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DNA Based Hybrid Ma...
DNA Based Hybrid Material for Interface Engineering in Polymer Solar Cells
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- Elfwing, Anders (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Cai, Wanzhu (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Ouyang, Liangqi (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Liu, Xianjie (author)
- Linköpings universitet,Ytors Fysik och Kemi,Tekniska fakulteten
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- Xia, Yuxin (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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- Tang, Zheng (author)
- Tech Univ Dresden, Germany
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- Inganäs, Olle (author)
- Linköpings universitet,Biomolekylär och Organisk Elektronik,Tekniska fakulteten
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(creator_code:org_t)
- 2018-03-05
- 2018
- English.
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In: ACS Applied Materials and Interfaces. - : AMER CHEMICAL SOC. - 1944-8244 .- 1944-8252. ; 10:11, s. 9579-9586
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Subject headings
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- A new solution processable electron transport material (ETM) is introduced for use in photovoltaic devices, which consists of a metallic conjugated polyelectrolyte, poly(4-(2,3-dihydrothieno[3,4-b]-[1,4]dioxin-2-yl-methoxy)-1-butanesulfonic acid (PEDOT-S), and surfactant-functionalized deoxyribonucleic acid (DNA) (named DNA:CTMA:PEDOT-S). This ETM is demonstrated to effectively work for bulk-heterojunction organic photovoltaic devices (OPV) based on different electron acceptor materials. The fill factor, the open circuit voltage, and the overall power conversion efficiency of the solar cells with a DNA:CTMA:PEDOT-S modified cathode are comparable to those of devices with a traditional lithium fluoride/aluminum cathode. The new electron transport layer has high optical transmittance, desired work function and selective electron transport. A dipole effect induced by the use of the surfactant cetyltrimethylammonium chloride (CTMA) is responsible for lowering the electrode work function. The DNA:CTMA complex works as an optical absorption dilutor, while PEDOT-S provides the conducting pathway for electron transport, and allows thicker layer to be used, enabling printing. This materials design opens a new pathway to harness and optimize the electronic and optical properties of printable interface materials.
Subject headings
- NATURVETENSKAP -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Condensed Matter Physics (hsv//eng)
Keyword
- organic photovoltaic device; electron transport material; DNA based hybrid material; self-doped polyelectrolyte; high optical transmittance
Publication and Content Type
- ref (subject category)
- art (subject category)
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