ν . The total number of prompt fission neutrons, νtot, increases with increasing incident neutron energy. The prompt-neutron multiplicity is also a function of the fragment mass and the total kinetic energy of the fragmentation. Those data are only known in sufficient detail for a few thermal-neutron-induced fission reactions on, for example, 233,235U and 239Pu. The enthralling question has always been asked how the additional excitation energy is shared between the fission fragments. The answer to this question is important in the analysis of fission-fragment data taken with the double-energy technique. Although in the traditional approach the excess neutrons are distributed equally across the mass distribution, a few experiments showed that those neutrons are predominantly emitted by the heavy fragments.Purpose: We investigated the consequences of the ν(A,TKE,En) distribution on the fission fragment observables.Methods: Experimental data obtained for the 234U(n, f) reaction with a Twin Frisch Grid Ionization Chamber, were analyzed assuming two different methods for the neutron evaporation correction. The effect of the two different methods on the resulting fragment mass and energy distributions is studied.Results: We found that the preneutron mass distributions obtained via the double-energy technique become slightly more symmetric, and that the impact is larger for postneutron fission-fragment distributions. In the most severe cases, a relative yield change up to 20–30% was observed.Conclusions: We conclude that the choice of the prompt-neutron correction method has strong implications on the understanding and modeling of the fission process and encourages new experiments to measure fission fragments in coincidence with prompt fission neutrons. Even more, the correct determination of postneutron fragment yields has an impact on the reliable assessment of the nuclear waste inventory, as well as on the correct prediction of delayed neutron precursor yields.
|
|
12. |
- Al-Adili, Ali, et al.
(författare)
-
Indication of anisotropic TKE and mass emission in 234U(n,f)
- 2012
-
Ingår i: Physics Procedia. - : Elsevier BV. ; , s. 158-164
-
Konferensbidrag (refereegranskat)abstract
- The neutron-induced fission of 234U has been studied for neutron energies ranging from 200 keV to 5 MeV. Special focus was put around the prominent vibrational resonance in the sub-barrier region around 800 keV incident neutron energy. The aim was to investigate the fission fragment (FF) characteristics and search for fluctuations in energy and mass distributions. The strong angular anisotropy in the case of 234U(n,f) was verified and correlations with changes in energy and mass distributions were found. The TKE around the resonance increases contrary to earlier literature data. Furthermore, the TKE and mass distribution were found to be dependent on emission angle. At the resonance, the TKE was smallest near the 0° emission of the FF. This effect was consistent and coherent with a change in the mass distribution around the resonance. The mass distribution was observed to be less asymmetric near 0° emission. From a fitting analysis based on the Multi-Modal Random Neck-Rupture (MMRNR) model, we found the yield of the standard-1 mode increasing around the resonance. Because the TKE is increasing at larger angles and the mass distribution becomes more symmetric also at larger angles, we conclude that this behavior is due to an increase of the standard-1 mode at these larger angles. Based on the formalism of MMRNR, such difference in angular distribution may be an indication of a different outer barrier height for the standard-1 and standard-2 modes.
|
|
13. |
- Al-Adili, Ali
(författare)
-
Investigation of 234U(n,f) with a Frisch-grid ionization chamber
- 2011
-
Licentiatavhandling (övrigt vetenskapligt/konstnärligt)abstract
- This work treats three topics. The main topic concerns neutron-induced fission of 234U. The main goal is to investigate the fission-fragments properties as a function of the incident neutron energy. The study was carried out using a twin Frisch-grid ionization chamber. The first fluctuations on fragment properties are presented, in terms of strong angular anisotropy oscillation. The second part of the work treats the data-acquisition systems in use, particularly for neutron-induced fission experiments. Modern digital systems are studied and compared with the conventional analogue systems. It was shown that the digital systems are superior in drift stability, pile-up correction and extended the possibilities of offline analysis. The third part of the work concerns the Frisch-grid inefficiency. The Frisch grid was introduced in the chamber to remove the angular dependency from the induced charge. However, the shielding is not perfect and a correction is needed for the small angular dependency. Two contradicting methods have been presented in literature, one adding, and the second subtracting the angular-dependent part from the detected signal. An experiment with Cf(sf) was designed and performed to solve the pending ambiguity. The results support the additive model.
|
|
14. |
- Al-Adili, Ali, et al.
