1. |
- Carleer, M. R., et al.
(author)
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Validation of water vapour profiles from the Atmospheric Chemistry Experiment (ACE)
- 2008
-
In: Atmospheric Chemistry and Physics Discussion: An Interactive Open Access Journal of the European Geosciences Union. ; 8:2, s. 4499-4559
-
Journal article (peer-reviewed)abstract
- The Atmospheric Chemistry Experiment (ACE) mission was launched in August 2003 to sound the atmosphere by solar occultation. Water vapour (H2O), one of the most important molecules for climate and atmospheric chemistry, is one of the key species provided by the two principal instruments, the infrared Fourier Transform Spectrometer (ACE-FTS) and the MAESTRO UV-Visible spectrometer (ACE-MAESTRO). The first instrument performs measurements on several lines in the 1362–2137 cm−1 range, from which vertically resolved H2O concentration profiles are retrieved, from 7 to 90 km altitude. ACE-MAESTRO measures profiles using the water absorption band in the near infrared part of the spectrum at 926.0–969.7 nm. This paper presents a comprehensive validation of the ACE-FTS profiles. We have compared the H2O volume mixing ratio profiles with space-borne (SAGE II, HALOE, POAM III, MIPAS, SMR) observations and measurements from balloon-borne frostpoint hygrometers and a ground based lidar. We show that the ACE-FTS measurements provide H2O profiles with small retrieval uncertainties in the stratosphere (better than 5% from 15 to 70 km, gradually increasing above). The situation is unclear in the upper troposphere, due mainly to the high variability of the water vapour volume mixing ratio in this region. A new water vapour data product from the ACE-MAESTRO (Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation) is also presented and initial comparisons with ACE-FTS are discussed.
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2. |
- Gabriel, A., et al.
(author)
-
Zonal asymmetries in middle atmospheric ozone and water vapour derived from Odin satellite data 2001-2010
- 2011
-
In: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 11:18, s. 9865-9885
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Journal article (peer-reviewed)abstract
- Stationary wave patterns in middle atmospheric ozone (O(3)) and water vapour (H(2)O) are an important factor in the atmospheric circulation, but there is a strong gap in diagnosing and understanding their configuration and origin. Based on Odin satellite data from 2001 to 2010 we investigate the stationary wave patterns in O(3) and H(2)O as indicated by the seasonal long-term means of the zonally asymmetric components O(3)* = O(3)-[O(3)] and H(2)O* = H(2)O-[H(2)O] ([O(3)], [H(2)O]: zonal means). At mid-and polar latitudes we find a pronounced wave one pattern in both constituents. In the Northern Hemisphere, the wave patterns increase during autumn, maintain their strength during winter and decay during spring, with maximum amplitudes of about 10-20% of the zonal mean values. During winter, the wave one in O(3)* shows a maximum over the North Pacific/Aleutians and a minimum over the North Atlantic/Northern Europe and a double-peak structure with enhanced amplitude in the lower and in the upper stratosphere. The wave one in H(2)O* extends from the lower stratosphere to the upper mesosphere with a westward shift in phase with increasing height including a jump in phase at upper stratosphere altitudes. In the Southern Hemisphere, similar wave patterns occur mainly during southern spring. By comparing the observed wave patterns in O(3)* and H(2)O* with a linear solution of a steady-state transport equation for a zonally asymmetric tracer component we find that these wave patterns are primarily due to zonally asymmetric transport by geostrophically balanced winds, which are derived from observed temperature profiles. In addition temperature-dependent photochemistry contributes substantially to the spatial structure of the wave pattern in O(3)*. Further influences, e. g., zonal asymmetries in eddy mixing processes, are discussed.
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3. |
- Hultgren, Kristoffer, et al.
(author)
-
What caused the exceptional mid-latitudinal Noctilucent Cloud event in July 2009?
- 2011
-
In: Journal of Atmospheric and Solar-Terrestrial Physics. - : Elsevier BV. - 1364-6826 .- 1879-1824. ; 73:14-15, s. 2125-2131
-
Journal article (peer-reviewed)abstract
- Noctilucent Clouds (NLCs) are rarely observed at mid-latitudes. In July 2009, strong NLCs were recorded from both Paris and Nebraska, located at latitudes 48 degrees N and 41 degrees N, respectively. The main focus of this work is on the atmospheric conditions that have led to NLCs at these latitudes. We investigate to what extent these clouds may be explained by local formation or by transport from higher latitudes. The dynamical situation is analyzed in terms of wind fields created from Aura/MLS temperature data and measured by radar. We discuss possible tidal effects on the transport and examine the general planetary wave activity during these days. The winds do not seem sufficient to transport NLC particles long southward distances. Hence a local formation is rather likely. In order to investigate the possibility of local NLC formation, the CARMA microphysical model has been applied with temperature data from MLS as input. The results from the large-scale datasets are compared to NLC observations by Odin and to local NLC, temperature and wind measurements by lidar and radar. The reason for the exceptional NLC formation is most likely a combination of local temperature variations by diurnal tides, advantageously located large-scale planetary waves, and general mesospheric temperature conditions that were 5-10 K colder than in previous years. The results also point to that NLCs are very unlikely to occur at latitudes below 50 degrees N during daytime. This conclusion can be made from a tidal temperature mode with cold temperatures during nighttime and temperatures above the limit for NLC occurrence during daytime. The best time for observing mid-latitude NLCs is during the early morning hours.
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4. |
- Högberg, Charlotta, et al.
