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UV-induced dissocia...
UV-induced dissociation of CH2BrI probed by intense femtosecond XUV pulses
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- Kockert, Hansjochen (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- Lee, Jason W. L. (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.;Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,University of Oxford,German Electron Synchrotron (DESY)
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- Allum, Felix (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- Amini, Kasra (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- Bari, Sadia (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Bomme, Cedric (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Brausse, Felix (author)
- Max Born Inst, D-12489 Berlin, Germany.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy
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- Brouard, Mark (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- Burt, Michael (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- de Miranda, Barbara Cunha (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Duesterer, Stefan (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Eng-Johnsson, Per (author)
- Lund University,Lunds universitet,Lunds lasercentrum, LLC,Annan verksamhet, LTH,Lunds Tekniska Högskola,Atomfysik,Fysiska institutionen,Institutioner vid LTH,LTH profilområde: Avancerade ljuskällor,LTH profilområden,Lund Laser Centre, LLC,Other operations, LTH,Faculty of Engineering, LTH,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH,LTH Profile Area: Photon Science and Technology,LTH Profile areas,Faculty of Engineering, LTH
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- Erk, Benjamin (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Geleoc, Marie (author)
- Univ Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay
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- Geneaux, Romain (author)
- Univ Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay
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- Gentleman, Alexander S. (author)
- Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England.,University of Oxford
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- Guillemin, Renaud (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Goldsztejn, Gildas (author)
- Max Born Inst, D-12489 Berlin, Germany.;Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy,Paris-Sorbonne University
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- Holland, David M. P. (author)
- Daresbury Lab, Warrington WA4 4AD, Cheshire, England.,Daresbury Laboratory
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- Ismail, Iyas (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Journel, Loic (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Kierspel, Thomas (author)
- Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany.,University of Hamburg
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- Kuepper, Jochen (author)
- Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany.;Univ Hamburg, Ctr Ultrafast Imaging, D-22761 Hamburg, Germany.;Univ Hamburg, Dept Chem, D-20146 Hamburg, Germany.,University of Hamburg
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- Lahl, Jan (author)
- Lund University,Lunds universitet,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Mackenzie, Stuart R. (author)
- Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, Oxford OX1 3QZ, England.,University of Oxford
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- Maclot, Sylvain, 1986 (author)
- Lund University,Lunds universitet,Gothenburg University,Göteborgs universitet,Institutionen för fysik (GU),Department of Physics (GU),Lund Univ, Dept Phys, S-22100 Lund, Sweden.;Gothenburg Univ, Dept Phys, Box 100, S-40530 Gothenburg, Sweden.,Atomfysik,Fysiska institutionen,Institutioner vid LTH,Lunds Tekniska Högskola,Atomic Physics,Department of Physics,Departments at LTH,Faculty of Engineering, LTH
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- Manschwetus, Bastian (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Mereshchenko, Andrey S. (author)
- St Petersburg State Univ, St Petersburg 199034, Russia.,Saint Petersburg State University
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- Mullins, Terence (author)
- Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.
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- Olshin, Pavel K. (author)
- St Petersburg State Univ, St Petersburg 199034, Russia.,Saint Petersburg State University
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- Palaudoux, Jérôme (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,The French National Centre for Scientific Research (CNRS),Paris-Sorbonne University
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- Penent, Francis (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Piancastelli, Maria Novella (author)
- Uppsala University,Uppsala universitet,Kemisk och biomolekylär fysik,Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Rompotis, Dimitrios (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.,German Electron Synchrotron (DESY),European XFEL GmbH
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- Rouzee, Arnaud (author)
- Max Born Inst, D-12489 Berlin, Germany.,Max Born Institute for Nonlinear Optics and Short Pulse Spectroscopy
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- Ruchon, Thierry (author)
- Univ Paris Saclay, CEA, CNRS, LIDYL, F-91191 Gif Sur Yvette, France.,University of Paris-Saclay
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- Rudenko, Artem (author)
- Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
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- Schirmel, Nora (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Simon, Marc (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Techert, Simone (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.,German Electron Synchrotron (DESY)
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- Travnikova, Oksana (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Trippel, Sebastian (author)
- Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Ctr Ultrafast Imaging, D-22761 Hamburg, Germany.,University of Hamburg
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- Vallance, Claire (author)
- Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England.,University of Oxford
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- Wang, Enliang (author)
- Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
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- Wiese, Joss (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;Deutsch Elektronen Synchrotron DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany.;Univ Hamburg, Dept Chem, D-20146 Hamburg, Germany.,University of Hamburg
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- Ziaee, Farzaneh (author)
- Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
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- Marchenko, Tatiana (author)
- Sorbonne Univ, CNRS, Lab Chim Phys Matiere & Rayonnement, F-75005 Paris, France.,Paris-Sorbonne University
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- Rolles, Daniel (author)
- Kansas State Univ, Dept Phys, JR Macdonald Lab, Manhattan, KS 66506 USA.,Kansas State University
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- Boll, Rebecca (author)
- Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.;European XFEL, D-22869 Schenefeld, Germany.,German Electron Synchrotron (DESY),European XFEL GmbH
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Univ Oxford, Dept Chem, Chem Res Lab, Oxford OX1 3TA, England University of Oxford (creator_code:org_t)
- 2022-02-11
- 2022
- English.