(författare)
-
Ion counting efficiencies at the IGISOL facility
- 2014
-
Rapport (övrigt vetenskapligt/konstnärligt)abstract
- At the IGISOL-JYFLTRAP facility, fission mass yields can be studied at high precision. Fission fragments from a U target are passing through a Ni foil and entering a gas filled chamber. The collected fragments are guided through a mass separator to a Penning trap where their masses are identified. This simulation work focuses on how different fission fragment properties (mass, charge and energy) affect the stopping efficiency in the gas cell. In addition, different experimental parameters are varied (e. g. U and Ni thickness and He gas pressure) to study their impact on the stopping efficiency. The simulations were performed using the Geant4 package and the SRIM code. The main results suggest a small variation in the stopping efficiency as a function of mass, charge and kinetic energy. It is predicted that heavy fragments are stopped about 9% less efficiently than the light fragments. However it was found that the properties of the U, Ni and the He gas influences this behavior. Hence it could be possible to optimize the efficiency.
|
|
15. |
- Al-Adili, Ali, et al.
(författare)
-
Isomer yields in nuclear fission
- 2021
-
Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 2100-014X. ; 256
-
Tidskriftsartikel (refereegranskat)abstract
- The generation of angular momentum in the fission process is still an open question. To shed light on this topic, we started a series of measurements at the IGISOL-JYFLTRAP facility in Finland. Highprecision measurements of isomeric yield ratios (IYR) are performed with a Penning trap, partly with the aim to extract average root-mean-square (rms) quantities of fragment spin distributions. The newly installed Phase-Imaging Ion-Cyclotron Resonance (PI-ICR) technique allows the separation of masses down to tens of keV, which is suffcient to disentangle many isomers. In this paper, we first summarize the previous measurements on the neutron and proton-induced fission of uranium and thorium, e.g. the odd cadmium and indium isotopes (119 ≤ A ≤ 127). The measurements revealed systematic trends as function of mass number, which stimulated further exploration. A recent measurement was performed at IGISIOL and several new IYR data will soon be published, for the first time. Secondly, we employ the TALYS nuclear-reaction code to model one of the newly measured isomer yields. Detailed GEF and TALYS calculations are discussed for the fragment angular momentum distribution in 134I.
|
|
16. |
- Al-Adili, Ali
(författare)
-
Measurements of the 234U(n,f) Reaction with a Frisch-Grid Ionization Chamber up to En=5 MeV
- 2013
-
Doktorsavhandling (övrigt vetenskapligt/konstnärligt)abstract
- This study on the neutron-induced fission of 234U was carried out at the 7 MV Van de Graaff accelerator of IRMM in Belgium. A Twin Frisch-Grid Ionization Chamber (TFGIC) was used to study 234U(n,f) between En = 0.2 and 5.0 MeV. The reaction is important for fission modelling of the second-chance fission in 235U(n,f). The fission fragment (FF) angular-, energy and mass distributions were determined using the 2E-method highlighting especially the region of the vibrational resonance at En = 0.77 MeV.The experiment used both conventional analogue and modern digital acquisition systems in parallel. Several advantages were found in the digital case, especially a successful pile-up correction. The shielding limitations of the Frisch-grid, called "grid-inefficiency", result in an angular-dependent energy signal. The correction of this effect has been a long-standing debate and a solution was recently proposed using the Ramo-Shockley theorem. Theoretical predictions from the latter were tested and verified in this work using two different grids. Also the neutron-emission corrections as a function of excitation energy were investigated. Neutron corrections are crucial for the determination of FF masses. Recent theoretical considerations attribute the enhancement of neutron emission to the heavier fragments exclusively, contrary to the average increase assumed earlier. Both methods were compared and the impact of the neutron multiplicities was assessed. The effects found are significant and highlight the importance of further experimental and theoretical investigation.In this work, the strong angular anisotropy of 234U(n,f ) was confirmed. In addition, and quite surprisingly, the mass distribution was found to be angular-dependent and correlated to the vibrational resonances. The anisotropy found in the mass distribution was consistent with an anisotropy in the total kinetic energy (TKE), also correlated to the resonances. The experimental data were parametrized assuming fission modes based on the Multi-Modal Random Neck-Rupture model. The resonance showed an increased yield from the Standard-1 fission mode and a consistent increased TKE. The discovered correlation between the vibrational resonances and the angular-dependent mass distributions for the asymmetric fission modes may imply different outer fission-barrier heights for the two standard modes.
|
|
17. |
- Al-Adili, Ali, et al.
