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Self-Assembly and Magnetic Order of Bi-Molecular 2D Spin Lattices of M(II,III) Phthalocyanines on Au(111)

Baljozovic, Milos (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
Liu, Xunshan (författare)
Univ Bern, Dept Chem Biochem & Pharmaceut Sci, Freiestr 3, CH-3012 Bern, Switzerland.
Popova, Olha (författare)
Univ Basel, Dept Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland.
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Girovsky, Jan (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
Nowakowski, Jan (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
Rossmann, Harald (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.
Nijs, Thomas (författare)
Univ Basel, Dept Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland.
Moradi, Mina (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.;Univ Appl Sci & Arts Northwestern Switzerland, Sch Life Sci, Grundenstr 40, CH-4132 Muttenz, Switzerland.
Mousavi, S. Fatemeh (författare)
Univ Basel, Dept Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland.
Plumb, Nicholas C. (författare)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
Radovic, Milan (författare)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
Ballav, Nirmalya (författare)
Indian Inst Sci Educ & Res, Dept Chem, Pune 411008, Maharashtra, India.
Dreiser, Jan (författare)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.
Decurtins, Silvio (författare)
Univ Bern, Dept Chem Biochem & Pharmaceut Sci, Freiestr 3, CH-3012 Bern, Switzerland.
Pašti, Igor (författare)
KTH,Strukturer,Univ Belgrade, Fac Phys Chem, Studentski Trg 12-16, Belgrade 11000, Serbia.;KTH Royal Inst Technol, Sch Ind Engn & Management, Dept Mat Sci & Engn, Brinellvagen 23, S-10044 Stockholm, Sweden.
Skorodumova, Natalia V. (författare)
Uppsala universitet,KTH,Materialvetenskap,Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden.,Materialteori,KTH Royal Inst Technol, Sch Ind Engn & Management, Dept Mat Sci & Engn, Brinellvagen 23, S-10044 Stockholm, Sweden.
Liu, Shi-Xia (författare)
Univ Bern, Dept Chem Biochem & Pharmaceut Sci, Freiestr 3, CH-3012 Bern, Switzerland.
Jung, Thomas A. (författare)
Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.;Univ Basel, Dept Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland.
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Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland Univ Bern, Dept Chem Biochem & Pharmaceut Sci, Freiestr 3, CH-3012 Bern, Switzerland. (creator_code:org_t)
2021-08-19
2021
Engelska.
Ingår i: MAGNETOCHEMISTRY. - : MDPI. - 2312-7481. ; 7:8
Relaterad länk:
https://doi.org/10.3...
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https://urn.kb.se/re...
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  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
Stäng  
  • Single layer low-dimensional materials are presently of emerging interest, including in the context of magnetism. In the present report, on-surface supramolecular architecturing was further developed and employed to create surface supported two-dimensional binary spin arrays on atomically clean non-magnetic Au(111). By chemical programming of the modules, different checkerboards were produced combining phthalocyanines containing metals of different oxidation and spin states, diamagnetic zinc, and a metal-free 'spacer'. In an in-depth, spectro-microscopy and theoretical account, we correlate the structure and the magnetic properties of these tunable systems and discuss the emergence of 2D Kondo magnetism from the spin-bearing components and via the physico-chemical bonding to the underlying substrate. The contributions of the individual elements, as well as the role of the electronic surface state in the bottom substrate, are discussed, also looking towards further in-depth investigations.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

Nyckelord

self-assembly
metal phthalocyanines
scanning tunneling microscopy (STM)
X-ray absorption spectroscopy (XAS)
X-ray magnetic circular dichroism (XMCD)
Kondo screening
Ruderman-Kittel-Kasuya-Yosida (RKKY) exchange interaction

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