(author)
-
The SPARC water vapour assessment II: Profile-to-profile and climatological comparisons of stratospheric δd(H2O) observations from satellite
- 2019
-
In: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 19:4, s. 2497-2526
-
Journal article (peer-reviewed)abstract
- Within the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II), we evaluated five data sets of δD(H2O) obtained from observations by Odin/SMR (Sub-Millimetre Radiometer), Envisat/MIPAS (Environmental Satellite/Michelson Interferometer for Passive Atmospheric Sounding), and SCISAT/ACE-FTS (Science Satellite/Atmospheric Chemistry Experiment - Fourier Transform Spectrometer) using profile-to-profile and climatological comparisons. These comparisons aimed to provide a comprehensive overview of typical uncertainties in the observational database that could be considered in the future in observational and modelling studies. Our primary focus is on stratospheric altitudes, but results for the upper troposphere and lower mesosphere are also shown. There are clear quantitative differences in the measurements of the isotopic ratio, mainly with regard to comparisons between the SMR data set and both the MIPAS and ACE-FTS data sets. In the lower stratosphere, the SMR data set shows a higher depletion in δD than the MIPAS and ACE-FTS data sets. The differences maximise close to 50hPa and exceed 200%. With increasing altitude, the biases decrease. Above 4hPa, the SMR data set shows a lower δD depletion than the MIPAS data sets, occasionally exceeding 100%. Overall, the δD biases of the SMR data set are driven by HDO biases in the lower stratosphere and by H2O biases in the upper stratosphere and lower mesosphere. In between, in the middle stratosphere, the biases in δD are the result of deviations in both HDO and H2O. These biases are attributed to issues with the calibration, in particular in terms of the sideband filtering, and uncertainties in spectroscopic parameters. The MIPAS and ACE-FTS data sets agree rather well between about 100 and 10hPa. The MIPAS data sets show less depletion below approximately 15hPa (up to about 30%), due to differences in both HDO and H2O. Higher up this behaviour is reversed, and towards the upper stratosphere the biases increase. This is driven by increasing biases in H2O, and on occasion the differences in δD exceed 80%. Below 100hPa, the differences between the MIPAS and ACE-FTS data sets are even larger. In the climatological comparisons, the MIPAS data sets continue to show less depletion in δD than the ACE-FTS data sets below 15hPa during all seasons, with some variations in magnitude. The differences between the MIPAS and ACE-FTS data have multiple causes, such as differences in the temporal and spatial sampling (except for the profile-to-profile comparisons), cloud influence, vertical resolution, and the microwindows and spectroscopic database chosen. Differences between data sets from the same instrument are typically small in the stratosphere. Overall, if the data sets are considered together, the differences in δD among them in key areas of scientific interest (e.g. tropical and polar lower stratosphere, lower mesosphere, and upper troposphere) are too large to draw robust conclusions on atmospheric processes affecting the water vapour budget and distribution, e.g. the relative importance of different mechanisms transporting water vapour into the stratosphere.
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5. |
- Khosrawi, Farahnaz, et al.
(author)
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Assessment of the interannual variability and influence of the QBO and upwelling on tracer-tracer distributions of N2O and O3 in the tropical lower stratosphere
- 2013
-
In: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 13:7, s. 3619-3641
-
Journal article (peer-reviewed)abstract
- A modified form of tracer-tracer correlations of N2O and O3 has been used as a tool for the evaluation of atmospheric photochemical models. Applying this method monthly averages of N2O and O3 are derived for both hemispheres by partitioning the data into altitude (or potential temperature) bins and then averaging over a fixed interval of N2O. In a previous study, the method has been successfully applied to the validation of two Chemical Transport Models (CTMs) and one Chemistry-Climate Model (CCM) using 1-year climatology derived from the Odin Sub Millimetre Radiometer (Odin/SMR). However, the applicability of a 1-year climatology of monthly averages of N2O and O3 has been questioned due to the inability of some CCMs to simulate a specific year for the evaluation of CCMs. In this study, satellite measurements from Odin/SMR, the Aura Microwave Limb Sounder (Aura/MLS), the Michelson Interferometer for Passive Atmospheric Sounding on ENVISAT (ENVISAT/MIPAS), and the Cryogenic Infrared Spectrometers and Telescopes for the Atmosphere (CRISTA-1 and CRISTA-2) as well as model simulations from the Whole Atmosphere Community Climate Model (WACCM) are considered. By using seven to eight years of satellite measurements derived between 2003 and 2010 from Odin/SMR, Aura/MLS, ENVISAT/MIPAS and six years of model simulations from WACCM the interannual variability of lower stratospheric monthly averages of N2O and O3 is assessed. It is shown that the interannual variability of the monthly averages of N2O and O3 is low and thus can be easily distinguished from model deficiencies. Further, it is investigated why large differences between Odin/SMR observations and model simulations from the Karlsruhe Simulation Model of the Middle Atmosphere (KASIMA) and the atmospheric general circulation model ECHAM5/Messy1 are found for the Northern and Southern Hemisphere tropics (0° to 30° N and 0° to −30° S, respectively). The differences between model simulations and observations are most likely caused by an underestimation of the quasi-biennial oscillation and tropical upwelling by the models as well as due to biases and/or instrument noise from the satellite instruments. Finally, an inter-comparison between Odin/SMR, Aura/MLS, ENVISAT/MIPAS and WACCM was performed. The comparison shows that these data sets are generally in good agreement but that also some known biases of the data sets are clearly visible in the monthly averages, thus showing that this method is not only a valuable tool for model evaluation but also for satellite inter-comparisons.
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6. |
- Khosrawi, F., et al.
