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  • Shang, YuchenState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)

Ultrahard bulk amorphous carbon from collapsed fullerene

  • Artikel/kapitelEngelska2021

Förlag, utgivningsår, omfång ...

  • 2021-11-24
  • Nature Publishing Group,2021
  • printrdacarrier

Nummerbeteckningar

  • LIBRIS-ID:oai:DiVA.org:umu-191359
  • https://urn.kb.se/resolve?urn=urn:nbn:se:umu:diva-191359URI
  • https://doi.org/10.1038/s41586-021-03882-9DOI

Kompletterande språkuppgifter

  • Språk:engelska
  • Sammanfattning på:engelska

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Klassifikation

  • Ämneskategori:ref swepub-contenttype
  • Ämneskategori:art swepub-publicationtype

Anmärkningar

  • Amorphous materials inherit short- and medium-range order from the corresponding crystal and thus preserve some of its properties while still exhibiting novel properties1,2. Due to its important applications in technology, amorphous carbon with sp2 or mixed sp2–sp3 hybridization has been explored and prepared3,4, but synthesis of bulk amorphous carbon with sp3 concentration close to 100% remains a challenge. Such materials inherit the short-/medium-range order of diamond and should also inherit its superior properties5. Here, we successfully synthesized millimetre-sized samples—with volumes 103–104 times as large as produced in earlier studies—of transparent, nearly pure sp3 amorphous carbon by heating fullerenes at pressures close to the cage collapse boundary. The material synthesized consists of many randomly oriented clusters with diamond-like short-/medium-range order and possesses the highest hardness (101.9 ± 2.3 GPa), elastic modulus (1,182 ± 40 GPa) and thermal conductivity (26.0 ± 1.3 W m−1 K−1) observed in any known amorphous material. It also exhibits optical bandgaps tunable from 1.85 eV to 2.79 eV. These discoveries contribute to our knowledge about advanced amorphous materials and the synthesis of bulk amorphous materials by high-pressure and high-temperature techniques and may enable new applications for amorphous solids.

Ämnesord och genrebeteckningar

Biuppslag (personer, institutioner, konferenser, titlar ...)

  • Liu, ZhaodongState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China; Synergetic Extreme Condition User Facility, Jilin University, Changchun, China (författare)
  • Dong, JiajunState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Yao, MingguangState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Yang, ZhenxingState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Li, QuanjunState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Zhai, ChunguangState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Shen, FangrenState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Hou, XuyuanState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China (författare)
  • Wang, LinEarth and Planets Laboratory, Carnegie Institution for Science, DC, Washington, United States; Bayerisches Geoinstitut, University of Bayreuth, Bayreuth, Germany (författare)
  • Zhang, NianqiangKey Laboratory of Structures Dynamic Behavior and Control of Ministry of Education, Harbin Institute of Technology, Harbin, China (författare)
  • Zhang, WeiKey Laboratory of Automobile Materials MOE, School of Materials Science and Engineering, Electron Microscopy Center, and International Center of Future Science, Jilin University, Changchun, China (författare)
  • Fu, RongSchool of Materials Science and Engineering, State Key Laboratory of Advanced Special Steel, Shanghai University, Shanghai, China (författare)
  • Ji, JianfengShanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai, China (författare)
  • Zhang, XingminShanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai, China (författare)
  • Lin, HeShanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai, China (författare)
  • Fei, YingweiEarth and Planets Laboratory, Carnegie Institution for Science, DC, Washington, United States (författare)
  • Sundqvist, BertilUmeå universitet,Institutionen för fysik,State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China(Swepub:umu)besu0001 (författare)
  • Wang, WeihuaInstitute of Physics, Chinese Academy of Sciences, Beijing, China (författare)
  • Liu, BingbingState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China; Synergetic Extreme Condition User Facility, Jilin University, Changchun, China (författare)
  • State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, ChinaState Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun, China; Synergetic Extreme Condition User Facility, Jilin University, Changchun, China (creator_code:org_t)

Sammanhörande titlar

  • Ingår i:Nature: Nature Publishing Group599:7886, s. 599-6040028-08361476-4687

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  • Nature (Sök värdpublikationen i LIBRIS)

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