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Transparent and Cap...
Transparent and Capacitive Bioanode Based on Specifically Engineered Glucose Oxidase
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- Gonzalez-Arribas, Elena (författare)
- Malmö högskola,Institutionen för biomedicinsk vetenskap (BMV)
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- Pankratov, Dmitry (författare)
- Malmö högskola,Institutionen för biomedicinsk vetenskap (BMV),A.N. Bach Institute of Biochemistry, Moscow, 119071, Russian Federation; National Research Center “Kurchatov Institute”, Moscow, 123182, Russian Federation
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- Gounel, Sebastien (författare)
- CNRS, CRPP, UPR 8641, Pessac, 33600, France
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- Mano, Nicolas (författare)
- CNRS, CRPP, UPR 8641, Pessac, 33600, France
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- Blum, Zoltan (författare)
- Malmö högskola,Institutionen för biomedicinsk vetenskap (BMV)
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- Shleev, Sergey (författare)
- Malmö högskola,Institutionen för biomedicinsk vetenskap (BMV),A.N. Bach Institute of Biochemistry, Moscow, 119071, Russian Federation; National Research Center “Kurchatov Institute”, Moscow, 123182, Russian Federation
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(creator_code:org_t)
- 2016-04-13
- 2016
- Engelska.
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Ingår i: Electroanalysis. - : John Wiley & Sons. - 1040-0397 .- 1521-4109. ; 28:6, s. 1290-1297
- Relaterad länk:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
Ämnesord
Stäng
- Here the authors detail an optimized transparent capacitive glucose oxidizing bioanode, capable of supplying current densities of 10 μA cm-2 at applied potentials of 0.1 V-0.2 V vs. SCE, when continuously performing in a simple phosphate buffer, pH 7.4 and artificial human tears, both with a glucose concn. of 0.05 mM only. When operating in pulse mode, the bioanode was able to deliver current densities ≤21 μA cm-2 at the beginning of the pulse with 571 μC cm-2 total charges stored. The biogenic part of the enzymic device was a recombinant glucose oxidase mutant from Penicillium amagasakiense with high catalytic efficiency towards glucose, up to 14.5x104 M-1 s-1. The nonbiogenic part of the anodic system was based on a poly(3,4-ethylenedioxythiophene)-graphene nanocomposite, as a highly capacitive component with a capacitance d. in the 1 mF cm-2 range, multi-walled carbon nanotubes, as an addnl. nanostructuring element, and a conductive org. complex, as an electron shuttle between the redox enzyme and the electrode surface. The bioanode could potentially serve as a prototype of a double-function enzymic anode for hybrid elec. power biodevices, energizing smart contact lenses.
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- art (ämneskategori)
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