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Bacterial cellulose...
Bacterial cellulose assisted synthesis of hierarchical pompon-like SAPO-34 for CO2 adsorption
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- Gong, Jie (author)
- College of Chemical and Environmental Engineering, Jiangsu University of Technology, Changzhou, 213001, Jiangsu, PR China
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- Tong, Fei (author)
- College of Chemical and Environmental Engineering, Jiangsu University of Technology, Changzhou, 213001, Jiangsu, PR China
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- Zhang, Chunyong (author)
- College of Chemical and Environmental Engineering, Jiangsu University of Technology, Changzhou, 213001, Jiangsu, PR China
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- Nobandegani, Mojtaba Sinaei (author)
- Luleå tekniska universitet,Kemiteknik
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- Yu, Liang, 1986- (author)
- Luleå tekniska universitet,Kemiteknik
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- Zhang, Lixiong (author)
- State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemistry and Chemical Engineering, Nanjing Tech University, Nanjing, 210009, PR China
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(creator_code:org_t)
- Elsevier, 2022
- 2022
- English.
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In: Microporous and Mesoporous Materials. - : Elsevier. - 1387-1811 .- 1873-3093. ; 331
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https://doi.org/10.1...
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https://doi.org/10.1...
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Abstract
Subject headings
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- In the present work, a biosynthesis route for the preparation of hierarchical pompon-like SAPO-34 was developed. Commercially available bacterial cellulose aerogel was used as template. SiO2 loaded bacterial cellulose aerogel was used as silica source and a simple hydrothermal treatment was used for crystallization. XRD, FT-IR, SEM, TEM, N2 adsorption-desorption and TG techniques were employed to characterize the obtained samples. The hierarchical pompon-like SAPO-34 showed a spherical morphology that was comprised of nanosheets with a thickness less than 30 nm. The specific surface area of the hierarchical pompon-like SAPO-34 was 498 m2/g that was higher than the trigonal SAPO-34 crystals of 465 m2/g. The ultrasonic treatment experiment indicated a high stability of the pompon-like structure. In addition, the hierarchical pompon-like SAPO-34 exhibited a CO2 adsorption capacity of 2.26 mmol/g at 100 kPa and 298K and the corresponding CO2/CH4 ideal separation factor was 5.7, which was higher than that of trigonal SAPO-34 crystals. The saturated adsorption capacity and b-value were estimated using single site Langmuir, Toth and Sips adsorption isotherm models and the observed results were constant. Compared with trigonal SAPO-34, hierarchical pompon-like SAPO-34 displayed a higher saturated adsorption capacity, but a lower b-value.
Subject headings
- NATURVETENSKAP -- Kemi -- Materialkemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Materials Chemistry (hsv//eng)
Keyword
- Adsorption
- Aerogels
- Biochemistry
- Carbon dioxide
- Cellulose
- Crystal structure
- Morphology
- Silica gel
- B value
- Bacterial cellulose
- Biosynthesis route
- Cellulose aerogels
- CO2 adsorption
- Hierarchical pompon-like SAPO-34
- SAPO-34
- Saturated adsorption capacity
- Silica sources
- Simple+
- Biosynthesis
- Chemical Technology
- Kemisk teknologi
Publication and Content Type
- ref (subject category)
- art (subject category)
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