(författare)
-
Neutron-multiplicity experiments for enhanced fission modelling
- 2017
-
Ingår i: EPJ Web of Conferences. - : EDP Sciences. - 9782759890200
-
Konferensbidrag (refereegranskat)abstract
- The nuclear de-excitation process of fission fragments (FF) provides fundamental information for the understanding of nuclear fission and nuclear structure in neutron-rich isotopes. The variation of the prompt-neutron multiplicity, ν(A), as a function of the incident neutron energy (En) is one of many open questions. It leads to significantly different treatments in various fission models and implies that experimental data are analyzed based on contradicting assumptions. One critical question is whether the additional excitation energy (Eexc) is manifested through an increase of ν(A) for all fragments or for the heavy ones only. A systematic investigation of ν(A) as a function of En has been initiated. Correlations between prompt-fission neutrons and fission fragments are obtained by using liquid scintillators in conjunction with a Frisch-grid ionization chamber. The proof-of-principle has been achieved on the reaction 235U(nth,f) at the Van De Graff (VdG) accelerator of the JRC-Geel using a fully digital data acquisition system. Neutrons from 252Cf(sf) were measured separately to quantify the neutron-scattering component due to surrounding shielding material and to determine the intrinsic detector efficiency. Prelimenary results on ν(A) and spectrum in correlation with FF properties are presented.
|
|
18. |
- Al-Adili, Ali, et al.
(författare)
-
On the Frisch–Grid signal in ionization chambers
- 2012
-
Ingår i: Nuclear Instruments and Methods in Physics Research Section A. - : Elsevier. - 0168-9002 .- 1872-9576. ; 671, s. 103-107
-
Tidskriftsartikel (refereegranskat)abstract
- A recent theoretical approach concerning the grid-inefficiency (GI) problem in Twin Frisch–Grid Ionization Chambers was validated experimentally. The experimental verification focused on the induced signal on the anode plate. In this work the investigation was extended by studying the grid signal. The aim was to verify the grid-signal dependency on the grid inefficiency σ. The measurements were made with fission fragments from 252Cf(sf), using two different grids, with 1 and 2 mm wire distances, leading to the GI values: σ=0.031 and σ=0.083, respectively. The theoretical grid signal was confirmed because the detected grid pulse-height distribution was smaller for the larger σ. By applying the additive GI correction approach, the two grid pulse heights were consistent. In the second part of the work, the corrected grid signal was used to deduce emission angles of the fission fragments. It is inconvenient to treat the grid signal by means of conventional analogue electronics, because of its bipolarity. Therefore, the anode and grid signals were summed to create a unipolar, angle-dependent pulse height. Until now the so-called summing method has been the well-established approach to deduce the angle from the grid signal. However, this operation relies strongly on an accurate and stable calibration between the two summed signals. By application of digital-signal processing, the grid signal's bipolarity is no longer an issue. Hence one can bypass the intermediate summation step of the two different pre-amplifier signals, which leads to higher stability. In this work the grid approach was compared to the summing method in three cases: 252Cf(sf), 235U(n,f) and 234U(n,f). By using the grid directly, the angular resolution was found equally good in the first case but gave 7% and 20% improvements, respectively, in the latter cases.
|
|
19. |
- Al-Adili, Ali, et al.
(författare)
-
Possible anisotropy in the emission of fission fragments
- 2012
-
Ingår i: Conference: 13th international conference on nuclear reaction mechanisms, At Villa Monastero, Varenna, Italy, Volume: pp. 223-225. ; , s. 223-225
-
Konferensbidrag (refereegranskat)abstract
- This study on 234U(n,f) focused on the vibrational resonance at the incident neutron energy En=770 keV. Due to the strong angular anisotropy, Fluctuations of the fission fragment (FF) properties were predicted. The bipolar angular anisotropy was verified in this work and a possible new correlation to anisotropic FF emission has been observed. The mass distribution was found to have the biggest difference in asymmetry, at the vibrational resonance and was less asymmetric in emission along the axis of the beam direction. A corresponding anisotropy in the total kinetic energy was also observed. The observed effect was consistent with the change in the mass distribution. At last, the experimental data were fitted based on the Multi-Modal Random Neck Rupture (MM-RNR) model. The yield of the standard-1 mode was found to increase at the resonance.
|
|
20. |
- Al-Adili, Ali, et al.
