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Anisotropic X-Ray S...
Anisotropic X-Ray Scattering of Transiently Oriented Water
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- Kim, Kyung Hwan (author)
- Stockholms universitet,Fysikum,POSTECH, Republic of Korea,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.;POSTECH, Dept Chem, Pohang 37673, South Korea.
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- Späh, Alexander (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Pathak, Harshad (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Yang, Cheolhee (author)
- POSTECH, Dept Chem, Pohang 37673, South Korea.
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- Bonetti, Stefano (author)
- Stockholms universitet,Fysikum,Ca’ Foscari University of Venice, Italy,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.;Ca Foscari Univ Venice, Dept Mol Sci & Nanosyst, I-30172 Venice, Italy.
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- Amann-Winkel, Katrin (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Mariedahl, Daniel (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Schlesinger, Daniel (author)
- Stockholms universitet,Fysikum,Institutionen för miljövetenskap,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.;Stockholm Univ, Dept Environm Sci, S-11418 Stockholm, Sweden.;Stockholm Univ, Bolin Ctr Climate Res, S-11418 Stockholm, Sweden.
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- Sellberg, Jonas A. (author)
- KTH,Biomedicinsk fysik och röntgenfysik,Albanova VinnExcellence Center for Protein Technology, ProNova,KTH Royal Inst Technol, AlbaNova Univ Ctr, Dept Appl Phys, Biomed & Xray Phys, S-10691 Stockholm, Sweden.
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- Mendez, Derek (author)
- Lawrence Berkeley Natl Lab, Moleeular Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA.
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- van der Schot, Gijs (author)
- Uppsala universitet,Molekylär biofysik
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- Hwang, Harold Y. (author)
- MIT, Dept Chem, Cambridge, MA 02139 USA.
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- Clark, Jesse (author)
- SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
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- Shigeki, Owada (author)
- Japan Synchrotron Radiat Res Inst, Kouto 1-1-1, Sayo, Hyogo 6795198, Japan.
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- Tadashi, Togashi (author)
- Japan Synchrotron Radiat Res Inst, Kouto 1-1-1, Sayo, Hyogo 6795198, Japan.
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- Harada, Yoshihisa (author)
- Univ Tokyo, Inst Solid State Phys, Kouto 1-1-1, Sayo, Hyogo 6795148, Japan.
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- Ogasawara, Hirohito (author)
- SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA.
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- Katayama, Tetsuo (author)
- Japan Synchrotron Radiat Res Inst, Kouto 1-1-1, Sayo, Hyogo 6795198, Japan.
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- Nilsson, Anders (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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- Perakis, Fivos (author)
- Stockholms universitet,Fysikum,Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden.
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(creator_code:org_t)
- American Physical Society (APS), 2020
- 2020
- English.
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In: Physical Review Letters. - : American Physical Society (APS). - 0031-9007 .- 1079-7114. ; 125:7
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Abstract
Subject headings
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- We study the structural dynamics of liquid water by time-resolved anisotropic x-ray scattering under the optical Kerr effect condition. In this way, we can separate the anisotropic scattering decay of 160 fs from the delayed temperature increase of similar to 0.1 K occurring at 1 ps and quantify transient changes in the O-O pair distribution function. Polarizable molecular dynamics simulations reproduce well the experiment, indicating transient alignment of molecules along the electric field, which shortens the nearest-neighbor distances. In addition, analysis of the simulated water local structure provides evidence that two hypothesized fluctuating water configurations exhibit different polarizability.
Subject headings
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Kim, Kyung Hwan
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Späh, Alexander
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Pathak, Harshad
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Yang, Cheolhee
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Bonetti, Stefano
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Amann-Winkel, Ka ...
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show more...
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Mariedahl, Danie ...
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Schlesinger, Dan ...
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Sellberg, Jonas ...
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Mendez, Derek
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van der Schot, G ...
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Hwang, Harold Y.
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Clark, Jesse
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Shigeki, Owada
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Tadashi, Togashi
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Harada, Yoshihis ...
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Ogasawara, Hiroh ...
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Katayama, Tetsuo
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Nilsson, Anders
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Perakis, Fivos
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- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Condensed Matter ...
- Articles in the publication
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Physical Review ...
- By the university
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Royal Institute of Technology
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Stockholm University
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Uppsala University