Search: WFRF:(Robb A.) >
Correlation-Driven ...
-
Barillot, T.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
Correlation-Driven Transient Hole Dynamics Resolved in Space and Time in the Isopropanol Molecule
- Article/chapterEnglish2021
Publisher, publication year, extent ...
-
American Physical Society,2021
Numbers
-
LIBRIS-ID:oai:gup.ub.gu.se/307593
-
https://gup.ub.gu.se/publication/307593URI
-
https://doi.org/10.1103/PhysRevX.11.031048DOI
-
https://lup.lub.lu.se/record/c91298de-d6c6-42a6-bd5d-5e0af878edfbURI
-
https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-455870URI
Supplementary language notes
Part of subdatabase
Classification
-
Subject category:ref swepub-contenttype
-
Subject category:art swepub-publicationtype
Notes
-
The possibility of suddenly ionized molecules undergoing extremely fast electron hole (or hole) dynamics prior to significant structural change was first recognized more than 20 years ago and termed charge migration. The accurate probing of ultrafast electron hole dynamics requires measurements that have both sufficient temporal resolution and can detect the localization of a specific hole within the molecule. We report an investigation of the dynamics of inner valence hole states in isopropanol where we use an x-ray pump-x-ray probe experiment, with site and state-specific probing of a transient hole state localized near the oxygen atom in the molecule, together with an ab initio theoretical treatment. We record the signature of transient hole dynamics and make the first tentative observation of dynamics driven by frustrated Auger-Meitner transitions. We verify that the effective hole lifetime is consistent with our theoretical prediction. This state-specific measurement paves the way to widespread application for observations of transient hole dynamics localized in space and time in molecules and thus to charge transfer phenomena that are fundamental in chemical and material physics.
Subject headings and genre
Added entries (persons, corporate bodies, meetings, titles ...)
-
Alexander, O.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Cooper, B.Imperial College London,University College London,Paul Scherrer Institute,Argonne National Laboratory,Swiss Federal Institute of Technology,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.;UCL, Dept Phys & Astron, Atom Mol Opt & Positron Phys Grp, Gower St, London WC1E 6BT, England.,Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.;Paul Scherrer Inst, CH-5232 Villigen, Switzerland.;Ecole Polytech Fed Lausanne EPFL, LUXS Lab Ultrafast Xray Sci, Inst Chem Sci & Engn, CH-1015 Lausanne, Switzerland.
(author)
-
Driver, T.Stanford Linear Accelerator Center (SLAC),Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.;SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA.;SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
(author)
-
Garratt, D.Imperial College London,Argonne National Laboratory,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.,Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
(author)
-
Li, S.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Accelerator Directorate, Menlo Pk, CA 94025 USA.
(author)
-
Al Haddad, A.Argonne National Laboratory,Paul Scherrer Institute,Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.;Paul Scherrer Inst, CH-5232 Villigen, Switzerland.
(author)
-
Sanchez-Gonzalez, A.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Agåker, M.Uppsala universitet,Uppsala University,Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory,Stanford Linear Accelerator Center (SLAC),Kemisk och biomolekylär fysik,Lund Univ, MAX IV Lab, Box 118, SE-22100 Lund, Sweden.,SLAC Natl Accelerator Lab, Accelerator Directorate, Menlo Pk, CA 94025 USA.(Swepub:uu)maaga227
(author)
-
Arrell, C.Paul Scherrer Institute,Swiss Federal Institute of Technology,Paul Scherrer Inst, CH-5232 Villigen, Switzerland.,Ecole Polytech Fed Lausanne, Lab Mol Nanodynam, CH-1015 Lausanne, Switzerland.
(author)
-
Bearpark, M. J.Imperial College London,Imperial Coll London, Dept Chem, Mol Sci Res Hub, London W12 0BZ, England.
(author)
-
Berrah, N.University of Connecticut,Univ Connecticut, Dept Phys, Storrs, CT 06268 USA.
(author)
-
Bostedt, C.
(author)
-
Bozek, J.Orme Merisiers, Synchrotron SOLEIL, BP 48, F-91192 Gif Sur Yvette, France.
(author)
-
Brahms, C.
(author)
-
Bucksbaum, P. H.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA.
(author)
-
Clark, A.
(author)
-
Doumy, G.
(author)
-
Feifel, RaimundUniversity of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, S-41258 Gothenburg, Sweden.(Swepub:gu)xfeira
(author)
-
Frasinski, L. J.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Squibb, Richard J.Gothenburg University,Göteborgs universitet,University of Gothenburg,Institutionen för fysik (GU),Department of Physics (GU),Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.,Univ Gothenburg, Dept Phys, Origovagen 6B, S-41258 Gothenburg, Sweden.(Swepub:gu)xsquri
(author)
-
Johnson, A. S.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Kjellsson, L.Uppsala universitet,Uppsala University,Kemisk och biomolekylär fysik(Swepub:uu)ludkj681
(author)
-
Kolorenč, P.Charles University in Prague,Charles Univ Prague, Fac Math & Phys, Inst Theoret Phys, V Holesovickach 2, Prague 18000, Czech Republic.