(author)
-
Sensitivity of polar stratospheric cloud formation to changes in water vapour and temperature
- 2015
-
In: Atmospheric Chemistry and Physics Discussions. - : Copernicus GmbH. - 1680-7375 .- 1680-7367. ; 15:13, s. 17743-17796
-
Research review (peer-reviewed)abstract
- More than a decade ago it was suggested that a cooling of stratospheric temperatures by 1 K or an increase of 1 ppmv of stratospheric water vapour could promote denitrification, the permanent removal of nitrogen species from the stratosphere by solid polar stratospheric cloud (PSC) particles. In fact, during the two Arctic winters 2009/10 and 2010/11 the strongest denitrification in the recent decade was observed. Sensitivity studies along air parcel trajectories are performed to test how a future stratospheric water vapour (H 2 O) increase of 1 ppmv or a temperature decrease of 1 K would affect PSC formation. We perform our study based on measurements made during the Arctic winter 2010/11. Air parcel trajectories were calculated 6 days backward in time based on PSCs detected by CALIPSO (Cloud Aerosol Lidar and Infrared Pathfinder satellite observations). The sensitivity study was performed on single trajectories as well as on a trajectory ensemble. The sensitivity study shows a clear prolongation of the potential for PSC formation and PSC existence when the temperature in the stratosphere is decreased by 1 K and water vapour is increased by 1 ppmv. Based on 15 years of satellite measurements (2000-2014) from UARS/HALOE, Envisat/MIPAS, Odin/SMR, Aura/MLS, Envisat/SCIAMACHY and SCISAT/ACE-FTS it is further investigated if there is a decrease in temperature and/or increase of water vapour (H 2 O) observed in the polar regions similar to that observed at midlatitudes and in the tropics. Although in the polar regions no significant trend is found in the lower stratosphere, we found from the observations a correlation between cold winters and enhanced water vapour mixing ratios.
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7. |
- Khosrawi, F., et al.
(author)
-
The SPARC water vapour assessment II: Comparison of stratospheric and lower mesospheric water vapour time series observed from satellites
- 2018
-
In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 11:7, s. 4435-4463
-
Journal article (peer-reviewed)abstract
- Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 different satellite instruments were compared in the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II). This comparison aimed to provide a comprehensive overview of the typical uncertainties in the observational database that can be considered in the future in observational and modelling studies, e.g addressing stratospheric water vapour trends. The time series comparisons are presented for the three latitude bands, the Antarctic (80°-70°S), the tropics (15°S-15°N) and the Northern Hemisphere mid-latitudes (50°-60°N) at four different altitudes (0.1, 3, 10 and 80hPa) covering the stratosphere and lower mesosphere. The combined temporal coverage of observations from the 15 satellite instruments allowed the consideration of the time period 1986-2014. In addition to the qualitative comparison of the time series, the agreement of the data sets is assessed quantitatively in the form of the spread (i.e. the difference between the maximum and minimum volume mixing ratios among the data sets), the (Pearson) correlation coefficient and the drift (i.e. linear changes of the difference between time series over time). Generally, good agreement between the time series was found in the middle stratosphere while larger differences were found in the lower mesosphere and near the tropopause. Concerning the latitude bands, the largest differences were found in the Antarctic while the best agreement was found for the tropics. From our assessment we find that most data sets can be considered in future observational and modelling studies, e.g. addressing stratospheric and lower mesospheric water vapour variability and trends, if data set specific characteristics (e.g. drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
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8. |
- Kiefer, M., et al.
(author)
-
The SPARC water vapour assessment II: biases and drifts of water vapour satellite data records with respect to frost point hygrometer records
- 2023
-
In: Atmospheric Measurement Techniques. - 1867-1381 .- 1867-8548. ; 16:19, s. 4589-4642
-
Journal article (peer-reviewed)abstract
- Satellite data records of stratospheric water vapour have been compared to balloon-borne frost point hygrometer (FP) profiles that are coincident in space and time. The satellite data records of 15 different instruments cover water vapour data available from January 2000 through December 2016. The hygrometer data are from 27 stations all over the world in the same period. For the comparison, real or constructed averaging kernels have been applied to the hygrometer profiles to adjust them to the measurement characteristics of the satellite instruments. For bias evaluation, we have compared satellite profiles averaged over the available temporal coverage to the means of coincident FP profiles for individual stations. For drift determinations, we analysed time series of relative differences between spatiotemporally coincident satellite and hygrometer profiles at individual stations. In a synopsis we have also calculated the mean biases and drifts (and their respective uncertainties) for each satellite record over all applicable hygrometer stations in three altitude ranges (10-30 hPa, 30-100 hPa, and 100 hPa to tropopause). Most of the satellite data have biases <10 % and average drifts <1 % yr-1 in at least one of the respective altitude ranges. Virtually all biases are significant in the sense that their uncertainty range in terms of twice the standard error of the mean does not include zero. Statistically significant drifts (95 % confidence) are detected for 35 % of the ≈ 1200 time series of relative differences between satellites and hygrometers.
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9. |
- Lossow, Stefan, et al.
(author)
-
A reassessment of the discrepancies in the annual variation of delta D-H2O in the tropical lower stratosphere between the MIPAS and ACE-FTS satellite data sets
- 2020
-
In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 13:1, s. 287-308
-
Journal article (peer-reviewed)abstract
- The annual variation of delta D in the tropical lower stratosphere is a critical indicator for the relative importance of different processes contributing to the transport of water vapour through the cold tropical tropopause region into the stratosphere. Distinct observational discrepancies of the delta D annual variation were visible in the works of Steinwagner et al. (2010) and Randel et al. (2012). Steinwagner et al. (2010) analysed MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) observations retrieved with the IMK/IAA (Institut fur Meteorologie und Klimaforschung in Karlsruhe, Germany, in collaboration with the Instituto de Astrofisica de Andalucia in Granada, Spain) processor, while Randel et al. (2012) focused on ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer) observations. Here we reassess the discrepancies based on newer MIPAS (IMK/IAA) and ACE-FTS data sets, also showing for completeness results from SMR (Sub-Millimetre Radiometer) observations and a ECHAM/MESSy (European Centre for Medium-Range Weather Forecasts Hamburg and Modular Earth Sub-model System) Atmospheric Chemistry (EMAC) simulation (Eichinger et al., 2015b). Similar to the old analyses, the MIPAS data set yields a pronounced annual variation (maximum about 75 parts per thousand), while that derived from the ACE-FTS data set is rather weak (maximum about 25 parts per thousand). While all data sets exhibit the phase progression typical for the tape recorder, the annual maximum in the ACE-FTS data set precedes that in the MIPAS data set by 2 to 3 months. We critically consider several possible reasons for the observed discrepancies, focusing primarily on the MIPAS data set. We show that the delta D annual variation in the MIPAS data up to an altitude of 40 hPa is substantially impacted by a start altitude effect, i.e. dependency between the lowermost altitude where MIPAS retrievals are possible and retrieved data at higher altitudes. In itself this effect does not explain the differences with the ACE-FTS data. In addition, there is a mismatch in the vertical resolution of the MIPAS HDO and H2O data (being consistently better for HDO), which actually results in an artificial tape-recorder-like signal in delta D. Considering these MIPAS characteristics largely removes any discrepancies between the MIPAS and ACE-FTS data sets and shows that the MIPAS data are consistent with a delta D tape recorder signal with an amplitude of about 25 parts per thousand in the lowermost stratosphere.
