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Search: WFRF:(Eland John H. D. 1941) > (2018) > Acetylacetone photo...

Acetylacetone photodynamics at a seeded free-electron laser

Squibb, Richard J. (author)
Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, SE-41296 Gothenburg, Sweden.
Sapunar, M. (author)
Inst Ruder Boskov, Bijenicka Cesta 54, Zagreb 10000, Croatia.
Ponzi, A. (author)
Inst Ruder Boskov, Bijenicka Cesta 54, Zagreb 10000, Croatia.
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Richter, R. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.,Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, F-75005 Paris 05, France.,Univ Gothenburg, Dept Phys, Origovagen 6B, SE-41296 Gothenburg, Sweden.
Kivimäki, A. (author)
CNR, Ist Officina Mat, I-34149 Trieste, Italy.
Plekan, O. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.
Finetti, P. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.
Sisourat, N. (author)
Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, F-75005 Paris 05, France.
Zhaunerchyk, Vitali (author)
Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, SE-41296 Gothenburg, Sweden.
Marchenko, T. (author)
Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, F-75005 Paris 05, France.
Journel, L. (author)
Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, F-75005 Paris 05, France.
Guillemin, R. (author)
Cucini, R. (author)
Coreno, M. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.;CNR, Ist Struttura Matter, LD2 Unit, I-34149 Trieste, Italy.
Grazioli, C. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.;CNR, Ist Struttura Matter, LD2 Unit, I-34149 Trieste, Italy.
Di Fraia, M. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.;CNR, Ist Struttura Matter, LD2 Unit, I-34149 Trieste, Italy.
Callegari, C. (author)
Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.;CNR, Ist Struttura Matter, LD2 Unit, I-34149 Trieste, Italy.,Elettra Sincrotrone Trieste, Str Statale 14 Km 163-5, I-34149 Trieste, Italy.;Swinburne Univ Technol, Dept Chem & Biotechnol, Mol Model Discovery Lab, Melbourne, Vic 3122, Australia.
Prince, K.C. (author)
Decleva, P. (author)
CNR, Ist Officina Mat, I-34149 Trieste, Italy.;Univ Trieste, Dipartimento Sci Chim & Farmaceut, I-34127 Trieste, Italy.
Simon, M. (author)
Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, F-75005 Paris 05, France.
Eland, John H. D., 1941 (author)
Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, SE-41296 Gothenburg, Sweden.;Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, South Parks Rd, Oxford OX1 3QZ, England.
Doslic, N. (author)
Inst Ruder Boskov, Bijenicka Cesta 54, Zagreb 10000, Croatia.
Feifel, Raimund (author)
Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)
Piancastelli, Maria Novella (author)
Uppsala universitet,Molekyl- och kondenserade materiens fysik,Sorbonne Univ, UPMC Univ Paris 06, CNRS,UMR 7614, Lab Chim Phy Matiere & Rayonnement, Paris, France
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 (creator_code:org_t)
2018-01-04
2018
English.
In: Nature Communications. - : Springer Science and Business Media LLC. - 2041-1723. ; 9
Related links:
https://gup.ub.gu.se... (primary) (free)
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https://www.nature.c...
https://gup.ub.gu.se...
https://doi.org/10.1...
https://urn.kb.se/re...
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  • Journal article (peer-reviewed)
Abstract Subject headings
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  • Thefirst steps in photochemical processes, such as photosynthesis or animal vision, involvechanges in electronic and geometric structure on extremely short time scales. Time-resolvedphotoelectron spectroscopy is a natural way to measure such changes, but has been hinderedhitherto by limitations of available pulsed light sources in the vacuum-ultraviolet and soft X-ray spectral region, which have insufficient resolution in time and energy simultaneously. Theunique combination of intensity, energy resolution, and femtosecond pulse duration of theFERMI-seeded free-electron laser can now provide exceptionally detailed information onphotoexcitation–deexcitation and fragmentation in pump-probe experiments on the 50-femtosecond time scale. For the prototypical system acetylacetone we report here electronspectra measured as a function of time delay with enough spectral and time resolution tofollow several photoexcited species through well-characterized individual steps, interpretedusing state-of-the-art static and dynamics calculations. These results open the way forinvestigations of photochemical processes in unprecedented detail.

Subject headings

NATURVETENSKAP  -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
NATURVETENSKAP  -- Fysik (hsv//swe)
NATURAL SCIENCES  -- Physical Sciences (hsv//eng)

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art (subject category)

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