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- Ekholm, V.Uppsala University,Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory (author)
Core-hole localization and ultra-fast dissociation in SF6
- Article/chapterEnglish2020
Publisher, publication year, extent ...
- 2020-07-24
- IOP Publishing,2020
- printrdacarrier
Numbers
- LIBRIS-ID:oai:DiVA.org:kth-279883
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-279883URI
- https://doi.org/10.1088/1361-6455/aba204DOI
- https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-185287URI
- https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-420842URI
- https://lup.lub.lu.se/record/f578a603-5e92-47db-a45d-d400ccde9f73URI
Supplementary language notes
- Language:English
- Summary in:English
Part of subdatabase
- SwePubSwePub
Classification
Notes
- QC 20200915
- Resonant inelastic x-ray scattering spectra excited at the fluorine K resonances of SF(6)have been recorded. While a small but significant propensity for electronically parity-allowed transitions is found, the observation of parity-forbidden electronic transitions is attributed to vibronic coupling that breaks the global inversion symmetry of the electronic wavefunction and localizes the core hole. The dependence of the scattering cross section on the polarization of the incident radiation and the scattering angle is interpreted in terms of local pi/sigma symmetry around the S-F bond. This symmetry selectivity prevails during the dissociation that occurs during the scattering process.
Subject headings and genre
- NATURVETENSKAP Fysik hsv//swe
- NATURAL SCIENCES Physical Sciences hsv//eng
- NATURVETENSKAP Fysik Atom- och molekylfysik och optik hsv//swe
- NATURAL SCIENCES Physical Sciences Atom and Molecular Physics and Optics hsv//eng
- SF6
- resonant inelastic x-ray scattering
- symmetry selection rules
- ultrafast dynamics
- vibronic couplings
- resonant inelastic x-ray scattering
- SF
- symmetry selection rules
- ultrafast dynamics
- vibronic couplings
Added entries (persons, corporate bodies, meetings, titles ...)
- Chiuzbaian, G. S.Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.;Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France.,Lund Univ, MAX IV Lab, Box 118, SE-22100 Lund, Sweden.,Paris-Sorbonne University (author)
- S the, C.Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory(Swepub:lu)maxl-cos (author)
- Nicolaou, A.Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France. (author)
- Guarise, M.Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.;Ctr Nacl Pesquisa Energia & Mat CNPEM, BR-10000 Campinas, Brazil.,Brazilian Center For Research In Energy And Materials (CNPEM),Paris-Sorbonne University (author)
- Simon, M.Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University (author)
- Jaouen, N.Synchrotron SOLEIL, LOrme Merisiers, BP 48, F-91192 Gif Sur Yvette, France. (author)
- Luning, J.Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University (author)
- Hague, C. F.Sorbonne Univ, F-75005 Paris, France.;CNRS, LCPMR, F-75005 Paris, France.,Paris-Sorbonne University (author)
- Gel'mukhanov, FarisKTH Royal Institute of Technology,KTH,Teoretisk kemi och biologi,Royal Inst Technol, Sch Biotechnol, Theoret Chem & Biol, S-10691 Stockholm, Sweden.;Siberian Fed Univ, Krasnoyarsk 660041, Russia.;Fed Res Ctr KSC SB RAS, Kirensky Inst Phys, Krasnoyarsk 660036, Russia.,Siberian Federal University,Kirensky Institute of Physics, Siberian Branch, Russian Academy of Sciences(Swepub:kth)u1tlrmzw (author)
- Odelius, MichaelStockholm University,Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.(Swepub:su)odelius (author)
- Björneholm, OlleUppsala University,Uppsala universitet,Molekyl- och kondenserade materiens fysik(Swepub:lu)maxl-obn (author)
- Rubensson, Jan-ErikUppsala University,Uppsala universitet,Institutionen för fysik och astronomi(Swepub:uu)janerube (author)
- Lunds universitetMAX IV-laboratoriet (creator_code:org_t)
Related titles
- In:Journal of Physics B: IOP Publishing53:180953-40751361-6455
Internet link
- https://doi.org/10.1088/1361-6455/aba204
- https://doi.org/10.1088/1361-6455/aba204Fulltext
- https://uu.diva-portal.org/smash/get/diva2:1474003/FULLTEXT01.pdffulltext:print
- http://dx.doi.org/10.1088/1361-6455/aba204FULLTEXT
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-279883
- https://doi.org/10.1088/1361-6455/aba204
- https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-185287
- https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-420842
- https://lup.lub.lu.se/record/f578a603-5e92-47db-a45d-d400ccde9f73
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