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10. |
- Lossow, Stefan, 1977, et al.
(author)
-
A reassessment of the discrepancies in the annual variation of δD-H2O in the tropical lower stratosphere between the MIPAS and ACE-FTS satellite data sets
- 2020
-
In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 13:1, s. 287-308
-
Journal article (peer-reviewed)abstract
- The annual variation of δD in the tropical lower stratosphere is a critical indicator for the relative importance of different processes contributing to the transport of water vapour through the cold tropical tropopause region into the stratosphere. Distinct observational discrepancies of the δD annual variation were visible in the works of Steinwagner et al. (2010) and Randel et al. (2012). Steinwagner et al. (2010) analysed MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) observations retrieved with the IMK/IAA (Institut für Meteorologie und Klimaforschung in Karlsruhe, Germany, in collaboration with the Instituto de Astrofísica de Andalucía in Granada, Spain) processor, while Randel et al. (2012) focused on ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer) observations. Here we reassess the discrepancies based on newer MIPAS (IMK/IAA) and ACE-FTS data sets, also showing for completeness results from SMR (Sub-Millimetre Radiometer) observations and a ECHAM/MESSy (European Centre for Medium-Range Weather Forecasts Hamburg and Modular Earth Submodel System) Atmospheric Chemistry (EMAC) simulation (Eichinger et al., 2015b). Similar to the old analyses, the MIPAS data set yields a pronounced annual variation (maximum about 75 ‰), while that derived from the ACE-FTS data set is rather weak (maximum about 25 ‰). While all data sets exhibit the phase progression typical for the tape recorder, the annual maximum in the ACE-FTS data set precedes that in the MIPAS data set by 2 to 3 months. We critically consider several possible reasons for the observed discrepancies, focusing primarily on the MIPAS data set. We show that the δD annual variation in the MIPAS data up to an altitude of 40 hPa is substantially impacted by a “start altitude effect”, i.e. dependency between the lowermost altitude where MIPAS retrievals are possible and retrieved data at higher altitudes. In itself this effect does not explain the differences with the ACE-FTS data. In addition, there is a mismatch in the vertical resolution of the MIPAS HDO and H2O data (being consistently better for HDO), which actually results in an artificial tape-recorder-like signal in δD. Considering these MIPAS characteristics largely removes any discrepancies between the MIPAS and ACE-FTS data sets and shows that the MIPAS data are consistent with a δD tape recorder signal with an amplitude of about 25 ‰ in the lowermost stratosphere.
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11. |
- Lossow, Stefan, 1977, et al.
(author)
-
Comparison of HDO measurements from Envisat/MIPAS with observations by Odin/SMR and SCISAT/ACE-FTS
- 2011
-
In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 4:9, s. 1855-1874
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Journal article (peer-reviewed)abstract
- Measurements of thermal emission in the mid-infrared by Envisat/MIPAS allow the retrieval of HDO information roughly in the altitude range between 10 km and 50 km. From June 2002 to March 2004 MIPAS performed measurements in the full spectral resolution mode. To assess the quality of the HDO data set obtained during that period comparisons with measurements by Odin/SMR and SCISAT/ACE-FTS were performed. Comparisons were made on profile-to-profile basis as well as using seasonal and monthly averages. All in all the comparisons yield favourable results. The largest deviations between MIPAS and ACE-FTS are observed below 15 km, where relative deviations can occasionally exceed 100%. Despite these deviations in the absolute amount of HDO the latitudinal structures observed by both instruments are consistent in this altitude range. Between 15 km and 20 km there is less good agreement, in particular in the Antarctic during winter and spring. Also in the tropics some deviations are found. Above 20 km there is a high consistency in the structures observed by all three instruments. MIPAS and ACE-FTS typically agree within 10%, with MIPAS mostly showing higher abundances than ACE-FTS. Both data sets show considerably more HDO than SMR. This bias can be explained basically by uncertainties in spectroscopic parameters. Above 40 km, where the MIPAS HDO retrieval reaches its limits, still good agreement with the structures observed by SMR is found for most seasons. This puts some confidence in the MIPAS data at these altitudes.
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12. |
- Lossow, Stefan, et al.
(author)
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Critical parameters for the retrieval of mesospheric water vapour and tempera- ture from Odin/SMR limb measurements at 557 GHz
- 2007
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In: Advances in Space Research. - : Elsevier BV. - 0273-1177 .- 1879-1948. ; 40:6, s. 835-845
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Journal article (peer-reviewed)abstract
- Limb measurements at 557 GHz by the Sub-millimetre and Millimetre Radiometer (SMR) onboard the Odin satellite provide water vapour and temperature information throughout the mesosphere. A sensitivity study for these retrievals has been performed, in order to identify the most critical parameters affecting the retrievals, with focus on the polar summer mesosphere conditions. Uncertainties in the instrument characterisation and the a priori value chosen for the pointing offset were found to have significant effects on the retrieved profiles. It is also shown that spectroscopic parameters play a role. An obvious improvement of the water and temperature retrieval can be obtained when we account for some of these critical parameters. However, some further improvement of the instrument behaviour characterisation is still needed
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13. |
- Lossow, Stefan, 1977, et al.
