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A window–space-directed assembly strategy for the construction of supertetrahedron-based zeolitic mesoporous metal–organic frameworks with ultramicroporous apertures for selective gas adsorption

Zhang, Lei (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China; Department of Chemistry, University of North Texas, Denton 76201, United States; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
Li, Fangfang (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
You, Jianjun (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
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Hua, Nengbin (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
Wang, Quanting (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
Si, Junhui (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
Chen, Wenzhe (författare)
College of Materials Science and Engineering, Fujian University of Technology, Fuzhou 350118, China; Collaborative Innovation Center for Intelligent and Green Mold and Die of Fujian Province, Fuzhou 350118, China
Wang, Wenjing (författare)
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
Wu, Xiaoyuan (författare)
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
Yang, Wenbin (författare)
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
Yuan, Daqiang (författare)
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China
Lu, Canzhong (författare)
CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China; Xiamen Institute of Rare Earth Materials, Chinese Academy of Sciences, Xiamen 361021, China
Liu, Yanrong (författare)
Luleå tekniska universitet,Energivetenskap
Al-Enizi, Abdullah M. (författare)
Department of Chemistry, College of Science, King Saud University, Riyadh 11451, Saudi Arabia
Nafady, Ayman (författare)
Department of Chemistry, College of Science, King Saud University, Riyadh 11451, Saudi Arabia
Ma, Shengqian (författare)
Department of Chemistry, University of North Texas, Denton 76201, United States
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 (creator_code:org_t)
Royal Society of Chemistry, 2021
2021
Engelska.
Ingår i: Chemical Science. - : Royal Society of Chemistry. - 2041-6520 .- 2041-6539. ; 12:16, s. 5767-5773
  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • Despite their scarcity due to synthetic challenges, supertetrahedron-based metal–organic frameworks (MOFs) possess intriguing architectures, diverse functionalities, and superb properties that make them in‑demand materials. Employing a new window–space-directed assembly strategy, a family of mesoporous zeolitic MOFs have been constructed herein from corner-shared supertetrahedra based on homometallic or heterometallic trimers [M3(OH/O)(COO)6] (M3 = Co3, Ni3 or Co2Ti). These MOFs consisted of close-packed truncated octahedral cages possessing a sodalite topology and large β-cavity mesoporous cages (~22 Å diameter) connected by ultramicroporous apertures (~5.6 Å diameter). Notably, the supertetrahedron-based sodalite topology MOF composed with the Co2Ti trimer exhibited high thermal and chemical stability as well as the ability to efficiently separate acetylene (C2H2) from carbon dioxide (CO2).

Ämnesord

TEKNIK OCH TEKNOLOGIER  -- Maskinteknik -- Energiteknik (hsv//swe)
ENGINEERING AND TECHNOLOGY  -- Mechanical Engineering -- Energy Engineering (hsv//eng)

Nyckelord

Energiteknik
Energy Engineering

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