WFRF:(Ji Tuo)
Sökning: WFRF:(Ji Tuo) > Porous Metallosalen...
- Li, JingIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio 44325, United States. State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing, China (författare)
Porous Metallosalen Hypercrosslinked Ionic Polymers for Cooperative CO2 Cycloaddition Conversion
- Artikel/kapitelEngelska2020
Förlag, utgivningsår, omfång ...
- 2019-12-18
- American Chemical Society (ACS),2020
- printrdacarrier
Nummerbeteckningar
- LIBRIS-ID:oai:DiVA.org:ltu-78602
- https://urn.kb.se/resolve?urn=urn:nbn:se:ltu:diva-78602URI
- https://doi.org/10.1021/acs.iecr.9b05304DOI
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- Språk:engelska
- Sammanfattning på:engelska
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Anmärkningar
- Validerad;2020;Nivå 2;2020-04-22 (johcin)
- Metallosalen-based porous ionic polymers have the potential to combine the merits of homogeneous organometallics and heterogeneous porous ionic catalysts in carbon dioxide (CO2) cycloaddition conversion. Herein, a series of porous metallosalen hypercrosslinked ionic polymers (M-HIPs) were synthesized through a simple method. The M-HIPs with high metal and Br anion concentrations were evaluated by catalyzing CO2 cycloaddition with epoxides. Because of the cooperative effect between Br anions and metal active species in the porous channel, M-HIPs exhibited a high CO2 catalytic performance even under ambient conditions. Among the M-HIPs (M = Co, Al, Zn), Co-HIP showed the best catalytic performance for various epoxides and was stable after five runs. Density functional theory calculations support the fact that Co-HIP had the lowest energy barrier, which agreed with the experimental results.
Ämnesord och genrebeteckningar
- TEKNIK OCH TEKNOLOGIER Maskinteknik Energiteknik hsv//swe
- ENGINEERING AND TECHNOLOGY Mechanical Engineering Energy Engineering hsv//eng
- Energiteknik
- Energy Engineering
Biuppslag (personer, institutioner, konferenser, titlar ...)
- Han, YulanIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio 44325, United States State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing, China (författare)
- Ji, TuoIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio, United States (författare)
- Wu, NanhuaLuleå tekniska universitet,Energivetenskap,State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing , China(Swepub:ltu)nanwun (författare)
- Lin, HanIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio , United States (författare)
- Jiang, JunSchool of Chemistry and Materials Science, University of Science and Technology of China, Hefei, China (författare)
- Zhu, JiahuaIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio , United States (författare)
- Intelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio 44325, United States. State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing, ChinaIntelligent Composites Laboratory, Department of Chemical and Biomolecular Engineering, The University of Akron, Akron, Ohio 44325, United States State Key Laboratory of Materials-Oriented Chemical Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), College of Chemical Engineering, Nanjing Tech University, Nanjing, China (creator_code:org_t)
Sammanhörande titlar
- Ingår i:Industrial & Engineering Chemistry Research: American Chemical Society (ACS)59:2, s. 676-6840888-58851520-5045
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- Li, Jing
- Han, Yulan
- Ji, Tuo
- Wu, Nanhua
- Lin, Han
- Jiang, Jun
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- Zhu, Jiahua
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