(author)
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Influence of the Antarctic ozone hole on the polar mesopause region as simulated by the Canadian Middle Atmosphere Model
- 2012
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In: Journal of Atmospheric and Solar-Terrestrial Physics. - : Elsevier BV. - 1364-6826. ; 74, s. 111-123
-
Journal article (peer-reviewed)abstract
- It is well established that variations in polar stratospheric winds can affect mesospheric temperatures through changes in the filtering of gravity wave fluxes, which drive a residual circulation in the mesosphere. The Canadian Middle Atmosphere Model (CMAM) is used to examine this vertical coupling mechanism in the context of the mesospheric response to the Antarctic ozone hole. It is found that the response differs significantly between late spring and early summer, because of a changing balance between the competing effects of parametrised gravity wave drag (GWD) and changes in resolved wave drag local to the mesosphere. In late spring, the strengthened stratospheric westerlies arising from the ozone hole lead to reduced eastward GWD in the mesosphere and a warming of the polar mesosphere, just as in the well known mesospheric response to sudden stratospheric warmings, but with an opposite sign. In early summer, with easterly flow prevailing over most of the polar stratosphere, the strengthened easterly wind shear within the mesosphere arising from the westward GWD anomaly induces a positive resolved wave drag anomaly through baroclinic instability. The polar cooling induced by this process completely dominates the upper mesospheric response to the ozone hole in early summer. Consequences for the past and future evolution of noctilucent clouds are discussed.
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14. |
- Lossow, Stefan, et al.
(author)
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Middle atmospheric water vapour and dynamics in the vicinity of the polar vortex during the Hygrosonde-2 campaign
- 2009
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In: Atmospheric Chemistry And Physics. - 1680-7316 .- 1680-7324. ; 9, s. 4407-4417
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Journal article (peer-reviewed)abstract
- The Hygrosonde-2 campaign took place on 16 December 2001 at Esrange/Sweden (68° N, 21° E) with the aim to investigate the small scale distribution of water vapour in the middle atmosphere in the vicinity of the Arctic polar vortex. In situ balloon and rocket-borne measurements of water vapour were performed by means of OH fluorescence hygrometry. The combined measurements yielded a high resolution water vapour profile up to an altitude of 75 km. Using the characteristic of water vapour being a dynamical tracer it was possible to directly relate the water vapour data to the location of the polar vortex edge, which separates air masses of different character inside and outside the polar vortex. The measurements probed extra-vortex air in the altitude range between 45 km and 60 km and vortex air elsewhere. Transitions between vortex and extra-vortex usually coincided with wind shears caused by gravity waves which advect air masses with different water vapour volume mixing ratios. From the combination of the results from the Hygrosonde-2 campaign and the first flight of the optical hygrometer in 1994 (Hygrosonde-1) a clear picture of the characteristic water vapour distribution inside and outside the polar vortex can be drawn. Systematic differences in the water vapour concentration between the inside and outside of the polar vortex can be observed all the way up into the mesosphere. It is also evident that in situ measurements with high spatial resolution are needed to fully account for the small-scale exchange processes in the polar winter middle atmosphere.
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15. |
- Lossow, Stefan, et al.
(author)
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Observations of the mesospheric semi-annual oscillation (MSAO) in water vapour by Odin/SMR
- 2008
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In: Atmospheric Chemistry And Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 8, s. 6527-6540
-
Journal article (peer-reviewed)abstract
- Mesospheric water vapour measurements taken by the SMR instrument aboard the Odin satellite between 2002 and 2006 have been analysed with focus on the mesospheric semi-annual circulation in the tropical and subtropical region. This analysis provides the first complete picture of mesospheric SAO in water vapour, covering altitudes above 80 km where previous studies were limited. Our analysis shows a clear semi-annual variation in the water vapour distribution in the entire altitude range between 65 km and 100 km in the equatorial area. Maxima occur near the equinoxes below 75 km and around the solstices above 80 km. The phase reversal occurs in the small layer in-between, consistent with the downward propagation of the mesospheric SAO in the zonal wind in this altitude range. The SAO amplitude exhibits a double peak structure in the equatorial region, with maxima at about 75 km and 81 km. The observed amplitudes show higher values than an earlier analysis based on UARS/HALOE data. The upper peak amplitude remains relatively constant with latitude. The lower peak amplitude decreases towards higher latitudes, but recovers in the Southern Hemisphere subtropics. On the other hand, the annual variation is much more prominent in the Northern Hemisphere subtropics. Furthermore, higher volume mixing ratios during summer and lower values during winter are observed in the Northern Hemisphere subtropics, as compared to the corresponding latitude range in the Southern Hemisphere.
