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A scalable metal-organic framework as a durable physisorbent for carbon dioxide capture

Lin, Jian-Bin (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada
Nguyen, Tai T. T. (author)
Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada
Vaidhyanathan, Ramanathan (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada; Indian Institute of Science Education and Research, Dr. Homi Bhabha Road, Pashan, Pune, Maharashtra, 411008, India
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Burner, Jake (author)
Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada
Taylor, Jared M. (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada; ZoraMat Solutions Inc., Calgary, Alberta, Canada
Durekova, Hana (author)
Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada
Akhtar, Farid (author)
Luleå tekniska universitet,Materialvetenskap
Mah, Roger K. (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada; ZoraMat Solutions Inc., Calgary, Alberta, Canada
Ghaffari-Nik, Omid (author)
Svante Inc., Vancouver, British Columbia, Canada
Marx, Stefan (author)
BASF SE, Ludwigshafen am Rhein, Germany
Fylstra, Nicholas (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada
Iremonger, Simon S. (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada
Dawson, Karl W. (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada
Sarkar, Partha (author)
Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada
Hovington, Pierre (author)
Svante Inc., Vancouver, British Columbia, Canada
Rajendran, Arvind (author)
Department of Chemical and Materials Engineering, University of Alberta, Edmonton, Alberta, Canada
Woo, Tom K. (author)
Department of Chemistry and Biomolecular Science, University of Ottawa, Ottawa, Ontario, Canada
Shimizu, George K. H. (author)
Department of Chemistry, University of Calgary, Calgary, Alberta, Canada; ZoraMat Solutions Inc., Calgary, Alberta, Canada
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 (creator_code:org_t)
American Association for the Advancement of Science, 2021
2021
English.
In: Science. - : American Association for the Advancement of Science. - 0036-8075 .- 1095-9203. ; 374:6574, s. 1464-1469
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Metal-organic frameworks (MOFs) as solid sorbents for carbon dioxide (CO2) capture face the challenge of merging efficient capture with economical regeneration in a durable, scalable material. Zinc-based Calgary Framework 20 (CALF-20) physisorbs CO2 with high capacity but is also selective over water. Competitive separations on structured CALF-20 show not just preferential CO2 physisorption below 40% relative humidity but also suppression of water sorption by CO2, which was corroborated by computational modeling. CALF-20 has a low enthalpic regeneration penalty and shows durability to steam (>450,000 cycles) and wet acid gases. It can be prepared in one step, formed as composite materials, and its synthesis can be scaled to multikilogram batches.  

Subject headings

NATURVETENSKAP  -- Kemi -- Materialkemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Materials Chemistry (hsv//eng)

Keyword

Engineering Materials
Materialteknik

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