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n-Type Organic Electrochemical Transistors with High Transconductance and Stability

Wang, Yazhou (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Zhu, Genming (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Zeglio, Erica (författare)
Karolinska Institutet,KTH,Science for Life Laboratory, SciLifeLab,Center for the Advancement of Integrated Medical and Engineering Sciences, AIMES,Nanobioteknologi,Department of Neuroscience, Karolinska Institute, Stockholm 17177, Sweden,CBH Digital Futures
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Castillo, Tania Cecilia Hidalgo (författare)
Biological and Environmental Science and Engineering (BESE) Organic Bioelectronics Laboratory, King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia
Haseena, Sheik (författare)
Department of Chemistry, SRM University AP, Amaravati 522240, India
Ravva, Mahesh Kumar (författare)
Department of Chemistry, SRM University AP, Amaravati 522240, India
Cong, Shengyu (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Chen, Junxin (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Lan, Liuyuan (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Li, Zhengke (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China
Herland, Anna (författare)
Karolinska Institutet,KTH,Nanobioteknologi,Science for Life Laboratory, SciLifeLab,Center for the Advancement of Integrated Medical and Engineering Sciences, AIMES,Department of Neuroscience, Karolinska Institute, Stockholm 17177, Sweden,CBH Digital Futures
Mcculloch, Iain (författare)
Department of Chemistry Chemistry Research Laboratory, University of Oxford, Oxford OX1 3TA, U.K.
Inal, Sahika (författare)
Biological and Environmental Science and Engineering (BESE) Organic Bioelectronics Laboratory, King Abdullah University of Science and Technology (KAUST), Thuwal 23955-6900, Saudi Arabia
Yue, Wan (författare)
Guangzhou Key Laboratory of Flexible Electronic Materials and Wearable Devices School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou 510275, People's Republic of China; Department of Chemistry Chemistry Research Laboratory, University of Oxford, Oxford OX1 3TA, U.K.
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 (creator_code:org_t)
2023-01-08
2023
Engelska.
Ingår i: Chemistry of Materials. - : American Chemical Society (ACS). - 0897-4756 .- 1520-5002. ; 35:2, s. 405-415
Relaterad länk:
https://urn.kb.se/re...
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https://doi.org/10.1...
http://kipublication...
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  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • An n-type conjugated polymer based on diazaisoindigo (AIID) and fluorinated thiophene units is introduced. Combining the strong electron-accepting properties of AIID with backbone fluorination produced gAIID-2FT, leading to organic electrochemical transistors (OECTs) with normalized values of 4.09 F cm-1 V-1 s-1 and a normalized transconductance (gm,norm) of 0.94 S cm-1. The resulting OECTs exhibit exceptional operational stability and long shelf-life in ambient conditions, preserving 100% of the original maximum drain current after over 3 h of continuous operation and 28 days of storage in the air. Our work highlights the advantages of integrating strong electron acceptors with donor fluorination to boost the performance and stability of n-type OECTs.

Ämnesord

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

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