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  • Patra Kumar, KajwalUppsala universitet,Kemisk och biomolekylär fysik (author)

Ultrafast dynamics and scattering of protic ionic liquids induced by XFEL pulses

  • Article/chapterEnglish2021

Publisher, publication year, extent ...

  • International Union Of Crystallography,2021
  • electronicrdacarrier

Numbers

  • LIBRIS-ID:oai:DiVA.org:uu-456491
  • https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-456491URI
  • https://doi.org/10.1107/S1600577521007657DOI

Supplementary language notes

  • Language:English
  • Summary in:English

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  • Subject category:ref swepub-contenttype
  • Subject category:art swepub-publicationtype

Notes

  • X-rays are routinely used for structural studies through scattering, and femtosecond X-ray lasers can probe ultrafast dynamics. We aim to capture the femtosecond dynamics of liquid samples using simulations and deconstruct the interplay of ionization and atomic motion within the X-ray laser pulse. This deconstruction is resolution dependent, as ionization influences the low momentum transfers through changes in scattering form factors, while atomic motion has a greater effect at high momentum transfers through loss of coherence. Our methodology uses a combination of classical molecular dynamics and plasma simulation on a protic ionic liquid to quantify the contributions to the scattering signal and how these evolve with time during the X-ray laser pulse. Our method is relevant for studies of organic liquids, biomolecules in solution or any low-Z materials at liquid densities that quickly turn into a plasma while probed with X-rays.

Subject headings and genre

Added entries (persons, corporate bodies, meetings, titles ...)

  • Dawod, Ibrahim EliahUppsala universitet,Kemisk och biomolekylär fysik,Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden.;European XFEL, Holzkoppel 4, DE-22869 Schenefeld, Germany.(Swepub:uu)ibrel100 (author)
  • Martin, Andrew, VRMIT Univ, Sch Sci, 124 La Trobe St, Melbourne, Vic 3000, Australia. (author)
  • Greaves, Tamar L.RMIT Univ, Sch Sci, 124 La Trobe St, Melbourne, Vic 3000, Australia. (author)
  • Persson, DanielUppsala universitet,Avdelningen för beräkningsvetenskap(Swepub:uu)daper021 (author)
  • Caleman, CarlUppsala universitet,Molekylär biofysik,Kemisk och biomolekylär fysik,Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden.;DESY, Ctr Free Electron Laser Sci, Notkestr 85, DE-22607 Hamburg, Germany.(Swepub:uu)cajca839 (author)
  • Timneanu, NicusorUppsala universitet,Molekylär biofysik,Kemisk och biomolekylär fysik,Uppsala Univ, Dept Phys & Astron, Box 516, SE-75120 Uppsala, Sweden.(Swepub:uu)nti19847 (author)
  • Uppsala universitetKemisk och biomolekylär fysik (creator_code:org_t)

Related titles

  • In:Journal of Synchrotron Radiation: International Union Of Crystallography28:5, s. 1296-13080909-04951600-5775

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