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  • Wang, Yu-ChengStockholms universitet,Institutionen för material- och miljökemi (MMK) (author)

Porous Carbon Membrane-Supported Atomically Dispersed Pyrrole-Type Fe-N-4 as Active Sites for Electrochemical Hydrazine Oxidation Reaction

  • Article/chapterEnglish2020

Publisher, publication year, extent ...

  • 2020-06-10
  • Wiley,2020
  • printrdacarrier

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  • LIBRIS-ID:oai:DiVA.org:su-183651
  • https://urn.kb.se/resolve?urn=urn:nbn:se:su:diva-183651URI
  • https://doi.org/10.1002/smll.202002203DOI

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  • Language:English
  • Summary in:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • The rational design of catalytically active sites in porous materials is essential in electrocatalysis. Herein, atomically dispersed Fe-N-x sites supported by hierarchically porous carbon membranes are designed to electrocatalyze the hydrazine oxidation reaction (HzOR), one of the key techniques in electrochemical nitrogen transformation. The high intrinsic catalytic activity of the Fe-N-x single-atom catalyst together with the uniquely mixed micro-/macroporous membrane support positions such an electrode among the best-known heteroatom-based carbon anodes for hydrazine fuel cells. Combined with advanced characterization techniques, electrochemical probe experiments, and density functional theory calculation, the pyrrole-type Fe-N-4 structure is identified as the real catalytic site in HzOR.

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  • Wan, Li-Yang (author)
  • Cui, Pei-Xin (author)
  • Tong, Lei (author)
  • Ke, Yu-QiStockholms universitet,Institutionen för material- och miljökemi (MMK)(Swepub:su)yuke2144 (author)
  • Sheng, Tian (author)
  • Zhang, MiaoStockholms universitet,Institutionen för material- och miljökemi (MMK)(Swepub:su)mizh4435 (author)
  • Sun, Shu-Hui (author)
  • Liang, Hai-Wei (author)
  • Wang, Yue-Sheng (author)
  • Zaghib, Karim (author)
  • Wang, Hong (author)
  • Zhou, Zhi-You (author)
  • Yuan, JiayinStockholms universitet,Institutionen för material- och miljökemi (MMK)(Swepub:su)jiyu0266 (author)
  • Stockholms universitetInstitutionen för material- och miljökemi (MMK) (creator_code:org_t)

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  • In:Small: Wiley16:311613-68101613-6829

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