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- Vongvilai, PornrapeeKTH,Organisk kemi (author)
Racemase Activity of B. cepacia Lipase Leads to Dual-Function Asymmetric Dynamic Kinetic Resolution of alpha-Aminonitriles
- Article/chapterEnglish2011
Publisher, publication year, extent ...
- 2011-06-01
- Wiley,2011
- printrdacarrier
Numbers
- LIBRIS-ID:oai:DiVA.org:kth-37184
- https://urn.kb.se/resolve?urn=urn:nbn:se:kth:diva-37184URI
- https://doi.org/10.1002/anie.201007373DOI
Supplementary language notes
- Language:English
- Summary in:English
Part of subdatabase
- SwePubSwePub
Classification
Notes
- Uppdated from Manuscript to Article. QC 20120903
- Applaudable promiscuity: Racemase-type activity discovered for B. cepacia lipase with N-substituted α-aminonitriles is proposed to involve a C-C bond-breaking/forming mechanism in the hydrolase site of the enzyme, as supported by experimental data and calculations. This promiscuous activity in combination with the transacylation activity of the enzyme enabled the asymmetric synthesis of N-methyl α-aminonitrile amides in high yield (see scheme).
Subject headings and genre
- NATURVETENSKAP Kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences hsv//eng
- dynamic kinetic resolution
- enzyme catalysis
- racemase activity
- secondary amines
- Strecker reaction
- Chemistry
- Kemi
Added entries (persons, corporate bodies, meetings, titles ...)
- Linder, MatsKTH,Fysikalisk kemi(Swepub:kth)u157x78b (author)
- Sakulsombat, MorakotKTH,Organisk kemi(Swepub:kth)u1v5373p (author)
- Humble, Maria SvedendahlKTH,Biokemi(Swepub:kth)u1mmbr9s (author)
- Berglund, PerKTH,Biokemi(Swepub:kth)u1271chh (author)
- Brinck, ToreKTH,Fysikalisk kemi(Swepub:kth)u1ar43qu (author)
- Ramström, OlofKTH,Organisk kemi(Swepub:kth)u1aj7snf (author)
- KTHOrganisk kemi (creator_code:org_t)
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- In:Angewandte Chemie International Edition: Wiley50:29, s. 6592-65951433-78511521-3773
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