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Carbon-negative val...
Carbon-negative valorization of biomass waste into affordable green hydrogen and battery anodes
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- Yang, Hanmin, 1992- (author)
- KTH,Processer,KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Nurdiawati, Anissa (author)
- KTH,Industriell ekonomi och organisation (Inst.),KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Ind Econ & Management, S-10044 Stockholm, Sweden.
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- Gond, Ritambhara (author)
- Uppsala universitet,Strukturkemi
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- Chen, Shiwei (author)
- Shanghai Jiao Tong University, Sweden,Shanghai Jiao Tong Univ, Univ Michigan Shanghai Jiao Tong Univ Joint Inst, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China.
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- Wang, Shule (author)
- Nanjing Forestry University, China; Chinese Academy of Forestry, China,Nanjing Forestry Univ, Coll Chem Engn, Int Innovat Ctr Forest Chem & Mat, Longpan Rd 159, Nanjing 210037, Peoples R China.;Chinese Acad Forestry, Inst Chem Ind Forest Prod, Jiangsu Prov Key Lab Biomass Energy & Mat, 16 Suojin Five Village, Nanjing 210042, Peoples R China.
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- Tang, Bin (author)
- Zhengzhou University, China,Zhengzhou Univ, Engn Res Ctr Adv Funct Mat Mfg, Sch Chem Engn, Minist Educ, Zhengzhou 450001, Peoples R China.
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- Jin, Yanghao (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Zaini, Ilman Nuran (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Shi, Ziyi (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Wang, Wujun (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Energy Technol, Brinellvagen 68, S-100 44 Stockholm, Sweden.
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- Martin, Andrew R., 1968- (author)
- KTH,Energiteknik,KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Energy Technol, Brinellvagen 68, S-100 44 Stockholm, Sweden.
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- Younesi, Reza (author)
- Uppsala universitet,Strukturkemi
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- Sandström, Linda (author)
- RISE,Bioraffinaderi och energi,RISE AB, Div Bioecon & Hlth Biorefinery & Econ, Box 726, S-94128 Pitea, Sweden.
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- Jönsson, Pär G. (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Yang, Weihong (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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- Han, Tong (author)
- KTH Royal Institute of Technology, Sweden,KTH Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden.
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(creator_code:org_t)
- Elsevier BV, 2023
- 2023
- English.
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In: International journal of hydrogen energy. - : Elsevier BV. - 0360-3199 .- 1879-3487.
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Abstract
Subject headings
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- The global Sustainable Development Goals highlight the necessity for affordable and clean energy, designated as SDG7. A sustainable and feasible biorefinery concept is proposed for the carbon-negative utilization of biomass waste for affordable H2 and battery anode material production. Specifically, an innovative tandem biocarbon + NiAlO + biocarbon catalyst strategy is constructed to realize a complete reforming of biomass pyro-vapors into H2+CO (as a mixture). The solid residues from pyrolysis are upgraded into high-quality hard carbon (HCs), demonstrating potential as sodium ion battery (SIBs) anodes. The product, HC-1600-6h, exhibited great electrochemical performance when employed as (SIBs) anodes (full cell: 263 Wh/kg with ICE of 89%). Ultimately, a comprehensive process is designed, simulated, and evaluated. The process yields 75 kg H2, 169 kg HCs, and 891 kg captured CO2 per ton of biomass achieving approx. 100% carbon and hydrogen utilization efficiencies. A life cycle assessment estimates a biomass valorization process with negative-emissions (−0.81 kg CO2/kg-biomass, reliant on Sweden wind electricity). A techno-economic assessment forecasts a notably profitable process capable of co-producing affordable H2 and hard carbon battery anodes. The payback period of the process is projected to fall within two years, assuming reference prices of 13.7 €/kg for HCs and 5 €/kg for H2. The process contributes to a novel business paradigm for sustainable and commercially viable biorefinery process, achieving carbon-negative valorization of biomass waste into affordable energy and materials.
Subject headings
- TEKNIK OCH TEKNOLOGIER -- Maskinteknik -- Energiteknik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Mechanical Engineering -- Energy Engineering (hsv//eng)
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
- TEKNIK OCH TEKNOLOGIER -- Maskinteknik (hsv//swe)
- ENGINEERING AND TECHNOLOGY -- Mechanical Engineering (hsv//eng)
Keyword
- Biomass
- Pyrolysis
- Catalytic reforming
- Biochar
- Syngas
- Auger
- Energiteknik
- Energy Technology
- Chemical Engineering
- Kemiteknik
- Materials Science and Engineering
- Teknisk materialvetenskap
Publication and Content Type
- vet (subject category)
- art (subject category)
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- By the author/editor
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Yang, Hanmin, 19 ...
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Nurdiawati, Anis ...
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Gond, Ritambhara
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Chen, Shiwei
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Wang, Shule
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Tang, Bin
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Jin, Yanghao
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Zaini, Ilman Nur ...
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Shi, Ziyi
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Wang, Wujun
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Martin, Andrew R ...
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Younesi, Reza
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Sandström, Linda
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Jönsson, Pär G.
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Yang, Weihong
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Han, Tong
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ENGINEERING AND ...
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NATURAL SCIENCES
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ENGINEERING AND ...
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Royal Institute of Technology
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RISE
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Uppsala University