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Enhancing PbS Colloidal Quantum Dot Tandem Solar Cell Performance by Graded Band Alignment

Gao, Yijun (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Zheng, Jianghui (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Chen, Weijian (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia;Swinburne Univ Technol, Ctr Translat Atomat, Hawthorn, Vic 3122, Australia
visa fler...
Yuan, Lin (författare)
Uppsala universitet,Fysikalisk kemi,Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Teh, Zhi Li (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Yang, Jianfeng (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Cui, Xin (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Conibeer, Gavin (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Patterson, Robert (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia
Huang, Shujuan (författare)
Univ New South Wales, Australian Ctr Adv Photovolta, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia;Macquarie Univ, Sch Engn, Sydney, NSW 2109, Australia
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 (creator_code:org_t)
2019-09-12
2019
Engelska.
Ingår i: The Journal of Physical Chemistry Letters. - : American Chemical Society (ACS). - 1948-7185. ; 10:19, s. 5729-5734
  • Tidskriftsartikel (refereegranskat)
Abstract Ämnesord
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  • Colloidal quantum dot solids are attractive candidates for tandem solar cells because of their widely tunable bandgaps. However, the development of the quantum dot tandem solar cell has lagged far behind that of its single-junction counterpart. One of the fundamental problems with colloidal quantum dot solar cells is the relatively small diffusion length, which limits the quantum dot absorbing layer thickness and hence the power conversion efficiency. In this research, guided by optical modeling and utilizing a graded band alignment strategy, a two-terminal monolithic solution-processed quantum dot tandem solar cell has been successfully fabricated and a power conversion efficiency of 6.8% has been achieved. The band grading approach utilized the complementary tuning of work functions and band alignment through judicious choices of the nanoparticle surface chemistry and quantum dot confined size. This work demonstrates a general approach to improving the efficiency for tandem thin-film solar cells.

Ämnesord

NATURVETENSKAP  -- Kemi -- Fysikalisk kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Physical Chemistry (hsv//eng)
NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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