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Mechanochemical Def...
Mechanochemical Defluorinative Acylation of ortho-Hydroxyarylenaminones by CF3-Compounds: Synthesis of 3-Acylchromones
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- Mkrtchyan, Satenik (author)
- Department of Chemistry, Faculty of Natural Sciences, Matej Bel University, Tajovského 40, 97401, Banska Bystrica, Slovakia, Tajovského 40
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- Purohit, Vishal B. (author)
- International Centre for Research on Innovative Biobased Materials (ICRI-BioM) – International Research Agenda, Lodz University of Technology, Zeromskiego 116, 90-924, Lodz, Poland, Zeromskiego 116
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- Khutsishvili, Spartak (author)
- R. Agladze Institute of Inorganic Chemistry and Electrochemistry, Ivane Javakhishvili Tbilisi State University, 11 Mindeli St., 0186, Tbilisi, Georgia, 11 Mindeli St.
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- Nociarová, Jela (author)
- Department of Chemistry, Faculty of Natural Sciences, Matej Bel University, Tajovského 40, 97401, Banska Bystrica, Slovakia, Tajovského 40; Department of Inorganic Chemistry, Faculty of Natural Sciences, Comenius University, SK-84215, Bratislava, Slovakia
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- Yar, Muhammad (author)
- COMSATS University, Department of Chemistry, Abbottabad Campus, Abbottabad, KPK, 22060, Pakistan, Abbottabad Campus, KPK
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- Mahmood, Tariq (author)
- COMSATS University, Department of Chemistry, Abbottabad Campus, Abbottabad, KPK, 22060, Pakistan, Abbottabad Campus, KPK
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- Ayub, Khurshid (author)
- COMSATS University, Department of Chemistry, Abbottabad Campus, Abbottabad, KPK, 22060, Pakistan, Abbottabad Campus, KPK
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- Budzák, Šimon (author)
- Department of Chemistry, Faculty of Natural Sciences, Matej Bel University, Tajovského 40, 97401, Banska Bystrica, Slovakia, Tajovského 40
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- Skoršepa, Marek (author)
- Department of Chemistry, Faculty of Natural Sciences, Matej Bel University, Tajovského 40, 97401, Banska Bystrica, Slovakia, Tajovského 40
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- Iaroshenko, Viktor O. (author)
- KTH,Träkemi och massateknologi,Wallenberg Wood Science Center,Department of Chemistry, Faculty of Natural Sciences, Matej Bel University, Tajovského 40, 97401, Banska Bystrica, Slovakia, Tajovského 40
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(creator_code:org_t)
- Wiley, 2023
- 2023
- English.
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In: Advanced Synthesis and Catalysis. - : Wiley. - 1615-4150 .- 1615-4169. ; 365:12, s. 2026-2035
- Related links:
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https://doi.org/10.1...
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https://urn.kb.se/re...
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Abstract
Subject headings
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- An alternative strategy for the mechanochemical defluorinative acylation of ortho-hydroxyarylenaminones has been developed to synthesise 3-acylchromones utilizing CF3-compounds via activation of the C−F bound of the trifluoromethyl group in the presence of ytterbia (Yb2O3). The current protocol tolerated a wide range of coupling substrates to access a library of diversely substituted 3-acylchromones under the mechanochemically induced domino cyclisation mode. This is the first report for the deflourinative transformation of the inert CF3 group to the corresponding carbonyl functionality under the mechanochemical conditions.
Subject headings
- NATURVETENSKAP -- Kemi -- Organisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Organic Chemistry (hsv//eng)
Keyword
- 3-Acylchromones
- Acylation
- Catalysis
- Mechanochemistry
- Methodology
Publication and Content Type
- ref (subject category)
- art (subject category)
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Mkrtchyan, Saten ...
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Purohit, Vishal ...
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Khutsishvili, Sp ...
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Nociarová, Jela
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Yar, Muhammad
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Mahmood, Tariq
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Ayub, Khurshid
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Budzák, Šimon
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Skoršepa, Marek
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Iaroshenko, Vikt ...
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Chemical Science ...
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and Organic Chemistr ...
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Advanced Synthes ...
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Royal Institute of Technology