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  • Persson, IngemarLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten (author)

2D Transition Metal Carbides (MXenes) for Carbon Capture

  • Article/chapterEnglish2019

Publisher, publication year, extent ...

  • 2018-11-04
  • WILEY-V C H VERLAG GMBH,2019
  • electronicrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:liu-154119
  • https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-154119URI
  • https://doi.org/10.1002/adma.201805472DOI

Supplementary language notes

  • Language:English
  • Summary in:English

Part of subdatabase

Classification

  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • Funding Agencies|Swedish Research Council [2016-04412, 2016-00889, 642-2013-8020]; Knut and Alice Wallenbergs Foundation [KAW 2015.0043]; Swedish Foundation for Strategic Research (SSF) [EM16-0004, RIF 14-0074, FL12-0181]; Swedish Government Strategic Research Area in Materials Science on Functional Materials at Linkoping University (Faculty Grant SFO-Mat-LiU) [2009 00971]
  • Global warming caused by burning of fossil fuels is indisputably one of mankinds greatest challenges in the 21st century. To reduce the ever-increasing CO2 emissions released into the atmosphere, dry solid adsorbents with large surface-to-volume ratio such as carbonaceous materials, zeolites, and metal-organic frameworks have emerged as promising material candidates for capturing CO2. However, challenges remain because of limited CO2/N-2 selectivity and long-term stability. The effective adsorption of CO2 gas (approximate to 12 mol kg(-1)) on individual sheets of 2D transition metal carbides (referred to as MXenes) is reported here. It is shown that exposure to N-2 gas results in no adsorption, consistent with first-principles calculations. The adsorption efficiency combined with the CO2/N-2 selectivity, together with a chemical and thermal stability, identifies the archetype Ti3C2 MXene as a new material for carbon capture (CC) applications.

Subject headings and genre

Added entries (persons, corporate bodies, meetings, titles ...)

  • Halim, JosephLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)josha78 (author)
  • Lind, HansLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)hanli61 (author)
  • Hansen, Thomas W.Tech Univ Denmark DTU, Denmark (author)
  • Wagner, Jakob B.Tech Univ Denmark DTU, Denmark (author)
  • Näslund, Lars-ÅkeLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)larna84 (author)
  • Darakchieva, VanyaLinköpings universitet,Halvledarmaterial,Tekniska fakulteten(Swepub:liu)vanda79 (author)
  • Palisaitis, JustinasLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)juspa01 (author)
  • Rosén, JohannaLinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)johro07 (author)
  • Persson, Per O ALinköpings universitet,Tunnfilmsfysik,Tekniska fakulteten(Swepub:liu)perpe25 (author)
  • Linköpings universitetTunnfilmsfysik (creator_code:org_t)

Related titles

  • In:Advanced Materials: WILEY-V C H VERLAG GMBH31:20935-96481521-4095

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