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16. |
- Lossow, Stefan, 1977-
(author)
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Observations of water vapour in the middle atmosphere
- 2008
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Doctoral thesis (other academic/artistic)abstract
- Water vapour is the most important greenhouse gas and plays a fundamental role in the climate system and for the chemistry of the Earth's atmosphere. This thesis presents observations of water vapour in the middle atmosphere with a particular focus on the mesosphere. The majority of these observations presented in this thesis have been performed by the Swedish satellite Odin, providing global observations since 2001. Further observations come from the Hygrosonde-2 campaign in December 2001 based on balloon and rocket-borne measurements. A general overview of Odin's water vapour measurements in the middle atmosphere is given. The optimisation of the mesospheric water vapour retrieval is presented in detail.The analysis of the observations has focused mainly on different dynamical aspects utilising the characteristic of water vapour as a dynamical tracer in the middle atmosphere. One application is the mesospheric part of the semi-annual oscillation (SAO). The observations reveal that this oscillation is the dominant pattern of variability between 30°S and 10°N in the mesosphere up to an altitude of 80 km. Above 90 km the SAO is dominating at all latitudes in the tropics and subtropics. It is shown that the SAO exhibits a distinct phase change between 75 km and 80 km in the tropical region.This thesis also presents the first satellite observations of water vapour in the altitude range between 90 km and 110 km, extending the observational database up into the lower thermosphere. In the polar regions water vapour exhibits the annual maximum during winter time above 95 km, mainly caused by upwelling during this season. This behaviour is different from that observed in the subjacent part of the mesosphere where the annual maximum occurs during summer time.The Hygrosonde-2 campaign provided a high resolution measurement of water vapour in the vicinity of the polar vortex edge. This edge prevents horizontal transport causing different water vapour characteristics inside and outside the polar vortex. The observations show that this separating behaviour extends high up into the mesosphere. Small scale transitions in the Hygrosonde-2 profile between conditions inside and outside the vortex coincided with wind shears caused by gravity waves.
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17. |
- Lossow, Stefan, 1977, et al.
(author)
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The SPARC water vapour assessment II: Profile-to-profile comparisons of stratospheric and lower mesospheric water vapour data sets obtained from satellites
- 2019
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In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 12:5, s. 2693-2732
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Journal article (peer-reviewed)abstract
- This work is distributed under the Creative Commons Attribution 4.0 License. Within the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II), profile-to-profile comparisons of stratospheric and lower mesospheric water vapour were performed by considering 33 data sets derived from satellite observations of 15 different instruments. These comparisons aimed to provide a picture of the typical biases and drifts in the observational database and to identify data-set-specific problems. The observational database typically exhibits the largest biases below 70 hPa, both in absolute and relative terms. The smallest biases are often found between 50 and 5 hPa. Typically, they range from 0.25 to 0.5 ppmv (5 % to 10 %) in this altitude region, based on the 50 % percentile over the different comparison results. Higher up, the biases increase with altitude overall but this general behaviour is accompanied by considerable variations. Characteristic values vary between 0.3 and 1 ppmv (4 % to 20 %). Obvious data-set-specific bias issues are found for a number of data sets. In our work we performed a drift analysis for data sets overlapping for a period of at least 36 months. This assessment shows a wide range of drifts among the different data sets that are statistically significant at the 2 σ uncertainty level. In general, the smallest drifts are found in the altitude range between about 30 and 10 hPa. Histograms considering results from all altitudes indicate the largest occurrence for drifts between 0.05 and 0.3 ppmv decade-1. Comparisons of our drift estimates to those derived from comparisons of zonal mean time series only exhibit statistically significant differences in slightly more than 3 % of the comparisons. Hence, drift estimates from profile-to-profile and zonal mean time series comparisons are largely interchangeable. As for the biases, a number of data sets exhibit prominent drift issues. In our analyses we found that the large number of MIPAS data sets included in the assessment affects our general results as well as the bias summaries we provide for the individual data sets. This is because these data sets exhibit a relative similarity with respect to the remaining data sets, despite the fact that they are based on different measurement modes and different processors implementing different retrieval choices. Because of that, we have by default considered an aggregation of the comparison results obtained from MIPAS data sets. Results without this aggregation are provided on multiple occasions to characterise the effects due to the numerous MIPAS data sets. Among other effects, they cause a reduction of the typical biases in the observational database.
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18. |
- Lossow, Stefan, 1977, et al.
(author)
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Wintertime water vapor in the polar upper mesosphere and lower thermosphere : First satellite observations by Odin submillimeter radiometer
- 2009
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In: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 114, s. D10304-
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Journal article (peer-reviewed)abstract
- In this paper we present Odin submillimeter radiometer (Odin/SMR) water vapor measurements in the upper mesosphere and lower thermosphere with focus on the polar latitudes in winter. Measurements since 2003 have been compiled to provide a first overview of the water vapor distribution in this altitude range. Our observations show a distinct seasonal increase of the water vapor concentration during winter at a given altitude above 90 km. Above 95 km the observations exhibit the annual water vapor maximum during wintertime. Model simulations from the Hamburg Model of the Neutral and Ionized Atmosphere (HAMMONIA) and the Whole Atmosphere Community Climate Model version 3 (WACCM3) show results that are very similar to the observations. We suggest that the observed increase in water vapor during winter is mainly caused by a combination of upwelling of moister air from lower altitudes and diffusion processes. Distinct interhemispheric differences in the winter water vapor distribution in the upper mesosphere and lower thermosphere can be observed, both in the observations and the model results. The seasonal water vapor increase in the polar regions is much more pronounced in the Southern Hemisphere winter where higher concentrations can be observed. This observation is most likely due to interhemispheric differences in the underlying dynamics and diffusion processes
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19. |
- Nedoluha, G.E., et al.
(author)
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The SPARC water vapor assessment II: intercomparison of satellite and ground-based microwave measurements
- 2017
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In: Atmospheric Chemistry and Physics. - : Copernicus GmbH. - 1680-7316 .- 1680-7324. ; 17:23, s. 14543-14558
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Journal article (peer-reviewed)abstract
- As part of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapor assessment (WAVAS-II), we present measurements taken from or coincident with seven sites from which ground-based microwave instruments measure water vapor in the middle atmosphere. Six of the ground-based instruments are part of the Network for the Detection of Atmospheric Composition Change (NDACC) and provide datasets that can be used for drift and trend assessment. We compare measurements from these ground-based instruments with satellite datasets that have provided retrievals of water vapor in the lower mesosphere over extended periods since 1996. We first compare biases between the satellite and ground-based instruments from the upper stratosphere to the upper mesosphere. We then show a number of time series comparisons at 0.46 hPa, a level that is sensitive to changes in H2O and CH4 entering the stratosphere but, because almost all CH4 has been oxidized, is relatively insensitive to dynamical variations. Interannual variations and drifts are investigated with respect to both the Aura Microwave Limb Sounder (MLS; from 2004 onwards) and each instrument's climatological mean. We find that the variation in the interannual difference in the mean H2O measured by any two instruments is typically similar to 1%. Most of the datasets start in or after 2004 and show annual increases in H2O of 0-1% yr(-1). In particular, MLS shows a trend of between 0.5% yr(-1) and 0.7% yr(-1) at the comparison sites. However, the two longest measurement datasets used here, with measurements back to 1996, show much smaller trends of +0.1% yr(-1) (at Mauna Loa, Hawaii) and -0.1% yr(-1) (at Lauder, New Zealand).
