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Controlling Electro...
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Moser, MaximilianUniversity of Oxford, Department of Chemistry, Oxford, UK
(author)
Controlling Electrochemically Induced Volume Changes in Conjugated Polymers by Chemical Design : from Theory to Devices
- Article/chapterEnglish2021
Publisher, publication year, extent ...
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2021-04-17
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Wiley,2021
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Numbers
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LIBRIS-ID:oai:DiVA.org:liu-175346
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https://urn.kb.se/resolve?urn=urn:nbn:se:liu:diva-175346URI
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https://doi.org/10.1002/adfm.202100723DOI
Supplementary language notes
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Language:English
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Summary in:English
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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Funding agencies: KAUSTKing Abdullah University of Science & Technology; Office of Sponsored Research (OSR) [OSR-2018-CRG/CCF-3079, OSR-2019-CRG8-4086, OSR-2018-CRG7-3749]; ERC Synergy Grant SC2 [610115]; European UnionEuropean Commission [952911, 862474]; EPSRCUK Research & Innovation (UKRI)Engineering & Physical Sciences Research Council (EPSRC) [EP/T026219/1]; Knut and Alice Wallenberg FoundationKnut & Alice Wallenberg Foundation; Wallenberg Wood Science Center [KAW 2018.0452]; Swedish Government Strategic Research Area in Materials Science on Advanced Functional Materials at Linkoping University (Faculty Grant SFO-Mat-LiU) [2009-00971]; TomKat Center for Sustainable Energy at Stanford University
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Electrochemically induced volume changes in organic mixed ionic-electronic conductors (OMIECs) are particularly important for their use in dynamic microfiltration systems, biomedical machinery, and electronic devices. Although significant advances have been made to maximize the dimensional changes that can be accomplished by OMIECs, there is currently limited understanding of how changes in their molecular structures impact their underpinning fundamental processes and their performance in electronic devices. Herein, a series of ethylene glycol functionalized conjugated polymers is synthesized, and their electromechanical properties are evaluated through a combined approach of experimental measurements and molecular dynamics simulations. As demonstrated, alterations in the molecular structure of OMIECs impact numerous processes occurring during their electrochemical swelling, with sidechain length shortening decreasing the number of incorporated water molecules, reducing the generated void volumes and promoting the OMIECs to undergo different phase transitions. Ultimately, the impact of these combined molecular processes is assessed in organic electrochemical transistors, revealing that careful balancing of these phenomena is required to maximize device performance.
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Gladisch, Johannes,1987-Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten(Swepub:liu)johgl24
(author)
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Ghosh, SarbaniLinköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten,Birla Institute of Technology and Science (BITS), Department of Chemical Engineering, Pilani, India(Swepub:liu)sargh53
(author)
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Hidalgo, Tania CeciliaKing Abdullah University of Science and Technology (KAUST), Biological Sciences and Engineering Division, Thuwal, Saudi Arabia
(author)
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Ponder Jr., James F.George W. Woodruff School of Mechanical Engineering, Georgia Institute of Technology, Atlanta, GA, USA
(author)
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Sheelamanthula, RajendarKing Abdullah University of Science and Technology (KAUST), Physical Science and Engineering Division, Thuwal, Saudi Arabia
(author)
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Thiburce, QuentinStanford University, Department of Materials Science and Engineering, Stanford, CA, USA
(author)
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Gasparini, NicolaImperial College London, Department of Chemistry and Center for Plastic Electronics, London, UK
(author)
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Wadsworth, AndrewUniversity of Oxford, Department of Chemistry, Oxford, UK
(author)
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Salleo, AlbertoStanford University, Department of Materials Science and Engineering, Stanford, CA, USA
(author)
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Inal, SahikaKing Abdullah University of Science and Technology (KAUST), Biological Sciences and Engineering Division, Thuwal, Saudi Arabia
(author)
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Berggren, Magnus,1968-Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten(Swepub:liu)magbe98
(author)
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Zozoulenko, Igor,1962-Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten(Swepub:liu)igozo50
(author)
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Stavrinidou, Eleni,1986-Linköpings universitet,Laboratoriet för organisk elektronik,Tekniska fakulteten(Swepub:liu)elest58
(author)
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McCulloch, IainUniversity of Oxford, Department of Chemistry, Oxford, UK; King Abdullah University of Science and Technology (KAUST), Physical Science and Engineering Division, Thuwal, Saudi Arabia
(author)
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University of Oxford, Department of Chemistry, Oxford, UKLaboratoriet för organisk elektronik
(creator_code:org_t)
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In:Advanced Functional Materials: Wileyn/a:n/a1616-301X1616-3028
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