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- Yang, Bin,1987-Stockholms universitet,Institutionen för organisk kemi (author)
Enantioselective Palladium-Catalyzed Carbonylative Carbocyclization of Enallenes via Cross-Dehydrogenative Coupling with Terminal Alkyne : Efficient Construction of a-Chirality of Ketones
- Article/chapterEnglish2017
Publisher, publication year, extent ...
- 2017-03-27
- Wiley,2017
- electronicrdacarrier
Numbers
- LIBRIS-ID:oai:DiVA.org:su-141526
- https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-141526URI
- https://doi.org/10.1002/anie.201612385DOI
Supplementary language notes
- Language:English
- Summary in:English
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- SwePubSwePub
Classification
Notes
- An enantioselective PdII/Brønsted acid-catalyzed carbonylative carbocyclization of enallenes ending with a cross-dehydrogenative coupling (CDC) with a terminal alkyne was developed. VAPOL phosphoric acid was found as the best co-catalyst among the examined 28 chiral acids, for inducing the enantioselectivity of α-chiral ketones. As a result, a number of chiral cyclopentenones were easily synthesized in good to excellent enantiomeric ratio with good yields.
Subject headings and genre
- NATURVETENSKAP Kemi Organisk kemi hsv//swe
- NATURAL SCIENCES Chemical Sciences Organic Chemistry hsv//eng
- asymmetric carbocyclization
- enallenes
- homogeneous catalysis
- oxidation
- palladium
- Organic Chemistry
- organisk kemi
Added entries (persons, corporate bodies, meetings, titles ...)
- Qiu, YouaiStockholms universitet,Institutionen för organisk kemi(Swepub:su)yoqiu (author)
- Jiang, TuoStockholms universitet,Institutionen för organisk kemi(Swepub:su)tuji1572 (author)
- Wulff, William D. (author)
- Yin, Xiaopeng (author)
- Zhu, CanStockholms universitet,Institutionen för organisk kemi(Swepub:su)zcan (author)
- Bäckvall, Jan-E.Stockholms universitet,Institutionen för organisk kemi(Swepub:su)backv (author)
- Stockholms universitetInstitutionen för organisk kemi (creator_code:org_t)
Related titles
- In:Angewandte Chemie International Edition: Wiley56:16, s. 4535-45391433-78511521-3773
Internet link
- https://su.diva-portal.org/smash/get/diva2:1087131/FULLTEXT01.pdffulltext:print
- https://su.diva-portal.org/smash/get/diva2:1087131/FULLTEXT02.pdffulltext:postprint
- http://su.diva-portal.org/smash/get/diva2:1087131/FULLTEXT02
- https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-141526
- https://doi.org/10.1002/anie.201612385
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