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Multidimensional re...
Multidimensional resonant nonlinear spectroscopy with coherent broadband x-ray pulses
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- Bennett, Kochise (author)
- Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA.
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- Zhang, Yu (author)
- Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.
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- Kowalewski, Markus (author)
- Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.
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- Hua, Weijie (author)
- KTH,Teoretisk kemi och biologi,Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;KTH Royal Inst Technol, Sch Biotechnol, Dept Theoret Chem & Biol, S-10691 Stockholm, Sweden.
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- Mukamel, Shaul (author)
- Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.;Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA.;Freiburg Inst Adv Studies FRIAS, Freiburg, Germany.
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Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA;Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. (creator_code:org_t)
- IOP PUBLISHING LTD, 2016
- 2016
- English.
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In: Physica Scripta. - : IOP PUBLISHING LTD. - 0031-8949 .- 1402-4896. ; T169
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Subject headings
Close
- New x-ray free electron laser (XFEL) and high harmonic generation (HHG) light sources are capable of generating short and intense pulses that make x-ray nonlinear spectroscopy possible. Multidimensional spectroscopic techniques, which have long been used in the nuclear magnetic resonance, infrared, and optical regimes to probe the electronic structure and nuclear dynamics of molecules by sequences of short pulses with variable delays, can thus be extended to the attosecond x-ray regime. This opens up the possibility of probing core-electronic structure and couplings, the real-time tracking of impulsively created valence-electronic wavepackets and electronic coherences, and monitoring ultrafast processes such as nonadiabatic electron-nuclear dynamics near conical-intersection crossings. We survey various possible types of multidimensional x-ray spectroscopy techniques and demonstrate the novel information they can provide about molecules.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
Keyword
- x-ray
- spectroscopy
- Raman
- four-wave-mixing
Publication and Content Type
- ref (subject category)
- art (subject category)
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