WFRF:(Schubert Ulrich S.)
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A multidonor-photosensitizer-multiacceptor triad for long-lived directional charge separation
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- Schlotthauer, Tina (author)
- Friedrich Schiller Univ Jena, Lab Organ & Macromol Chem IOMC, Humboldtstr 10, D-07743 Jena, Germany.
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- Schroot, Robert (author)
- Friedrich Schiller Univ Jena, Lab Organ & Macromol Chem IOMC, Humboldtstr 10, D-07743 Jena, Germany.
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- Glover, Starla (author)
- Uppsala universitet,Fysikalisk kemi
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- Friedrich Schiller Univ Jena, Lab Organ & Macromol Chem IOMC, Humboldtstr 10, D-07743 Jena, Germany Fysikalisk kemi (creator_code:org_t)
- 2017
- 2017
- English.
- In: Physical Chemistry, Chemical Physics - PCCP. - : Royal Society of Chemistry (RSC). - 1463-9076 .- 1463-9084. ; 19:42, s. 28572-28578
- Journal article (peer-reviewed)
Abstract
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- The modular assembly of a directional photoredox-active multidonor-photosensitizer-multiacceptor (Dn-P-A(m)) architecture is presented. The triad assembly features a central Ru(II) sensitizer equipped with pendant polymer chains consisting of multiple triarylamine (pTARA) and naphthalene diimide (pNDI) units, respectively. Upon excitation, the efficient formation (496%) of charge separation (CS) was observed featuring similar CS lifetimes (400 ns) as related molecular triads. In contrast, a significant additional longer-lived CS component (2400 ns, 30%) is observed indicating multiple contributing pathways.
Subject headings
- NATURVETENSKAP -- Kemi -- Fysikalisk kemi (hsv//swe)
- NATURAL SCIENCES -- Chemical Sciences -- Physical Chemistry (hsv//eng)
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