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Resonant Inelastic X-Ray Scattering Reveals Hidden Local Transitions of the Aqueous OH Radical

Kjellsson, Ludvig (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik
Nanda, K. D. (author)
Univ Southern Calif, Dept Chem, Los Angeles, CA 90007 USA.
Rubensson, Jan-Erik (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik
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Doumy, G. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
Southworth, S. H. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
Ho, P. J. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
March, A. M. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
Al Haddad, A. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
Kumagai, Y. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
Tu, M-F (author)
Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA.;Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.
Schaller, R. D. (author)
Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA.;Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.
Debnath, T. (author)
Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.
Yusof, M. S. Bin Mohd (author)
Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.
Arnold, C. (author)
DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-20146 Hamburg, Germany.;Hamburg Ctr Ultrafast Imaging, D-22607 Hamburg, Germany.
Schlotter, W. F. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.
Moeller, S. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.
Coslovich, G. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.
Koralek, J. D. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.
Minitti, M. P. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.
Vidal, M. L. (author)
Tech Univ Denmark, DTU Chem Dept Chem, DK-2800 Lyngby, Denmark.
Simon, M. (author)
Sorbonne Univ, F-75252 Paris 05, France.;CNRS, Lab Chim Phys Matiere & Rayonnement, F-75252 Paris 05, France.
Santra, R. (author)
DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-20146 Hamburg, Germany.;Hamburg Ctr Ultrafast Imaging, D-22607 Hamburg, Germany.
Loh, Z-H (author)
Nanyang Technol Univ, Div Chem & Biol Chem, Singapore 639798, Singapore.
Coriani, S. (author)
Tech Univ Denmark, DTU Chem Dept Chem, DK-2800 Lyngby, Denmark.
Krylov, A. , I (author)
Young, L. (author)
Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.;Univ Chicago, Dept Phys, Chicago, IL 60637 USA.;Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.
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 (creator_code:org_t)
AMER PHYSICAL SOC, 2020
2020
English.
In: Physical Review Letters. - : AMER PHYSICAL SOC. - 0031-9007 .- 1079-7114. ; 124:23
Related links:
https://urn.kb.se/re...
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https://doi.org/10.1...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Resonant inelastic x-ray scattering (RIXS) provides remarkable opportunities to interrogate ultra-fast dynamics in liquids. Here we use RIXS to study the fundamentally and practically important hydroxyl radical in liquid water, OH(aq). Impulsive ionization of pure liquid water produced a short-lived population of OH(aq), which was probed using femtosecond x-rays from an x-ray free-electron laser. We find that RIXS reveals localized electronic transitions that are masked in the ultraviolet absorption spectrum by strong charge-transfer transitions-thus providing a means to investigate the evolving electronic structure and reactivity of the hydroxyl radical in aqueous and heterogeneous environments. First-principles calculations provide interpretation of the main spectral features.

Subject headings

NATURVETENSKAP  -- Kemi -- Fysikalisk kemi (hsv//swe)
NATURAL SCIENCES  -- Chemical Sciences -- Physical Chemistry (hsv//eng)
NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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