(författare)
-
Prompt fission neutron yields in thermal fission of U-235 and spontaneous fission of Cf-252
- 2020
-
Ingår i: Physical Review C. - : American Physical Society (APS). - 2469-9985 .- 2469-9993. ; 102:6
-
Tidskriftsartikel (refereegranskat)abstract
- Background: The sharing of excitation energy between the fission fragments is one of the key issues in studying nuclear fission. One way to address this is by studying prompt-fission neutron multiplicities as a function of other fission observables such as the mass, (nu) over bar (A). These are vital benchmark data for both fission and nuclear deexcitation models, putting constrains on the fragment excitation energy and hence on the competing prompt neutron/gamma-ray emission. Despite numerous detailed studies, recent measurements done at JRC-Geel with the SCINTIA array in the epithermal region show surprisingly strong discrepancies to earlier thermal fission data and the Wahl systematics. Purpose: The purpose was to perform measurements of the prompt-fission neutron multiplicity, as a function of fragment mass and total kinetic energy (TKE), in U-235(n(th), f) and Cf-252(sf), to verify and extend the SCINTIA results. Another goal was to validate the analysis methods, and prepare for planned investigations at excitation energies up to 5.5 MeV. Methods: The experiments were conducted at the former 7 MV Van de Graaff facility in JRC-Geel, using a Twin Frisch-Grid Ionization Chamber and two liquid scintillation detectors. A neutron beam with an average energy of 0.5 MeV was produced via the Li-7(p,n) reaction. The neutrons were thermalized by a 12 cm thick block of paraffin. Digital data acquisition systems were utilized. Comprehensive simulations were performed to verify the methodology and to investigate the role of the mass and energy resolution on measured (nu) over bar (A) and (nu) over bar (TKE) values. The simulation results also revealed that the partial derivative(nu) over bar/partial derivative A and partial derivative(TKE) over bar/partial derivative(nu) over bar are affected by the mass and energy resolution. However, the effect is small for the estimated resolutions of this work. Detailed Fluka simulations were performed to calculate the fraction of thermal neutron-induced fission, which was estimated to be about 98%. Results: The experimental results on (nu) over bar (A) are in good agreement with earlier data for Cf-252(sf). For U-235(n(th), f), the (nu) over bar (A) data is very similar to the data obtained with SCINTIA, and therefore we verify these disclosed discrepancies to earlier thermal data and to the Wahl evaluation. The experimental results on (nu) over bar (TKE) are also in agreement with the data at epithermal energies. For Cf-252(sf) a slope value of partial derivative(TKE) over bar/partial derivative(nu) over bar = (-12.9 f 0.2) MeV/n was obtained. For U-235(n(th), f) the value is (-12.0 +/- 0.1) MeV/n. Finally, the neutron spectrum in the center-of-mass system was derived and plotted as a function of fragment mass. Conclusions: This work clearly proves the lack of accurate correlation between fission fragment and neutron data even in the best-studied reactions. The new results highlight the need of a new evaluation of the prompt-fission multiplicity for U-225(n(th), f).
|
|
21. |
|
|
22. |
- Al-Adili, Ali, et al.
(författare)
-
Sensitivity of Measured Fission Yields on Prompt-neutron Corrections
- 2014
-
Ingår i: Nuclear Data Sheets. - : Elsevier BV. - 0090-3752 .- 1095-9904. ; 119, s. 342-345
-
Tidskriftsartikel (refereegranskat)abstract
- Although the number of emitted prompt neutrons from the fission fragments increases as a function of excitation energy, it is not fully understood whether the increase in (nu) over bar (A) as a function of E-n is mass dependent. The share of excitation energies among the fragments is still under debate, but there are reasons to believe that the excess in neutron emission originates only from the heavy fragments, leaving (nu) over bar (light) (A) almost unchanged. We have investigated the consequences of a mass-dependent increase in (nu) over bar (A) on the final mass and energy distributions. The analysis have been performed on experimentally measured data on U-234(n, f). The assumptions concerning (nu) over bar (A) are essential when analysing measurements based on the 2E-technique, and impact significantly on the measured observables. For example, the post-neutron emission mass yield distribution revealed changes up to 10-30 %. The outcome of this work pinpoints the urgent need to determine (nu) over bar (A) experimentally, and in particular, how (nu) over bar (A) changes as a function of incident neutron energy. Many fission yields in the data libraries could be largely affected, since their analysis is based on a different assumption concerning the neutron emission.
|
|
23. |
- Al-Adili, Ali, et al.
