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UV-induced dissocia...
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Kockert, HansjochenUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
UV-induced dissociation of CH2BrI probed by intense femtosecond XUV pulses
- Article/chapterEnglish2022
Publisher, publication year, extent ...
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2022-02-11
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IOP Publishing,2022
Numbers
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LIBRIS-ID:oai:gup.ub.gu.se/335665
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https://gup.ub.gu.se/publication/335665URI
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https://doi.org/10.1088/1361-6455/ac489dDOI
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https://urn.kb.se/resolve?urn=urn:nbn:se:uu:diva-469221URI
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https://lup.lub.lu.se/record/28617817-770f-46d5-8668-defb902d2352URI
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Subject category:ref swepub-contenttype
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Subject category:art swepub-publicationtype
Notes
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The ultraviolet (UV)-induced dissociation and photofragmentation of gas-phase CH2BrI molecules induced by intense femtosecond extreme ultraviolet (XUV) pulses at three different photon energies are studied by multi-mass ion imaging. Using a UV-pump-XUV-probe scheme, charge transfer between highly charged iodine ions and neutral CH2Br radicals produced by C-I bond cleavage is investigated. In earlier charge-transfer studies, the center of mass of the molecules was located along the axis of the bond cleaved by the pump pulse. In the present case of CH2BrI, this is not the case, thus inducing a rotation of the fragment. We discuss the influence of the rotation on the charge transfer process using a classical over-the-barrier model. Our modeling suggests that, despite the fact that the dissociation is slower due to the rotational excitation, the critical interatomic distance for charge transfer is reached faster. Furthermore, we suggest that charge transfer during molecular fragmentation may be modulated in a complex way.
Subject headings and genre
Added entries (persons, corporate bodies, meetings, titles ...)
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Lee, Jason W. L.Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.;Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,University of Oxford,German Electron Synchrotron (DESY)
(author)
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Allum, FelixUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
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Amini, KasraUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
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Bari, SadiaDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Bomme, CedricDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Brausse, FelixMax Born Inst, D-12489 Berlin, Germany.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy
(author)
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Brouard, MarkUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
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Burt, MichaelUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
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de Miranda, Barbara CunhaSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Duesterer, StefanDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Eng-Johnsson, PerLund University,Lunds universitet,Lunds lasercentrum, LLC,Annan verksamhet, LTH,Lunds Tekniska Högskola,Atomfysik,Fysiska institutionen,Institutioner vid LTH,LTH profilområde: Avancerade ljuskällor,LTH profilområden,Lund Laser Centre, LLC,Other operations, LTH,Faculty of Engineering, LTH,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH(Swepub:lu)fysi-pj0
(author)
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Erk, BenjaminDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Geleoc, MarieUniv Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay
(author)
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Geneaux, RomainUniv Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay
(author)
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Gentleman, Alexander S.Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England.,University of Oxford
(author)
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Guillemin, RenaudSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Goldsztejn, GildasMax Born Inst, D-12489 Berlin, Germany.;Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy,Paris-Sorbonne University
(author)
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Holland, David M. P.Daresbury Lab, Warrington WA4 4AD, Cheshire, England.,Daresbury Laboratory
(author)
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Ismail, IyasSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Journel, LoicSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Kierspel, ThomasDeutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany.,University of Hamburg
(author)
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Kuepper, JochenDeutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany.;Univ Hamburg, Ctr Ultrafast Imaging, D-22761 Hamburg, Germany.;Univ Hamburg, Dept Chem, D-20146 Hamburg, Germany.,University of Hamburg
(author)
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Lahl, JanLund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-jlh
(author)
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Mackenzie, Stuart R.Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England.,University of Oxford
(author)
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Maclot, Sylvain,1986Lund University,Lunds universitet,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Lund Univ, Dept Phys, S-22100 Lund, Sweden.;Gothenburg Univ, Dept Phys, Box 100, S-40530 Gothenburg, Sweden.,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH(Swepub:lu)fysi-sam
(author)
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Manschwetus, BastianDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Mereshchenko, Andrey S.St Petersburg State Univ, St Petersburg 199034, Russia.,Saint Petersburg State University
(author)
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Mullins, TerenceDeutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.
(author)
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Olshin, Pavel K.St Petersburg State Univ, St Petersburg 199034, Russia.,Saint Petersburg State University
(author)
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Palaudoux, JérômeSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,The French National Centre for Scientific Research (CNRS),Paris-Sorbonne University(Swepub:lu)maxl-jop
(author)
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Penent, FrancisSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Piancastelli, Maria NovellaUppsala University,Uppsala universitet,Kemisk och biomolekylär fysik,Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University(Swepub:uu)mpi06700
(author)
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Rompotis, DimitriosDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.,German Electron Synchrotron (DESY),European XFEL GmbH
(author)
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Rouzee, ArnaudMax Born Inst, D-12489 Berlin, Germany.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy
(author)
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Ruchon, ThierryUniv Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay(Swepub:lu)fysi-tru
(author)
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Rudenko, ArtemKansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
(author)
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Schirmel, NoraDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Simon, MarcSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Techert, SimoneDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
(author)
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Travnikova, OksanaSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Trippel, SebastianDeutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Ctr Ultrafast Imaging, D-22761 Hamburg, Germany.,University of Hamburg
(author)
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Vallance, ClaireUniv Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
(author)
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Wang, EnliangKansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
(author)
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Wiese, JossDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Chem, D-20146 Hamburg, Germany.,University of Hamburg
(author)
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Ziaee, FarzanehKansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
(author)
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Marchenko, TatianaSorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
(author)
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Rolles, DanielKansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
(author)
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Boll, RebeccaDeutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.,German Electron Synchrotron (DESY),European XFEL GmbH
(author)
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Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.University of Oxford
(creator_code:org_t)
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In:JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS: IOP Publishing55:10953-40751361-6455
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Kockert, Hansjoc ...
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Lee, Jason W. L.
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Allum, Felix
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Amini, Kasra
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Bari, Sadia
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Bomme, Cedric
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Brausse, Felix
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Brouard, Mark
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Burt, Michael
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de Miranda, Barb ...
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Duesterer, Stefa ...
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Eng-Johnsson, Pe ...
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Erk, Benjamin
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Geleoc, Marie
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Geneaux, Romain
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Gentleman, Alexa ...
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Guillemin, Renau ...
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Goldsztejn, Gild ...
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Holland, David M ...
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Ismail, Iyas
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Journel, Loic
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Kierspel, Thomas
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Kuepper, Jochen
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Lahl, Jan
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Mackenzie, Stuar ...
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Maclot, Sylvain, ...
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Manschwetus, Bas ...
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Mereshchenko, An ...
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Mullins, Terence
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Olshin, Pavel K.
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Palaudoux, Jérôm ...
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Penent, Francis
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Piancastelli, Ma ...
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Rompotis, Dimitr ...
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Rouzee, Arnaud
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Ruchon, Thierry
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Rudenko, Artem
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Schirmel, Nora
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Simon, Marc
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Techert, Simone
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Travnikova, Oksa ...
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Trippel, Sebasti ...
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Vallance, Claire
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Wang, Enliang
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Wiese, Joss
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Ziaee, Farzaneh
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Marchenko, Tatia ...
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Rolles, Daniel
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Boll, Rebecca
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