Evaluation of the third-order optical nonlinearity of Au:SiO2 nanocomposites in the off-resonant spectral region

• The third-order nonlinear optical susceptibility (chi((3))) of Au:SiO2 nanocomposite films with different Au particle sizes was measured to be on the order of 10(-10) esu to 10(-9) esu in the off-resonant spectral region, and the particle size-dependent behavior of chi((3)) was observed. The results were found to deviate substantially from those of the conventional Maxwell-Garnet theory. By adapting the modified invariant imbedding method, which takes into account the effect of interparticle interactions on the nonlinear response, we successfully explain the enhanced third-order nonlinear susceptibility of metal-dielectric nanocomposites at off-resonant wavelengths.

Ämnesord

NATURVETENSKAP  -- Fysik -- Annan fysik (hsv//swe)

NATURAL SCIENCES  -- Physical Sciences -- Other Physics Topics (hsv//eng)

Nyckelord

Nanocomposite

Au:SiO2

Nonlinear refraction

Nonlinear absorption

Invariant imbedding method

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