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Search: WFRF:(Ilchen M.) > (2021)

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1.
  • Jahnke, T., et al. (author)
  • Inner-Shell-Ionization-Induced Femtosecond Structural Dynamics of Water Molecules Imaged at an X-Ray Free-Electron Laser
  • 2021
  • In: Physical Review X. - : American Physical Society. - 2160-3308. ; 11:4
  • Journal article (peer-reviewed)abstract
    • The ultrafast structural dynamics of water following inner-shell ionization is a crucial issue in high-energy radiation chemistry. We have exposed isolated water molecules to a short x-ray pulse from a free-electron laser and detected momenta of all produced ions in coincidence. By combining experimental results and theoretical modeling, we can image dissociation dynamics of individual molecules in unprecedented detail. We reveal significant molecular structural dynamics in H2O2+, such as asymmetric deformation and bond-angle opening, leading to two-body or three-body fragmentation on a timescale of a few femtoseconds. We thus reconstruct several snapshots of structural dynamics at different time intervals, which highlight dynamical patterns that are relevant as initiating steps of subsequent radiation-damage processes.
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2.
  • Varvarezos, Lazaros, et al. (author)
  • Near-threshold two-photon double ionization of Kr in the vacuum ultraviolet
  • 2021
  • In: Physical Review A. - 2469-9926. ; 103:2
  • Journal article (peer-reviewed)abstract
    • We report angle-resolved measurements on photoelectrons emitted upon near-threshold two-photon double ionization (TPDI) of Kr irradiated by free-electron laser (FEL) pulses. These photoelectron angular distributions (PADs) are compared with the results of semirelativistic R-matrix calculations. As reported by Augustin et al. [Phys. Rev. A 98, 033408 (2018)10.1103/PhysRevA.98.033408], it is found that the presence of autoionizing resonances within the bandwidth of the exciting FEL pulse strongly influences the PADs. In contrast to measurements on lower-Z targets such as Ne and Ar, the larger spin-orbit interaction, inherent in 4p-subshell hole states of Kr, permits us to resolve and study PADs associated with some of the fine-structure components of the Kr+ and Kr2+ ions.
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