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- Dell'Angela, M. (author)
Vacuum space charge effects in sub-picosecond soft X-ray photoemission on a molecular adsorbate layer
- Article/chapterEnglish2015
Publisher, publication year, extent ...
- 2015-03-18
- AIP Publishing,2015
- printrdacarrier
Numbers
- LIBRIS-ID:oai:DiVA.org:su-118293
- https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-118293URI
- https://doi.org/10.1063/1.4914892DOI
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- Language:English
- Summary in:English
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- Vacuum space charge induced kinetic energy shifts of O 1s and Ru 3d core levels in femtosecond soft X-ray photoemission spectra (PES) have been studied at a free electron laser (FEL) for an oxygen layer on Ru(0001). We fully reproduced the measurements by simulating the in-vacuum expansion of the photoelectrons and demonstrate the space charge contribution of the high-order harmonics in the FEL beam. Employing the same analysis for 400 nm pump-X-ray probe PES, we can disentangle the delay dependent Ru 3d energy shifts into effects induced by space charge and by lattice heating from the femtosecond pump pulse.
Subject headings and genre
- NATURVETENSKAP Kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences hsv//eng
- NATURVETENSKAP Fysik hsv//swe
- NATURAL SCIENCES Physical Sciences hsv//eng
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- Anniyev, T. (author)
- Beye, M. (author)
- Coffee, R. (author)
- Foehlisch, A. (author)
- Gladh, JörgenStockholms universitet,Fysikum(Swepub:su)gladh (author)
- Kaya, S. (author)
- Katayama, T. (author)
- Krupin, O. (author)
- Nilsson, AndersStockholms universitet,Fysikum,SUNCAT Center for Interface Science and Catalysis, USA; SLAC National Accelerator Laboratory, USA(Swepub:su)andersn (author)
- Nordlund, D. (author)
- Schlotter, W. F. (author)
- Sellberg, Jonas A.Stockholms universitet,Fysikum,SUNCAT Center for Interface Science and Catalysis, USA(Swepub:su)jose4950 (author)
- Sorgenfrei, F. (author)
- Turner, J. J. (author)
- Öström, HenrikStockholms universitet,Fysikum(Swepub:su)ostrom (author)
- Ogasawara, H. (author)
- Wolf, M. (author)
- Wurth, W. (author)
- Stockholms universitetFysikum (creator_code:org_t)
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- In:Structural Dynamics: AIP Publishing2:22329-7778
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