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Orbital dynamics during an ultrafast insulator to metal transition

Parchenko, Sergii (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.;Swiss Fed Inst Technol, Lab Mesoscop Syst, Dept Mat, CH-8093 Zurich, Switzerland.;Paul Scherrer Inst, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Paris, Eugenio (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
McNally, Daniel (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
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Abreu, Elsa (author)
Swiss Fed Inst Technol, Inst Quantum Elect, CH-8093 Zurich, Switzerland.
Dantz, Markus (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Bothschafter, Elisabeth M. (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Reid, Alexander H. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Schlotter, William F. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Lin, Ming-Fu (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Wandel, Scott F. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Coslovich, Giacomo (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Zohar, Sioan (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Dakovski, Georgi L. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Turner, J. J. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.;SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.;Stanford Univ, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Moeller, S. (author)
SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA.,Stanford Linear Accelerator Center (SLAC)
Tseng, Yi (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Radovic, Milan (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Saathe, Conny (author)
Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory
Agåker, Marcus (author)
Uppsala University,Lund University,Lunds universitet,Uppsala universitet,Molekyl- och kondenserade materiens fysik,Lund Univ, MAX IV Lab, Box 118, SE-22100 Lund, Sweden.,MAX IV-laboratoriet,MAX IV Laboratory
Nordgren, Joseph (author)
Uppsala University,Uppsala universitet,Molekyl- och kondenserade materiens fysik
Johnson, Steven L. (author)
Swiss Fed Inst Technol, Inst Quantum Elect, CH-8093 Zurich, Switzerland.;Paul Scherrer Inst, SwissFEL, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Schmitt, Thorsten (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
Staub, Urs (author)
Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.,Paul Scherrer Institute
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Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland;Swiss Fed Inst Technol, Lab Mesoscop Syst, Dept Mat, CH-8093 Zurich, Switzerland.;Paul Scherrer Inst, CH-5232 Villigen, Switzerland. Paul Scherrer Institute (creator_code:org_t)
AMER PHYSICAL SOC, 2020
2020
English.
In: Physical Review Research. - : AMER PHYSICAL SOC. - 2643-1564. ; 2:2
Related links:
https://doi.org/10.1...
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https://uu.diva-port... (primary) (Raw object)
http://dx.doi.org/10... (free)
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https://doi.org/10.1...
https://lup.lub.lu.s...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • We present ultrafast resonant inelastic x-ray scattering (RIXS) experiments performed at the vanadium L edge to track changes in the electronic structure of V2O3, a classical Mott-Hubbard material. The probed orbital excitations within the d shell of the V ion show a sub-ps time response, which evolves at later times to a state that appears electronically indistinguishable from the high-temperature metallic state. For low excitation fluences, a transient recovery or delay is observed, which could be related to a transient dimerization of the V-V bonds. Our results demonstrate the great potential for RIXS spectroscopy to study the ultrafast orbital dynamics in strongly correlated materials.

Subject headings

NATURVETENSKAP  -- Fysik -- Den kondenserade materiens fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Condensed Matter Physics (hsv//eng)

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