(author)
-
Kumagai, Y.Argonne National Laboratory,Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.
(author)
-
Larsen, E. W.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.(Swepub:lu)fysi-ewe
(author)
-
Matia-Hernando, P.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Robb, M.Imperial College London,Imperial Coll London, Dept Chem, Mol Sci Res Hub, London W12 0BZ, England.
(author)
-
Rubensson, Jan-ErikUppsala universitet,Uppsala University,Kemisk och biomolekylär fysik(Swepub:uu)janerube
(author)
-
Ruberti, M.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Sathe, C.Lund University,Lunds universitet,MAX IV-laboratoriet,MAX IV Laboratory,Lund Univ, MAX IV Lab, Box 118, SE-22100 Lund, Sweden.(Swepub:lu)maxl-cos
(author)
-
Squibb, Richard J.Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU)(Swepub:gu)xsquri
(author)
-
Tan, A.Imperial College London,Stanford Linear Accelerator Center (SLAC),Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.,SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA.
(author)
-
Tisch, J. W.G.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Vacher, M.Imperial College London,University of Nantes,Imperial Coll London, Dept Chem, Mol Sci Res Hub, London W12 0BZ, England.;Univ Nantes, CNRS, CEISAM UMR 6230, F-44000 Nantes, France.
(author)
-
Walke, D. J.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Wolf, T. J.A.
(author)
-
Wood, D.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Zhaunerchyk, VitaliUniversity of Gothenburg,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Univ Gothenburg, Dept Phys, Origovagen 6B, S-41258 Gothenburg, Sweden.(Swepub:gu)xzhavi
(author)
-
Walter, P.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
(author)
-
Osipov, T.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
(author)
-
Marinelli, A.
(author)
-
Maxwell, T. J.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Accelerator Directorate, Menlo Pk, CA 94025 USA.
(author)
-
Coffee, R.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
(author)
-
Lutman, A. A.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Accelerator Directorate, Menlo Pk, CA 94025 USA.
(author)
-
Averbukh, V.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Ueda, K.Tohoku University,Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan.;Tohoku Univ, Dept Chem, Aoba Ku, 6-3 Aramaki Aza Aoba, Sendai, Miyagi 9808578, Japan.
(author)
-
Cryan, J. P.Stanford Linear Accelerator Center (SLAC),SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA.;SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA.
(author)
-
Marangos, J. P.Imperial College London,Imperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(author)
-
Imperial College LondonImperial Coll London, Blackett Lab, Quantum Opt & Laser Sci Grp, London SW7 2BW, England.
(creator_code:org_t)
Related titles
-
In:Physical Review X: American Physical Society11:32160-3308
Internet link
Find in a library
To the university's database
- By the author/editor
-
Barillot, T.
-
Alexander, O.
-
Cooper, B.
-
Driver, T.
-
Garratt, D.
-
Li, S.
-
show more...
-
Al Haddad, A.
-
Sanchez-Gonzalez ...
-
Agåker, M.
-
Arrell, C.
-
Bearpark, M. J.
-
Berrah, N.
-
Bostedt, C.
-
Bozek, J.
-
Brahms, C.
-
Bucksbaum, P. H.
-
Clark, A.
-
Doumy, G.
-
Feifel, Raimund
-
Frasinski, L. J.
-
Squibb, Richard ...
-
Johnson, A. S.
-
Kjellsson, L.
-
Kolorenč, P.
-
Kumagai, Y.
-
Larsen, E. W.
-
Matia-Hernando, ...
-
Robb, M.
-
Rubensson, Jan-E ...
-
Ruberti, M.
-
Sathe, C.
-
Tan, A.
-
Tisch, J. W.G.
-
Vacher, M.
-
Walke, D. J.
-
Wolf, T. J.A.
-
Wood, D.
-
Zhaunerchyk, Vit ...
-
Walter, P.
-
Osipov, T.
-
Marinelli, A.
-
Maxwell, T. J.
-
Coffee, R.
-
Lutman, A. A.
-
Averbukh, V.
-
Ueda, K.
-
Cryan, J. P.
-
Marangos, J. P.
-
show less...
- About the subject
-
- NATURAL SCIENCES
-
NATURAL SCIENCES
-
and Physical Science ...
-
and Atom and Molecul ...
-
- NATURAL SCIENCES
-
NATURAL SCIENCES
-
and Physical Science ...
-
and Condensed Matter ...
- Articles in the publication
-
Physical Review ...
- By the university
-
University of Gothenburg
-
Lund University
-
Uppsala University