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20. |
- Orsolini, Y. J., et al.
(author)
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Descent from the polar mesosphere and anomalously high stratopause observed in 8 years of water vapor and temperature satellite observations by the Odin Sub-Millimeter Radiometer
- 2010
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In: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 115:12
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Journal article (peer-reviewed)abstract
- Using newly analyzed mesospheric water vapor and temperature observations from the Sub-Millimeter Radiometer instrument aboard the Odin research satellite over the period 2001-2009, we present evidence for an anomalously strong descent of dry mesospheric air from the lower mesosphere into the upper stratosphere in the winters of 2004, 2006, and 2009. In the three cases, the descent follows the recovery of the upper stratospheric polar vortex from a major midwinter stratospheric sudden warming. It is also accompanied by the rapid formation of an anomalously warm polar mesospheric layer, i.e., an elevated polar stratopause, near 75 km, and its slower descent to prewarming level (near 1 hPa) over 1.5-2 months. These three winters stand out in the current record of Odin/Sub-Millimeter Radiometer observations started in July 2001.
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21. |
- Orsolini, Y. J., et al.
(author)
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Modelling the descent of nitric oxide during the elevated stratopause event of January 2013
- 2017
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In: Journal of Atmospheric and Solar-Terrestrial Physics. - : Elsevier BV. - 1364-6826. ; 155, s. 50-61
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Journal article (peer-reviewed)abstract
- Using simulations with a whole-atmosphere chemistry-climate model nudged by meteorological analyses, global satellite observations of nitrogen oxide (NO) and water vapour by the Sub-Millimetre Radiometer instrument (SMR), of temperature by the Microwave Limb Sounder (MLS), as well as local radar observations, this study examines the recent major stratospheric sudden warming accompanied by an elevated stratopause event (ESE) that occurred in January 2013. We examine dynamical processes during the ESE, including the role of planetary wave, gravity wave and tidal forcing on the initiation of the descent in the mesosphere-lower thermosphere (MLT) and its continuation throughout the mesosphere and stratosphere, as well as the impact of model eddy diffusion. We analyse the transport of NO and find the model underestimates the large descent of NO compared to SMR observations. We demonstrate that the discrepancy arises abruptly in the MLT region at a time when the resolved wave forcing and the planetary wave activity increase, just before the elevated stratopause reforms. The discrepancy persists despite doubling the model eddy diffusion. While the simulations reproduce an enhancement of the semi-diurnal tide following the onset of the 2013 SSW, corroborating new meteor radar observations at high northern latitudes over Trondheim (63.4°N), the modelled tidal contribution to the forcing of the mean meridional circulation and to the descent is a small portion of the resolved wave forcing, and lags it by about ten days.
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22. |
- Read, William G., et al.
(author)
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The SPARC Water Vapor Assessment II: assessment of satellite measurements of upper tropospheric humidity
- 2022
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In: Atmospheric Measurement Techniques. - : Copernicus GmbH. - 1867-1381 .- 1867-8548. ; 15:11, s. 3377-3400
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Journal article (peer-reviewed)abstract
- Nineteen limb-viewing data sets (occultation, passive thermal, and UV scattering) and two nadir upper tropospheric humidity (UTH) data sets are intercompared and also compared to frost-point hygrometer balloon sondes. The upper troposphere considered here covers the pressure range from 300-100 hPa. UTH is a challenging measurement, because concentrations vary between 2-1000 ppmv (parts per million by volume), with sharp changes in vertical gradients near the tropopause. Cloudiness in this region also makes the measurement challenging. The atmospheric temperature is also highly variable ranging from 180-250 K. The assessment of satellite-measured UTH is based on coincident comparisons with balloon frost-point hygrometer sondes, multi-month mapped comparisons, zonal mean time series comparisons, and coincident satellite-to-satellite comparisons. While the satellite fields show similar features in maps and time series, quantitatively they can differ by a factor of 2 in concentration, with strong dependencies on the amount of UTH. Additionally, time-lag response-corrected Vaisala RS92 radiosondes are compared to satellites and the frost-point hygrometer measurements. In summary, most satellite data sets reviewed here show on average similar to 30 % agreement amongst themselves and frost-point data but with an additional similar to 30 % variability about the mean bias. The Vaisala RS92 sonde, even with a time-lag correction, shows poor behavior for pressures less than 200 hPa.
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23. |
- Seta, Takamasa, et al.
(author)
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Pressure broadening coefficients of the water vapor lines at 556.936 and 752.033 GHz
- 2008
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In: Journal of Quantitative Spectroscopy and Radiative Transfer. - : Elsevier BV. - 0273-1177 .- 0022-4073. ; 109:1, s. 144-150
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Journal article (peer-reviewed)abstract
- The air induced broadening coefficients of the pure rotational transitions of H2O at 556.936 GHz (110←101), and 752.033 GHz (211←202) were measured by terahertz time-domain spectroscopy. The air broadening coefficient was determined to be for the 556.936 GHz line and for the 752.033 GHz line, respectively. The present broadening coefficients for the 556.936 GHz water line are significantly smaller than those of Markov and Krupnov [Measurements of the pressure shift of the 1(10)–1(01) water line at 556.936 GHz produced by mixtures of gases. J Mol Spect 1995:172;211–4] but relatively close to the values of the HITRAN database. The measured data may improve the accuracy of the abundance of water vapor retrieved from spectra obtained by the Odin/SMR satellite instrument. The effect on the satellite retrieval processing is discussed.
