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Observation of Fesh...
Observation of Feshbach Resonances in the F + H2 → HF + H Reaction
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- Qiu, Minghui (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Department of Physics, Dalian Jiaotong University, P. R. China.
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- Ren, Zefeng (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Che, Li (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Dai, Dongxu (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Harich, Steven A. (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Wang, Xiuyan (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Yang, Xueming (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China
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- Xu, Chuanxiu (författare)
- Institute of Theoretical and Computational Chemistry, Department of Chemistry, Nanjing University
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- Xie, Daiqian (författare)
- Institute of Theoretical and Computational Chemistry, Department of Chemistry, Nanjing University
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- Gustafsson, Magnus (författare)
- Department of Chemistry and Biochemistry, University of Colorado, Boulder
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- Skodje, Rex T. (författare)
- Department of Chemistry and Biochemistry, University of Colorado, Boulder
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- Sun, Zhigang (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Center for Theoretical and Computational Chemistry, Dalian Institute of Chemical Physics, Dalian, Department of Computational Science, National University of Singapore
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- Zhang, Donghui (författare)
- State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Center for Theoretical and Computational Chemistry, Dalian Institute of Chemical Physics, Dalian, Department of Computational Science, National University of Singapore
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State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China, Department of Physics, Dalian Jiaotong University, P R. China. State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, People’s Republic of China (creator_code:org_t)
- American Association for the Advancement of Science (AAAS), 2006
- 2006
- Engelska.
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Ingår i: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 311:5766, s. 1440-1443
- Relaterad länk:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
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Stäng
- Reaction resonances, or transiently stabilized transition-state structures, have proven highly challenging to capture experimentally. Here, we used the highly sensitive H atom Rydberg tagging time-of-flight method to conduct a crossed molecular beam scattering study of the F + H2 → HF + H reaction with full quantum-state resolution. Pronounced forward-scattered HF products in the v′ = 2 vibrational state were clearly observed at a collision energy of 0.52 kcal/mol; this was attributed to both the ground and the first excited Feshbach resonances trapped in the peculiar HF(v′ = 3)-H′ vibrationally adiabatic potential, with substantial enhancement by constructive interference between the two resonances.
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Qiu, Minghui
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Ren, Zefeng
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Che, Li
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Dai, Dongxu
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Harich, Steven A ...
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Wang, Xiuyan
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Yang, Xueming
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Xu, Chuanxiu
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Xie, Daiqian
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Gustafsson, Magn ...
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Skodje, Rex T.
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Sun, Zhigang
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Zhang, Donghui
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