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Large pore aperture...
Large pore apertures in a series of metal organic frameworks
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Deng, Hexiang (author)
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Grunder, Sergio (author)
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Cordova, Kyle E. (author)
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Valente, Cory (author)
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Furukawa, Hiroyasu (author)
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Hmadeh, Mohamad (author)
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Gandara, Felipe (author)
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Whalley, Adam C. (author)
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Liu, Zheng (author)
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Asahina, Shunsuke (author)
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Kazumori, Hiroyoshi (author)
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O'Keeffe, Michael (author)
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- Terasaki, Osamu (author)
- Stockholms universitet,Institutionen för material- och miljökemi (MMK),NanoCentury KAIST Institute and Graduate School of Energy, Environment, Water, and Sustainability, Republic of Korea
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Stoddart, J. Fraser (author)
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Yaghi, Omar M. (author)
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(creator_code:org_t)
- American Association for the Advancement of Science (AAAS), 2012
- 2012
- English.
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In: Science. - : American Association for the Advancement of Science (AAAS). - 0036-8075 .- 1095-9203. ; 336:6084, s. 1018-1023
- Related links:
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https://urn.kb.se/re...
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https://doi.org/10.1...
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Abstract
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- We report a strategy to expand the pore aperture of metal-organic frameworks (MOFs) into a previously unattained size regime (>32 angstroms). Specifically, the systematic expansion of a well-known MOF structure, MOF-74, from its original link of one phenylene ring (I) to two, three, four, five, six, seven, nine, and eleven (II to XI, respectively), afforded an isoreticular series of MOF-74 structures (termed IRMOF-74-I to XI) with pore apertures ranging from 14 to 98 angstroms. All members of this series have non-interpenetrating structures and exhibit robust architectures, as evidenced by their permanent porosity and high thermal stability (up to 300 degrees C). The pore apertures of an oligoethylene glycol-functionalized IRMOF-74-VII and IRMOF-74-IX are large enough for natural proteins to enter the pores.
Subject headings
- NATURVETENSKAP -- Kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences (hsv//eng)
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Deng, Hexiang
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Grunder, Sergio
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Cordova, Kyle E.
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Valente, Cory
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Furukawa, Hiroya ...
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Hmadeh, Mohamad
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show more...
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Gandara, Felipe
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Whalley, Adam C.
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Liu, Zheng
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Asahina, Shunsuk ...
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Kazumori, Hiroyo ...
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O'Keeffe, Michae ...
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Terasaki, Osamu
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Stoddart, J. Fra ...
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Yaghi, Omar M.
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- NATURAL SCIENCES
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NATURAL SCIENCES
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Science
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Stockholm University