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Core-valence double...
Core-valence double photoionization of the CS2 molecule
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- Andersson, Egil, 1981- (author)
- Uppsala universitet,Mjukröntgenfysik
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- Niskanen, Johannes (author)
- KTH,Teoretisk kemi
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- Hedin, Lage (author)
- Uppsala universitet,Mjukröntgenfysik
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- Eland, John H. D. (author)
- Uppsala universitet,Mjukröntgenfysik
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- Linusson, Per (author)
- Stockholms universitet,Fysikum
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- Karlsson, Leif (author)
- Uppsala universitet,Mjukröntgenfysik
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- Rubensson, Jan-Erik (author)
- Uppsala universitet,Mjukröntgenfysik
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Carravetta, V. (author)
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- Ågren, Hans (author)
- KTH,Teoretisk kemi
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- Feifel, Raimund (author)
- Uppsala universitet,Mjukröntgenfysik
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(creator_code:org_t)
- AIP Publishing, 2010
- 2010
- English.
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In: Journal of Chemical Physics. - : AIP Publishing. - 0021-9606 .- 1089-7690. ; 133:9, s. 94305-
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Abstract
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- Double photoionization spectra of the CS2 molecule have been recorded using the TOF-PEPECO technique in combination with synchrotron radiation at the photon energies h nu=220, 230, 240, 243, and 362.7 eV. The spectra were recorded in the S 2p and C 1s inner-shell ionization regions and reflect dicationic states formed out of one inner-shell vacancy and one vacancy in the valence region. MCSCF calculations were performed to model the energies of the dicationic states. The spectra associated with a S 2p vacancy are well structured and have been interpreted in some detail by comparison to conventional S 2p and valence photoelectron spectra. The lowest inner-shell-valence dicationic state is observed at the vertical double ionization energy 188.45 eV and is associated with a (2p(3/2))(-1)(2 pi(g))(-1) double vacancy. The spectrum connected to the C 1s vacancy shows a distinct line at 310.8 eV, accompanied by additional broad features at higher double ionization energies. This line is associated with a (C 1s)(-1)(2 pi(g))(-1) double vacancy. (C-) 2010 American Institute of Physics. [doi: 10.1063/1.3469812]
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
- NATURVETENSKAP -- Fysik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences (hsv//eng)
Keyword
- carbon compounds
- inner-shell ionisation
- molecule-photon collisions
- photoionisation
- SCF calculations
- NATURAL SCIENCES
- NATURVETENSKAP
- Chemistry
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Andersson, Egil, ...
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Niskanen, Johann ...
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Hedin, Lage
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Eland, John H. D ...
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Linusson, Per
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Karlsson, Leif
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show more...
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Rubensson, Jan-E ...
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Carravetta, V.
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Ågren, Hans
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Feifel, Raimund
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show less...
- About the subject
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
- Articles in the publication
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Journal of Chemi ...
- By the university
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Stockholm University
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Royal Institute of Technology
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Uppsala University