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In: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS. - : IOP Publishing. - 0953-4075 .- 1361-6455. ; 55:1
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Abstract
Subject headings
Close
- The ultraviolet (UV)-induced dissociation and photofragmentation of gas-phase CH2BrI molecules induced by intense femtosecond extreme ultraviolet (XUV) pulses at three different photon energies are studied by multi-mass ion imaging. Using a UV-pump-XUV-probe scheme, charge transfer between highly charged iodine ions and neutral CH2Br radicals produced by C-I bond cleavage is investigated. In earlier charge-transfer studies, the center of mass of the molecules was located along the axis of the bond cleaved by the pump pulse. In the present case of CH2BrI, this is not the case, thus inducing a rotation of the fragment. We discuss the influence of the rotation on the charge transfer process using a classical over-the-barrier model. Our modeling suggests that, despite the fact that the dissociation is slower due to the rotational excitation, the critical interatomic distance for charge transfer is reached faster. Furthermore, we suggest that charge transfer during molecular fragmentation may be modulated in a complex way.
Subject headings
- NATURVETENSKAP -- Fysik -- Atom- och molekylfysik och optik (hsv//swe)
- NATURAL SCIENCES -- Physical Sciences -- Atom and Molecular Physics and Optics (hsv//eng)
Keyword
- free-electron lasers
- charge transfer
- ultrafast molecular dynamics
- free-electron lasers
Publication and Content Type
- ref (subject category)
- art (subject category)
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- By the author/editor
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Kockert, Hansjoc ...
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Lee, Jason W. L.
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Allum, Felix
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Amini, Kasra
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Bari, Sadia
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Bomme, Cedric
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show more...
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Brausse, Felix
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Brouard, Mark
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Burt, Michael
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de Miranda, Barb ...
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Duesterer, Stefa ...
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Eng-Johnsson, Pe ...
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Erk, Benjamin
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Geleoc, Marie
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Geneaux, Romain
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Gentleman, Alexa ...
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Guillemin, Renau ...
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Goldsztejn, Gild ...
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Holland, David M ...
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Ismail, Iyas
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Journel, Loic
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Kierspel, Thomas
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Kuepper, Jochen
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Lahl, Jan
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Mackenzie, Stuar ...
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Maclot, Sylvain, ...
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Manschwetus, Bas ...
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Mereshchenko, An ...
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Mullins, Terence
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Olshin, Pavel K.
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Palaudoux, Jérôm ...
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Penent, Francis
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Piancastelli, Ma ...
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Rompotis, Dimitr ...
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Rouzee, Arnaud
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Ruchon, Thierry
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Rudenko, Artem
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Schirmel, Nora
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Simon, Marc
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Techert, Simone
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Travnikova, Oksa ...
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Trippel, Sebasti ...
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Vallance, Claire
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Wang, Enliang
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Wiese, Joss
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Ziaee, Farzaneh
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Marchenko, Tatia ...
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Rolles, Daniel
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Boll, Rebecca
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- NATURAL SCIENCES
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NATURAL SCIENCES
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and Physical Science ...
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and Atom and Molecul ...
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JOURNAL OF PHYSI ...
- By the university
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University of Gothenburg
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Uppsala University
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Lund University