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Film Formation Kine...
Film Formation Kinetics of Polymer Donor and Nonfullerene Acceptor Active Layers During Printing Out of 1,2,4-Trimethylbenzene in Ambient Conditions
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- Jiang, Xinyu (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Grott, Sebastian (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Körstgens, Volker (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Wienhold, Kerstin S. (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Li, Zerui (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Zhang, Jinsheng (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Everett, Christopher R. (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1
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- Schwartzkopf, Matthias (författare)
- Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany, Notkestraße 85
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- Roth, Stephan V. (författare)
- KTH,Fiber- och polymerteknologi,Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany
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- Müller-Buschbaum, Peter (författare)
- Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str. 1, 85748, Garching, Germany, James-Franck-Str. 1; Heinz Maier-Leibnitz Zentrum (MLZ), Technical University of Munich, Lichtenbergstr. 1, 85748, Garching, Germany, Lichtenbergstr. 1
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Chair for Functional Materials, Department of Physics, TUM School of Natural Sciences, Technical University of Munich, James-Franck-Str 1, 85748, Garching, Germany, James-Franck-Str. 1 Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany, Notkestraße 85 (creator_code:org_t)
- 2023-01-24
- 2023
- Engelska.
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Ingår i: Solar RRL. - : Wiley. - 2367-198X. ; 7:6
- Relaterad länk:
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https://doi.org/10.1...
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Slot-die coating is a promising upscaling fabrication method to promote commercialization in the field of organic solar cells. Herein, the nonfullerene active layer blend of a conjugated polymer PffBT4T-2OD and a small molecule acceptor EH-IDTBR, which is printed out of the nonhalogenated solvent 1,2,4-trimethylbenzene, is studied. The film formation kinetics of the active layer PffBT4T-2OD:EH-IDTBR is probed in terms of the temporal evolutions in morphology as well as molecular conformation and aggregation as revealed by in situ grazing-incidence small angle X-ray scattering and UV–vis spectroscopy during the film printing process. A five-regime mesoscale domain growth process is observed in the active layer from the liquid state to the final dry state. The solvent evaporation-induced domain growth is accompanied with molecular stacking in a distinct J-type aggregation of the acceptor and a slight H-type aggregation of the donor molecules. The printed active layers exhibit an edge-on dominated PffBT4T-2OD and a face-on dominated EH-IDTBR crystallite structure. Compared to the neat PffBT4T-2OD and EH-IDTBR films, in the active layer, the crystallite structure deviates slightly in lattice spacing.
Ämnesord
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Nyckelord
- in situ GISAXS
- in situ UV–vis
- nonfullerene acceptors
- printing
- slot-die coating
Publikations- och innehållstyp
- ref (ämneskategori)
- art (ämneskategori)
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