id:"swepub:oai:DiVA.org:kth-193261"
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- Yu, Fengshou (author)
Electrocatalytic water oxidation by a macrocyclic Cu(II) complex in neutral phosphate buffer
- Article/chapterEnglish2016
Publisher, publication year, extent ...
- 2016
- Royal Society of Chemistry,2016
- printrdacarrier
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- LIBRIS-ID:oai:DiVA.org:kth-193261
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-193261URI
- https://doi.org/10.1039/c6cc04884fDOI
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- Language:English
- Summary in:English
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- SwePubSwePub
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Notes
- QC 20161007
- A single-site copper complex, [Cu(TMC)(H2O)](NO3)(2) (1, TMC = 1,4,8,11-tetramethyl-1,4,8,11-tetraazacyclotetradecane), was found to be the most active copper-based catalyst towards electrocatalytic water oxidation in neutral aqueous solution. Complex 1 leads to a cathodic shift of approximately 200 mV in potential to reach a current density of 1 mA cm(-2) in comparison with that of the previously reported dinuclear copper complex under the same conditions. Upon immobilization of complex 1 on carbon cloth, it shows greatly improved activity than other copper-based WOCs including CuOx and Cu2+.
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- NATURVETENSKAP Kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences hsv//eng
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- Li, Fei (author)
- Hu, Jixiang (author)
- Bai, Lichen (author)
- Zhu, Yong (author)
- Sun, Licheng,1962-KTH,Kemi(Swepub:kth)u1umfd9h (author)
- KTHKemi (creator_code:org_t)
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- In:Chemical Communications: Royal Society of Chemistry52:68, s. 10377-103801359-73451364-548X
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