Finite element modeling of UN-UO2 and UN-X-UO2 (X=Mo, W) composite nuclear fuels : temperature-dependent thermal conductivity and fuel performance

• In this study, the temperature-dependent effective thermal conductivity of the innovative UN-X-UO2 (X=Mo, W) nuclear fuel composite has been estimated in the temperature range from room temperature to 2000 K. This composite fuel concept is considered as a promising accident tolerant fuel for light water reactors (LWRs). Following the previously reported experimental composite design, the composite fuel thermal conductivity was calculated using Finite Element modeling (FEM), and it is compared with analytical models of thermal conductivity for 10, 30, 50, and 70 wt.% uncoated/coated UN microspheres in a UO2 matrix. The FEM results show an expected increase in the fuel thermal conductivity as the wt.% of the coated/uncoated UN microspheres increases – from 1.5 to 5.7 times the UO2 reference at 2000 K. However, the analytical models show an overestimation of the fuel thermal conductivity as the wt.% increases. The results also show that Mo and W coatings have similar thermal behaviors and the coating thickness varying from 1-5 μm has an insignificant effect on the thermal behavior of the composite. However, at higher weight fractions, the thermal conductivity of the fuel composite at room temperature is substantially influenced by the high thermal conductivity coatings exceeding that of UN. Thereafter, the thermal conductivity profiles from FEM were used in the fuel thermal performance evaluation during LWR normal operation to calculate the maximum centerline temperature of the fuel composites. The results show a significant decrease in the fuel maximum centerline temperature ranging from −72 K for 10 wt.% UN to −438 K for 70 wt.% UN compared to the UO2 under the same irradiation conditions, providing an enhanced safety margin and thermal and neutronic advantages.

Ämnesord

TEKNIK OCH TEKNOLOGIER  -- Materialteknik (hsv//swe)

ENGINEERING AND TECHNOLOGY  -- Materials Engineering (hsv//eng)

Nyckelord

Accident tolerant fuel

UN-X-UO2

Composite nuclear fuel

Thermal conductivity

Finite element modeling

Fuel performance

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