(författare)
-
Simulations of the fission-product stopping efficiency in IGISOL
- 2015
-
Ingår i: European Physical Journal A. - : Springer Science and Business Media LLC. - 1434-6001 .- 1434-601X. ; 51:59, s. 1-7
-
Tidskriftsartikel (refereegranskat)abstract
- At the Jyväskylä Ion Guide Isotope Separator On-Line (IGISOL) facility, independent fission yields are measured employing the Penning-trap technique. Fission products are produced, e.g. by impinging protons on a uranium target, and are stopped in a gas-filled chamber. The products are collected by a flow of He gas and guided through a mass separator to a Penning trap, where their masses are identified. This work investigates how fission-product properties, such as mass and energy, affect the ion stopping efficiency in the gas cell. The study was performed using the Geant4 toolkit and the SRIM code. The main results show a nearly mass-independent ion stopping with regard to the wide spread of ion masses and energies, with a proper choice of uranium target thickness. Although small variations were observed, in the order of 5%, the results are within the systematic uncertainties of the simulations. To optimize the stopping efficiency while reducing the systematic errors, different experimental parameters were varied; for instance material thicknesses and He gas pressure. Different parameters influence the mass dependence and could alter the mass dependencies in the ion stopping efficiency.
|
|
24. |
- Al-Adili, Ali, et al.
(författare)
-
Studying fission neutrons with 2E-2v and 2E
- 2018
-
Ingår i: SCIENTIFIC WORKSHOP ON NUCLEAR FISSION DYNAMICS AND THE EMISSION OF PROMPT NEUTRONS AND GAMMA RAYS (THEORY-4). - : EDP Sciences. - 9782759890316
-
Konferensbidrag (refereegranskat)abstract
- This work aims at measuring prompt-fission neutrons at different excitation energies of the nucleus. Two independent techniques, the 2E-2v and the 2E techniques, are used to map the characteristics of the mass-dependent prompt fission neutron multiplicity, 7(A), when the excitation energy is increased. The VERDI 2E-2v spectrometer is being developed at JRC-GEEL. The Fission Fragment (FF) energies are measured using two arrays of 16 silicon (Si) detectors each. The FFs velocities are obtained by time-of-flight, measured between micro-channel plates (MCP) and Si detectors. With MCPs placed on both sides of the fission source, VERDI allows for independent timing measurements for both fragments. Cf-252(sf) was measured and the present results revealed particular features of the 2E-2v technique. Dedicated simulations were also performed using the GEF code to study important aspects of the 2E-2v technique. Our simulations show that prompt neutron emission has a non-negligible impact on the deduced fragment data and affects also the shape of 17(A). Geometrical constraints lead to a total-kinetic energy-dependent detection efficiency. The 2E technique utilizes an ionization chamber together with two liquid scintillator detectors. Two measurements have been performed, one of Cf-252(sf) and another one of thermal-neutron induced fission in U-235(n,f). Results from Cf-252(sf) are reported here.
|
|
25. |
- Cannarozzo, Simone, et al.
(författare)
-
Global comparison between experimentally measured isomeric yield ratios and nuclear model calculations
- 2023
-
Ingår i: European Physical Journal A. - : Springer. - 1434-6001 .- 1434-601X. ; 59:12
-
Tidskriftsartikel (refereegranskat)abstract
- The level density steers transition probabilities between different states in the decay and de-excitation of excited nuclei. Reliable level density modelling is, therefore, key in describing, e.g., de-excitation of fission fragments, with implications on neutron and gamma-rays multiplicities, and also manifested in the population of isomeric states. We test six currently used level density models and the spin distribution in the level density by comparing calculations with measured isomeric yield ratios. The model calculations are performed with the TALYS code and experimental data for nuclear reactions populating spin isomers are retrieved from the EXFOR database. On average, calculations are in agreement with measured data. However, we find that the population of the high-spin state in an isomeric pair is clearly favoured in all of the six studied level density models. Further studies are then performed on the three used phenomenological level density models, to investigate the significance of their effect. We find that a significant reduction of the spin width distribution improves the agreement between calculated and experimentally observed isomeric yield ratios. This result is independent of the incident particle in the nuclear reaction. The needed reduction of the spin width distribution to comply with empirical data has, e.g., implications for studies in angular momentum generation in fission using isomeric yield rations, calculations of anti-neutrino spectra from nuclear reactors, as well as neutron and gamma-ray multiplicities in nuclear reactor calculations.
|
|