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24. |
- Stevens, M. H., et al.
(author)
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Bright polar mesospheric clouds formed by main engine exhaust from the space shuttle's final launch
- 2012
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In: Journal of Geophysical Research. - 0148-0227 .- 2156-2202. ; 117:19, s. Art. no. D19206-
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Journal article (peer-reviewed)abstract
- The space shuttle launched for the last time on 8 July 2011. As with most shuttle launches, the three main engines injected about 350 t of water vapor between 100 and 115 km off the east coast of the United States during its ascent to orbit. We follow the motion of this exhaust with a variety of satellite and ground-based data sets and find that (1) the shuttle water vapor plume spread out horizontally in all directions over a distance of 3000 to 4000 km in 18 h, (2) a portion of the plume reached northern Europe in 21 h to form polar mesospheric clouds (PMCs) that are brighter than over 99% of all PMCs observed in that region, and (3) the observed altitude dependence of the particle size is reversed with larger particles above smaller particles. We use a one- dimensional cloud formation model initialized with predictions of a plume diffusion model to simulate the unusually bright PMCs. We find that eddy mixing can move the plume water vapor down to the mesopause near 90 km where ice particles can form. If the eddy diffusion coefficient is 400 to 1000 m(2)/s, the predicted integrated cloud brightness is in agreement with both satellite and ground-based observations of the shuttle PMCs. The propellant mass of the shuttle is about 20% of that from all vehicles launched during the northern 2011 PMC season. We suggest that the brightest PMC population near 70 degrees N is formed by space traffic exhaust.
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25. |
- Stevens, M. H., et al.
(author)
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Space shuttle exhaust plumes in the lower thermosphere: Advective transport and diffusive spreading
- 2014
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In: Journal of Atmospheric and Solar-Terrestrial Physics. - : Elsevier BV. - 1364-6826. ; 108, s. 50-60
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Journal article (peer-reviewed)abstract
- The space shuttle main engine plume deposited between 100 and 115 km altitude is a valuable tracer for global-scale dynamical processes. Several studies have shown that this plume can reach the Arctic or Antarctic to form bursts of polar mesospheric clouds (PMCs) within a few days. The rapid transport of the shuttle plume is currently not reproduced by general circulation models and is not well understood. To help delineate the issues, we present the complete satellite datasets of shuttle plume observations by the Sounding of the Atmosphere using Broadband Emission Radiometry instrument and the Sub-Millimeter Radiometer instrument. From 2002 to 2011 these two instruments observed 27 shuttle plumes in over 600 limb scans of water vapor emission, from which we derive both advective meridional transport and diffusive spreading. Each plume is deposited at virtually the same place off the United States east coast so our results are relevant to northern mid-latitudes. We find that the advective transport for the first 6-18 h following deposition depends on the local time (LT) of launch: shuttle plumes deposited later in the day (similar to 13-22 LT) typically move south whereas they otherwise typically move north. For these younger plumes rapid transport is most favorable for launches at 6 and 18 LT, when the displacement is 100 in latitude corresponding to an average wind speed of 30 m/s. For plumes between 18 and 30 h old some show average sustained meridional speeds of 30 m/s. For plumes between 30 and 54 h old the observations suggest a seasonal dependence to the meridional transport, peaking near the beginning of year at 24 m/s. The diffusive spreading of the plume superimposed on the transport is on average 23 m/s in 24 h. The plume observations show large variations in both meridional transport and diffusive spreading so that accurate modeling requires knowledge of the winds specific to each case. The combination of transport and spreading from the STS-118 plume in August 2007 formed bright PMCs between 75 and 85 degrees N a day after launch. These are the highest latitude Arctic PMCs formed by shuttle exhaust reported to date.
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26. |
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27. |
- Wang, Tongmei, et al.
(author)
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Stable Water Isotopologues in the Stratosphere Retrieved from Odin/SMR Measurements
- 2018
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In: Remote Sensing. - : MDPI AG. - 2072-4292. ; 10:2
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Journal article (peer-reviewed)abstract
- Stable Water Isotopologues (SWIs) are important diagnostic tracers for understanding processes in the atmosphere and the global hydrological cycle. Using eight years (2002-2009) of retrievals from Odin/SMR (Sub-Millimetre Radiometer), the global climatological features of three SWIs, (H2O)-O-16, HDO and (H2O)-O-18, the isotopic composition D and O-18 in the stratosphere are analysed for the first time. Spatially, SWIs are found to increase with altitude due to stratospheric methane oxidation. In the tropics, highly depleted SWIs in the lower stratosphere indicate the effect of dehydration when the air comes through the cold tropopause, while, at higher latitudes, more enriched SWIs in the upper stratosphere during summer are produced and transported to the other hemisphere via the Brewer-Dobson circulation. Furthermore, we found that more (H2O)-O-16 is produced over summer Northern Hemisphere and more HDO is produced over summer Southern Hemisphere. Temporally, a tape recorder in (H2O)-O-16 is observed in the lower tropical stratosphere, in addition to a pronounced downward propagating seasonal signal in SWIs from the upper to the lower stratosphere over the polar regions. These observed features in SWIs are further compared to SWI-enabled model outputs. This helped to identify possible causes of model deficiencies in reproducing main stratospheric features. For instance, choosing a better advection scheme and including methane oxidation process in a specific model immediately capture the main features of stratospheric water vapor. The representation of other features, such as the observed inter-hemispheric difference of isotopic component, is also discussed.
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